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Title: Laser irradiation of carbon nanotube films: Effects and heat dissipation probed by Raman spectroscopy

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.4813485· OSTI ID:22122807
;  [1]; ;  [2]
  1. Instituto de Fisica 'Gleb Wataghin,' Unicamp, Campinas, 13083-859 Sao Paulo (Brazil)
  2. Centro de Componentes Semicondutores, Unicamp, Campinas, 13083-870 Sao Paulo (Brazil)

We investigate the thermal properties of thin films formed by single- and multi-walled carbon nanotubes submitted to laser irradiation using Raman scattering as a probe of both the tube morphology and the local temperature. The nanotubes were submitted to heating/cooling cycles attaining high laser intensities ({approx}1.4 MW/cm{sup 2}) under vacuum and in the presence of an atmosphere, with and without oxygen. We investigate the heat diffusion of the irradiated nanotubes to their surroundings and the effect of laser annealing on their properties. The presence of oxygen during laser irradiation gives rise to an irreversible increase of the Raman efficiency of the carbon nanotubes and to a remarkable increase of the thermal conductivity of multi-walled films. The second effect can be applied to design thermal conductive channels in devices based on carbon nanotube films using laser beams.

OSTI ID:
22122807
Journal Information:
Journal of Applied Physics, Vol. 114, Issue 2; Other Information: (c) 2013 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-8979
Country of Publication:
United States
Language:
English