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Title: Modelling excitonic-energy transfer in light-harvesting complexes

Journal Article · · AIP Conference Proceedings
DOI:https://doi.org/10.1063/1.4861701· OSTI ID:22264079
 [1];  [2]
  1. Institut für Physik, Humboldt-Universität zu Berlin, Germany and Department of Physics, Harvard University (United States)
  2. Department of Chemistry and Chemical Biology, Harvard University (United States)

The theoretical and experimental study of energy transfer in photosynthesis has revealed an interesting transport regime, which lies at the borderline between classical transport dynamics and quantum-mechanical interference effects. Dissipation is caused by the coupling of electronic degrees of freedom to vibrational modes and leads to a directional energy transfer from the antenna complex to the target reaction-center. The dissipative driving is robust and does not rely on fine-tuning of specific vibrational modes. For the parameter regime encountered in the biological systems new theoretical tools are required to directly compare theoretical results with experimental spectroscopy data. The calculations require to utilize massively parallel graphics processor units (GPUs) for efficient and exact computations.

OSTI ID:
22264079
Journal Information:
AIP Conference Proceedings, Vol. 1575, Issue 1; Conference: Latin-American school of physics Marcos Moshinsky Elaf: Nonlinear dynamics in Hamiltonian systems, Mexico City (Mexico), 22 Jul - 2 Aug 2013; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0094-243X
Country of Publication:
United States
Language:
English