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Title: Cross-flow, filter-sorbent catalyst for particulate, SO sub 2 and NO sub x control

Technical Report ·
DOI:https://doi.org/10.2172/7250477· OSTI ID:7250477

The objective of this program is to successfully carry out the experiment and design tasks described herein that will lead to the development a single-unit, cross flow filter-sorbent-catalyst. In the first stage of work we will investigate the SO{sub 2} removal and NO{sub x} reduction characteristics of different sorbent-catalyst compositions (in granular form), and we will conduct exploratory tests of cross-flow filters under conditions similar to those found in the combustion gases of small-scale combustors. In the second stage of the program, we will investigate the pollutant control characteristics of prototype filter-catalyst devices. The SO{sub 2} removal and NO{sub x} reduction efficiency of a unit-element' prototype will be investigated. This unit element' will be a slot reactor comprised of two flat porous walls, or slabs' of filter-sorbent-catalyst material separated by a 0.5 centimeter gap. The particulate collection efficiency and back-flushing requirements of a multi-element version of this device will be tested. A sorbent regeneration scheme will also be investigated. The sorbents under evaluation are: CuO, CeO{sub 2}, CuO-Al{sub 2}O{sub 3}, CeO{sub 2}-Al{sub 2}O{sub 3}, CuO-CeO{sub 2}, and CuO-CeO{sub 2}-Al{sub 2}O{sub 3}. Progress is described. 25 refs., 4 figs., 5 tabs.

Research Organization:
Little (Arthur D.), Inc., Cambridge, MA (United States)
Sponsoring Organization:
DOE/FE
DOE Contract Number:
AC22-89PC89805
OSTI ID:
7250477
Report Number(s):
DOE/PC/89805-T1; ADL-64303; ON: DE90008856
Country of Publication:
United States
Language:
English