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Title: Aerosol Single-Scattering Albedo and Asymmetry Parameter from MFRSR Observations during the ARM Aerosol IOP 2003

Multi-filter Rotating Shadowband Radiometers (MFRSRs) provide routine measurements of the aerosol optical depth ( << OLE Object: Microsoft Equation 3.0 >> ) at six wavelengths (0.415, 0.5, 0.615, 0.673, 0.870 and 0.94  << OLE Object: Picture (Metafile) >> ). The single-scattering albedo ( << OLE Object: Microsoft Equation 3.0 >> ) is typically estimated from the MFRSR measurements by assuming the asymmetry parameter ( << OLE Object: Microsoft Equation 3.0 >> ). In most instances, however, it is not easy to set an appropriate value of << OLE Object: Microsoft Equation 3.0 >> due to its strong temporal and spatial variability. Here, we introduce and validate an updated version of our retrieval technique that allows one to estimate simultaneously << OLE Object: Microsoft Equation 3.0 >> and << OLE Object: Microsoft Equation 3.0 >> for different types of aerosol. We use the aerosol and radiative properties obtained during the Atmospheric Science Program (ARM) Aerosol Intensive Operational Period (IOP) to validate our retrieval in two ways. First, the MFRSR-retrieved optical properties are compared with those obtained from independent surface, Aerosol Robotic Network (AERONET) and aircraft measurements. The MFRSR-retrieved optical properties are in reasonable agreement with these independent measurements. Second, we performmore » radiative closure experiments using the MFRSR-retrieved optical properties. The calculated broadband values of the direct and diffuse fluxes are comparable (~ 5 << OLE Object: Microsoft Equation 3.0 >> ) to those obtained from measurements.« less
Authors:
; ; ;
Publication Date:
OSTI Identifier:
910257
Report Number(s):
PNNL-SA-52291
KP1201030; TRN: US200723%%388
DOE Contract Number:
AC05-76RL01830
Resource Type:
Journal Article
Resource Relation:
Journal Name: Atmospheric Chemistry and Physics, 7(12):3341-3351; Journal Volume: 7; Journal Issue: 12
Research Org:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES; AEROSOLS; AIRCRAFT; ALBEDO; ASYMMETRY; OPTICAL PROPERTIES; RADIOMETERS; WAVELENGTHS; ATMOSPHERIC CHEMISTRY