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Title: Integral-capture measurements and cross-section adjustments for Nd, Sm, and Eu

Technical Report ·
OSTI ID:6156066

Integral-capture reaction rates are reported for /sup 143/Nd, /sup 144/Nd, /sup 145/Nd, /sup 147/Sm, /sup 151/Eu, /sup 152/Eu, /sup 153/Eu, and /sup 154/Eu irradiated in different neutron spectra in EBR-II. These reaction rates are based primarily on mass-spectrometric measurements of the isotopic atom ratios of the capture product to the target nuclide. The neutron spectra are characterized using passive neutron dosimetry and spectrum-unfolding with the FERRET least-squares data analysis code. Reaction rates for the neutron spectrum monitors were determined by the radiometric technique using Ge(Li) spectrometers. These rates are also reported here. The integral data for the rare-earth samples and for the spectrum monitors were used in multigroup flux/cross-section adtustment analyses with FERRET to generate adjustments to 47 group representations of the ENDF/B-IV capture cross sections for the rare-earth isotopes. These adjusted cross sections are in good agreement with recent differential data and with adjusted cross sections based on STEK integral data. Examples are given of the use of the adjusted cross sections and covariance matrices for cross-section evaluation.

Research Organization:
EG and G Idaho, Inc., Idaho Falls (USA); Hanford Engineering Development Lab., Richland, WA (USA)
DOE Contract Number:
AC07-76ID01570
OSTI ID:
6156066
Report Number(s):
EGG-PHYS-5182; ON: DE81029635; TRN: 81-016306
Country of Publication:
United States
Language:
English