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Title: High-field magnetoresistance of the Bechgaard salt (TMTSF)[sub 2]NO[sub 3]: Quantum oscillations in the spin-density-wave state and phase transitions

Journal Article · · Physical Review, B: Condensed Matter; (United States)
; ; ; ;  [1];  [2]
  1. Service National des Champs Magnetiques Pulses (CNRS-UMS 819), Laboratoire de Physique des Solides (CNRS URA 074), Complexe Scientifique de Rangueil, 31077 Toulouse (France)
  2. Laboratoire de Chimie Organique Structurale, Universite des Sciences et Techniques du Languedoc, place Eugene Bataillon, 34095 Montpellier Cedex 5 (France)

The transverse magnetoresistance of the Bechgaard salt (TMTSF)[sub 2]NO[sub 3] has been measured up to 37 T at ambient pressure in the temperature range from 2 to 77 K. When the magnetic field is parallel to the lowest conductivity direction [ital c][sup *] and for temperatures higher than [similar to]12 K, the data can be accounted for by a power law, the exponent of which decreases as the anion ordering takes place. At lower temperatures, the magnetic field increases the spin-density-wave (SDW) transition temperature, in overall agreement with theoretical predictions for the imperfect-nesting case. Two oscillation series, both linked to the SDW state, have been observed in the 2--10 K range. Their temperature-independent frequencies, measured from 2 to 8 K, are at (63[plus minus]2) and (248[plus minus]5) T, respectively. These oscillations have been studied (at 4.2 K) as a function of the field direction. They were found to deviate from the two-dimensional model since, in particular, their behavior differs according to whether the field is tilted on one side of the [ital c][sup *] direction or on the other. The oscillation data are discussed on the basis of recent calculations of Yakovenko.

DOE Contract Number:
W-7405-ENG-82
OSTI ID:
6903779
Journal Information:
Physical Review, B: Condensed Matter; (United States), Vol. 50:17; ISSN 0163-1829
Country of Publication:
United States
Language:
English