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  1. Measurements of the 96Zr(α,n) cross section for astrophysics and applications

    The reaction 96Zr(α,n) plays an important role in ν-driven wind nucleosynthesis in core-collapse supernovae and is a possible avenue for medical isotope production. Here, cross section measurements were performed using the activation technique at the Edwards Accelerator Laboratory. Results were analyzed along with world data on the 96Zr(α, n) cross section and 96Zr(α, α) differential cross section using large-scale Hauser-Feshbach calculations. We find general agreement between our data, previous measurements, and a statistical description of the reaction. However, we find a larger cross section at low energies compared to prior experimental results, allowing for a larger astrophysical reaction rate. Thismore » may impact results of core-collapse supernova ν-driven wind nucleosynthesis calculations, but does not significantly alter prior conclusions about 99Mo production for medical physics applications. The results from our large-scale Hauser-Feshbach calculations demonstrate that phenomenological optical potentials may yet be adequate to describe (α, n) reactions of interest for ν-driven wind nucleosynthesis, albeit with regionally-adjusted model parameters.« less
  2. Effect of radiation-induced defects on the superfluid density and optical conductivity of overdoped La 2 - x Sr x CuO 4

    Using a combination of time-domain THz spectroscopy (TDTS) and mutual inductance measurements, we have investigated the low-energy electrodynamic response of overdoped La$$_{2-x}$$Sr$$_x$$CuO$$_4$$ films that have been exposed to ion irradiation. Films went through three rounds of irradiation (2, 4, and 6 $$\times 10^{13}$$ ions/cm$^2$) and mututal inductance and TDTS experiments were performed between each step. Together with the as-grown film, this gives four different levels of disorder. The transport scattering rate that is measured directly in the THz experiments is an approximately linear function of the radiation dose at all temperatures. This is consistent with a proportionate increase in elasticmore » scattering from point-like 2D disorder. Here, in the superconducting state we find that the relation between T$$_c$$, the superfluid density, and the scattering rates are quantitatively at odds with the predictions based on the extant theory of Abrikosov-Gorkov-like pair breaking in a dirty d-wave superconductor. Increasing disorder causes only a small change in T$$_c$$ for the overdoped films, but the changes to the $$\omega \sim 0$$ superfluid density are much larger.« less
  3. Surface structures of L10-MnGa (001) by scanning tunneling microscopy and first-principles theory

    We report on the surface reconstructions of L10-ordered MnGa (001) thin films grown by molecular beam epitaxy on a 50 nm Mn3N2 (001) layer freshly grown on a magnesium oxide (001) substrate. Scanning tunneling microscopy, Auger electron spectroscopy, and reflection high energy electron diffraction, are combined with first-principles density functional theory calculations to determine the reconstructions of the L10-ordered MnGa (001) surface. We find two lowest energy reconstructions of the MnGa(001) face: a 1×1 Ga-terminated structure and a 1×2 structure with a Mn replacing a Ga in the 1×1 Ga-terminated surface. The 1×2 reconstruction forms a row structure along [100].more » The manganese:gallium stoichiometry within the surface based on the oretical modeling is in good agreement with experiment. Magnetic moment calculations for the two lowest energy structures reveal important surface and bulk effects leading to oscillatory total magnetization for ultra-thin MnGa(001) films.« less
  4. Structure and magnetism in Ga-rich MnGa/GaN thin films and unexpected giant perpendicular anisotropy in the ultra-thin film limit

    Here, we report structural, surface, and magnetic investigations of ferromagnetic Ga-rich MnGa thin and ultra-thin films grown on semiconducting GaN(0001) using molecular beam epitaxy. The Mn:Ga composition ratio is varied from ≈1 (stoichiometric) to ≈0.42 (very Ga-rich) for different samples. We find that the L10 MnGa phase is preserved down to a Mn:Ga ratio of ≈0.81. As the Ga concentration increases, we observe the coexistence of more Ga-rich phases, namely Mn3Ga5 and Mn2Ga5. Room temperature scanning tunneling microscopy imaging reveals highly epitaxial films, with atomically smooth and highly reconstructed surfaces. Magnetic characterizations show how the magnetic properties evolve with changingmore » composition and that giant perpendicular magnetic anisotropy is induced by reducing the size of our films.« less

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