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Title: Precursors for the Immobilization of Radioactive Cesium and Strontium from Spent Nuclear Fuel

Conference ·
OSTI ID:20979708
;  [1]
  1. Fuel Cycle and Materials Laboratory, Texas A and M University, College Station, TX 77843 (United States)

Next generation processes for the recycling of spent nuclear fuel are being developed by the US Department of Energy; this includes solvent extraction methods developed to isolate Cs and Sr fission products and immobilize them in a stable storage form. In this study, simulated (i.e., non-radioactive) cesium and strontium bearing liquid wastes were created and treated with carbon, silica, and alumina at 700 deg. C. The overall goal of this 2006 Nuclear Energy Research Initiative (NERI) project is to synthesize candidate ceramics for Cs and Sr storage and characterize their behavior. The initial results described here confirm the formation of stable compounds resembling strontianite (SrCO{sub 3}) and cesium-aluminosilicate (CsAlSi{sub 2}O{sub 4}). (authors)

Research Organization:
American Nuclear Society, 555 North Kensington Avenue, La Grange Park, IL 60526 (United States)
OSTI ID:
20979708
Resource Relation:
Conference: Advanced nuclear fuel cycles and systems (GLOBAL 2007), Boise - Idaho (United States), 9-13 Sep 2007; Other Information: Country of input: France; 7 refs; Related Information: In: Proceedings of GLOBAL 2007 conference on advanced nuclear fuel cycles and systems, 1873 pages.
Country of Publication:
United States
Language:
English