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Title: New relaxation processes in diluted Ho2Ti2O7

Journal Article · · Physica B: Condensed Matter
OSTI ID:968620

We have studied the spin relaxation in diluted spin ice Ho{sub 2-x}R{sub x}Ti{sub 2}O{sub 7} (R = La or Y) by means of neutron scattering. Remarkably, doping with nonmagnetic ions does not relieve the geometrical frustration and the dynamics of the freezing is unaltered whilst the cubic unit cell is maintained. When the nonmagnetic substitution starts to distort the lattice, a new relaxation process is revealed. We present new data from several diluted spin ice samples where Arrhenius behavior observed in the parent compound, Ho{sub 2}Ti{sub 2}O{sub 7} is superseded by other processes including a quantum tunnelling process.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
DE-AC05-00OR22725
OSTI ID:
968620
Journal Information:
Physica B: Condensed Matter, Vol. 405, Issue 2
Country of Publication:
United States
Language:
English

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