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Title: Nuclear spin conversion in diatomic molecules

A mechanism of the internal interaction in dimers that mixes different nuclear spin modifications has been proposed. It has been shown that the intramolecular current associated with transitions between electronic terms of different parities can generate different magnetic fields on nuclei, leading to transitions between spin modifications and to the corresponding changes in rotational states. In the framework of the known quantum relaxation process, this interaction initiates irreversible conversion of nuclear spin modifications. The estimated conversion rate for nitrogen at atmospheric pressure is quite high (10{sup -3}-10{sup -5} s{sup -1})
Authors:
;  [1]
  1. Russian Academy of Sciences, Institute of Automation and Electrometry, Siberian Branch (Russian Federation)
Publication Date:
OSTI Identifier:
22210556
Resource Type:
Journal Article
Resource Relation:
Journal Name: Journal of Experimental and Theoretical Physics; Journal Volume: 117; Journal Issue: 1; Other Information: Copyright (c) 2013 Pleiades Publishing, Ltd.; http://www.springer-ny.com; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; ATMOSPHERIC PRESSURE; CONVERSION; INTERACTIONS; MAGNETIC FIELDS; MODIFICATIONS; NITROGEN; NUCLEI; PARITY; RELAXATION; ROTATIONAL STATES; SPIN