Reconciliation of local and long-range tilt correlations in underdoped La2-xBaxCuO4(0 ≤ x ≤ 0.155)

Bozin, Emil S.; Zhong, Ruidan; Knox, Kevin R.; Gu, Genda; Hill, John P.; Tranquada, John M.; Billinge, Simon J. L.

doi:10.1103/PhysRevB.91.054521

Title: Reconciliation of local and long-range tilt correlations in underdoped La_2-xBa_xCuO₄(0 ≤ x ≤ 0.155)

Journal Article · Thu Feb 26 00:00:00 EST 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.91.054521· OSTI ID:1182483

Bozin, Emil S. ^[1]; Zhong, Ruidan ^[2]; Knox, Kevin R. ^[1]; Gu, Genda ^[1]; Hill, John P. ^[1]; Tranquada, John M. ^[1]; Billinge, Simon J. L. ^[3]

Brookhaven National Lab. (BNL), Upton, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Stony Brook Univ., Stony Brook, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Columbia Univ., New York, NY (United States)

In this study, a long standing puzzle regarding the disparity of local and long range CuO₆ octahedral tilt correlations in the underdoped regime of La_2-xBa_xCuO₄ is addressed by utilizing complementary neutron powder diffraction and inelastic neutron scattering (INS) approaches. Long-range and static CuO₆ tilt order with orthogonally inequivalent Cu-O bonds in the CuO₂ planes in the low temperature tetragonal (LTT) phase is succeeded on warming through the low-temperature transition by one with orthogonally equivalent bonds in the low temperature orthorhombic (LTO) phase. In contrast, the signatures of LTT-type tilts in the instantaneous local atomic structure persist on heating throughout the LTO crystallographic phase on the nanoscale, although becoming weaker as temperature increases. Analysis of the INS spectra for the x = 1/8 composition reveals the dynamic nature of the LTT-like tilt fluctuations within the LTO phase and their 3D character. The doping dependence of relevant structural parameters indicates that the magnitude of the Cu-O bond anisotropy has a maximum at x = 1/8 doping were bulk superconductivity is most strongly suppressed, suggesting that the structural anisotropy might be influenced by electron-phonon coupling and the particular stability of the stripe-ordered phase at this composition. The bond-length modulation that pins stripe order is found to be remarkably subtle, with no anomalous bond length disorder at low temperature, placing an upper limit on any in-plane Cu-O bondlength anisotropy. The results further reveal that although appreciable octahedral tilts persist through the high-temperature transition and into the high temperature tetragonal (HTT) phase, there is no significant preference between different tilt directions in the HTT regime. This study also exemplifies the importance of a systematic approach using complementary techniques when investigating systems exhibiting a large degree of complexity and subtle structural responses.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC00112704; AC52-06NA25396

OSTI ID:: 1182483

Alternate ID(s):: OSTI ID: 1179936; OSTI ID: 1188211

Report Number(s):: BNL-107315-2014-JA; BNL-107646-2015-JA; PRBMDO; R&D Project: PM032; KC0202010

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 91, Issue 5; ISSN 1098-0121

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 24 works

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Staging superstructures in high- $T_{c}$ Sr/O codoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4 + y}$ Ray, P. J.; Andersen, N. H.; Jensen, T. B. S. Physical Review B, Vol. 96, Issue 17 https://doi.org/10.1103/physrevb.96.174106	journal	November 2017
Nematicity and Charge Order in Superoxygenated ${La}_{2 - x} {Sr}_{x} {CuO}_{4 + y}$ Zhang, Zhiwei; Sutarto, R.; He, F. Physical Review Letters, Vol. 121, Issue 6 https://doi.org/10.1103/physrevlett.121.067602	journal	August 2018
Unconventional Continuous Structural Disorder at the Order-Disorder Phase Transition in the Hexagonal Manganites Skjaervo, Sandra H.; Meier, Quintin N.; Feygenson, Mikhail ETH Zurich https://doi.org/10.3929/ethz-b-000353107	text	January 2019

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Title: Reconciliation of local and long-range tilt correlations in underdoped La_2-xBa_xCuO₄(0 ≤ x ≤ 0.155)