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Title: Milestone M4FT-13LL0807071: International Collaboration - Radionuclide Interactions and Transport in Geologic Repository Environments - Pu Interaction with Bentonite

Technical Report ·
DOI:https://doi.org/10.2172/1113367· OSTI ID:1113367
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  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

The focus of this project is to investigate radionuclide interactions with natural and engineered materials, specifically the mineral bentonite that will be used in EU repositories and possibly in US high-level waste repository designs. These experiments are designed to develop a mechanistic understanding of Pu interactions with representative mineral substrates under granitic chemical conditions. The sorption/desorption experiments cover a large range of Pu concentrations and will be compared to sorption/desorption experiment with montmorillonite. The experiments are being coordinated with the Colloid Formation and Migration (CFM) international project led by Karlsruhe Institute of Technology and located at the Grimsel Test Site underground research laboratory in Switzerland. Experiments will be completed by 8/15/2014. Milestone M4FT-13LL0807071 is a progress report on this effort. The research is addressing the following FEPs/needs identified in the R&D Roadmap: 2.2.09.05 - radionuclide speciation and solubility in host rock; 2.2.09.55 - sorption of dissolved radionuclides in host rock; 2.2.09.59 - colloidal transport in host rock.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
1113367
Report Number(s):
LLNL-TR-646168
Country of Publication:
United States
Language:
English