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Title: Measurements of the mass and isotopic yields of the {sup 233}U(n{sub th},f) reaction at the Lohengrin spectrometer

Abstract

Over the last 10 years, a vast campaign of measurements has been initiated to improve the precision of neutron data for the involved key nuclei ({sup 232}Th, {sup 233}Pa and {sup 233}U) of the innovative Th -{sup 233}U cycle. This latter might indeed provide cleaner nuclear energy than the present U-Pu one. New measurements of charge and mass distributions of the fission products have been achieved at the Lohengrin spectrometer of the Inst. Laue-Langevin (ILL) during fall 2010 to complete the experimental data of {sup 233}U(n,f) that exist mainly for light fission fragments. That is why we performed measurements of mass and isotopic yields with a special focus on the heavy fission fragment part. Mass yields were measured by ion counting with an ionization chamber after separation by the Lohengrin spectrometer. Isotopic yields were derived from gamma spectrometry of mass-separated beams using HPGe clover detectors. This paper will present the results of these fission yield measurements along with details on the experimental set-up and the chosen analysis method. (authors)

Authors:
; ;  [1];  [2]; ; ; ;  [1];  [3];  [2]; ;  [4]; ;  [5];  [6];  [1];  [5];  [7]
  1. LPSC, UJF Grenoble 1, CNRS/IN2P3, Grenoble (France)
  2. IPN, CNRS/IN2P3, Univ. Paris-Sud (France)
  3. Dept. Chemical and Biological Sciences, Univ. Ruddersfield (United Kingdom)
  4. Institut Laue-Langevin, Grenoble (France)
  5. DSM/IRFU/SPhN, CEA Saclay (France)
  6. CENBG, Universite de Bordeaux 1 (France)
  7. DEN/DER/SPRC/LEPh, CEA Cadarache (France)
Publication Date:
OSTI Identifier:
22039866
Resource Type:
Conference
Resource Relation:
Conference: ANIMMA 2011: 2. International Conference on Advancements in Nuclear Instrumentation, Measurement Methods and their Applications, Ghent (Belgium), 6-9 Jun 2011; Other Information: Country of input: France; 17 refs.; IEEE Catalog Number: CFP1124I-CDR
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; 46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; ACCURACY; EXPERIMENTAL DATA; FISSION; FISSION FRAGMENTS; FISSION PRODUCTS; FISSION YIELD; GAMMA SPECTROSCOPY; HIGH-PURITY GE DETECTORS; IONIZATION CHAMBERS; MASS DISTRIBUTION; NUCLEAR DATA COLLECTIONS; PROTACTINIUM 233; SPECTROMETERS; THERMAL NEUTRONS; THORIUM 232; URANIUM 233

Citation Formats

Martin, F, Sage, C, Kessedjian, G, Bacri, C O, Bidaud, A, Billebaud, A, Capellan, N, Chabod, S, Cywinski, R, Doligez, X, Faust, H, Koester, U, Letourneau, A, Materna, T, Mathieu, L, Meplan, O, Panebianco, S, and Serot, O. Measurements of the mass and isotopic yields of the {sup 233}U(n{sub th},f) reaction at the Lohengrin spectrometer. United States: N. p., 2011. Web. doi:10.1109/ANIMMA.2011.6172920.
Martin, F, Sage, C, Kessedjian, G, Bacri, C O, Bidaud, A, Billebaud, A, Capellan, N, Chabod, S, Cywinski, R, Doligez, X, Faust, H, Koester, U, Letourneau, A, Materna, T, Mathieu, L, Meplan, O, Panebianco, S, & Serot, O. Measurements of the mass and isotopic yields of the {sup 233}U(n{sub th},f) reaction at the Lohengrin spectrometer. United States. https://doi.org/10.1109/ANIMMA.2011.6172920
Martin, F, Sage, C, Kessedjian, G, Bacri, C O, Bidaud, A, Billebaud, A, Capellan, N, Chabod, S, Cywinski, R, Doligez, X, Faust, H, Koester, U, Letourneau, A, Materna, T, Mathieu, L, Meplan, O, Panebianco, S, and Serot, O. 2011. "Measurements of the mass and isotopic yields of the {sup 233}U(n{sub th},f) reaction at the Lohengrin spectrometer". United States. https://doi.org/10.1109/ANIMMA.2011.6172920.
@article{osti_22039866,
title = {Measurements of the mass and isotopic yields of the {sup 233}U(n{sub th},f) reaction at the Lohengrin spectrometer},
author = {Martin, F and Sage, C and Kessedjian, G and Bacri, C O and Bidaud, A and Billebaud, A and Capellan, N and Chabod, S and Cywinski, R and Doligez, X and Faust, H and Koester, U and Letourneau, A and Materna, T and Mathieu, L and Meplan, O and Panebianco, S and Serot, O},
abstractNote = {Over the last 10 years, a vast campaign of measurements has been initiated to improve the precision of neutron data for the involved key nuclei ({sup 232}Th, {sup 233}Pa and {sup 233}U) of the innovative Th -{sup 233}U cycle. This latter might indeed provide cleaner nuclear energy than the present U-Pu one. New measurements of charge and mass distributions of the fission products have been achieved at the Lohengrin spectrometer of the Inst. Laue-Langevin (ILL) during fall 2010 to complete the experimental data of {sup 233}U(n,f) that exist mainly for light fission fragments. That is why we performed measurements of mass and isotopic yields with a special focus on the heavy fission fragment part. Mass yields were measured by ion counting with an ionization chamber after separation by the Lohengrin spectrometer. Isotopic yields were derived from gamma spectrometry of mass-separated beams using HPGe clover detectors. This paper will present the results of these fission yield measurements along with details on the experimental set-up and the chosen analysis method. (authors)},
doi = {10.1109/ANIMMA.2011.6172920},
url = {https://www.osti.gov/biblio/22039866}, journal = {},
number = ,
volume = ,
place = {United States},
year = {Fri Jul 01 00:00:00 EDT 2011},
month = {Fri Jul 01 00:00:00 EDT 2011}
}

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