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Title: A neutron scintillator based on transparent nanocrystalline CaF{sub 2}:Eu glass ceramic

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4945999· OSTI ID:22591577
;  [1]; ;  [1]; ;  [2]; ;  [3]; ;  [4];  [5]
  1. Georgia Tech Research Institute, Georgia Institute of Technology, Atlanta, Georgia 30332 (United States)
  2. School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332 (United States)
  3. George W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332 (United States)
  4. Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6460 (United States)
  5. Forschungszentrum Jülich GmbH, Jülich 52425 (Germany)

There are no efficient Eu{sup 2+} doped glass neutron scintillators reported due to low doping concentrations of Eu{sup 2+} and the amorphous nature of the glass matrix. In this work, an efficient CaF{sub 2}:Eu glass ceramic neutron scintillator was prepared by forming CaF{sub 2}:Eu nanocrystals in a {sup 6}Li-containing glass matrix. Through appropriate thermal treatments, the scintillation light yield of the transparent glass ceramic was increased by a factor of at least 46 compared to the as-cast amorphous glass. This improvement was attributed to more efficient energy transfer from the CaF{sub 2} crystals to the Eu{sup 2+} emitting centers. Further light yield improvement is expected if the refractive index of the glass matrix can be matched to the CaF{sub 2} crystal.

OSTI ID:
22591577
Journal Information:
Applied Physics Letters, Vol. 108, Issue 15; Other Information: (c) 2016 Author(s); Country of input: International Atomic Energy Agency (IAEA); ISSN 0003-6951
Country of Publication:
United States
Language:
English

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