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Title: Strain-Driven Approach to Quantum Criticality in AFe2As2 with A=K, Rb, and Cs

Journal Article · · Physical Review Letters
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  1. Karlsruhe Inst. of Technology (KIT) (Germany). Inst. fur Technologie
  2. Karlsruher Institut fur Technologie, Germany
  3. Renmin Univ. of China, Beijing (China). Dept. of Physics
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  5. Rice Univ., Houston, TX (United States). Dept. of Physics and Astronomy
  6. Univ. of Tokyo (Japan). Dept. of Advanced Materials Science; Kyoto Univ. (Japan). Dept. of Physics
  7. Karlsruhe Inst. of Technology (KIT) (Germany). Inst. fur Technologie; Karlsruhe Inst. of Technology (KIT) (Germany). Physikalisches Inst.

The iron-based superconductors AFe2As2 with A = K, Rb, Cs exhibit large Sommerfeld coefficients approaching those of heavy-fermion systems. We have investigated the magnetostriction and thermal expansion of this series to shed light on this unusual behavior. Quantum oscillations of the magnetostriction allow identifying the band-specific quasiparticle masses which by far exceed the band-structure derived masses. The divergence of the Grüneisen ratio derived from thermal expansion indicates that with increasing volume along the series a quantum critical point is approached. In conclusion, the critical fluctuations responsible for the enhancement of the quasiparticle masses appear to weaken the superconducting state.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); National Science Foundation of China
Grant/Contract Number:
AC52-06NA25396; 11374361; C-1411; PHY-1066293
OSTI ID:
1414118
Alternate ID(s):
OSTI ID: 1256164
Report Number(s):
LA-UR-15-28161; TRN: US1800644
Journal Information:
Physical Review Letters, Vol. 116, Issue 23; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 42 works
Citation information provided by
Web of Science

References (57)

Electronic specific heat of Ba 1 x K x Fe 2 As 2 from 2 to 380 K journal October 2013
Nodal gap in iron-based superconductor CsFe 2 As 2 probed by quasiparticle heat transport journal April 2013
Phonons in doped and undoped BaFe 2 As 2 investigated by inelastic x-ray scattering journal December 2009
Evolution from non-Fermi- to Fermi-liquid transport via isovalent doping in BaFe 2 ( As 1 x P x ) 2 superconductors journal May 2010
Magnetic Oscillations in Metals book October 2011
Orbital-dependent effects of electron correlations in microscopic models for iron-based superconductors journal April 2013
wannier90: A tool for obtaining maximally-localised Wannier functions journal May 2008
A Quantum Critical Point Lying Beneath the Superconducting Dome in Iron Pnictides journal March 2014
Universal Heat Conduction in the Iron Arsenide Superconductor KFe 2 As 2 : Evidence of a d -Wave State journal August 2012
Quantum criticality in the iron pnictides and chalcogenides journal May 2011
Orbital-Selective Mott Phase in Multiorbital Models for Alkaline Iron Selenides K 1 x Fe 2 y Se 2 journal April 2013
Maximally localized generalized Wannier functions for composite energy bands journal November 1997
Heat transport in RbFe 2 As 2 single crystals: Evidence for nodal superconducting gap journal January 2015
Fermi Surface of KFe 2 As 2 from Quantum Oscillations in Magnetostriction conference June 2014
Near-degeneracy of several pairing channels in multiorbital models for the Fe pnictides journal February 2009
Pressure and chemical substitution effects in the local atomic structure of BaFe 2 As 2 journal May 2011
Calorimetric study of single-crystal CsFe 2 As 2 journal June 2013
Spin fluctuations and superconductivity in a three-dimensional tight-binding model for BaFe 2 As 2 journal June 2010
Orbital character and electron correlation effects on two- and three-dimensional Fermi surfaces in KFe2As2 revealed by angle-resolved photoemission spectroscopy journal April 2014
Iron pnictides as a new setting for quantum criticality journal March 2009
Sign change of the Grüneisen parameter and magnetocaloric effect near quantum critical points journal November 2005
Local Quantum Criticality of an Iron-Pnictide Tetrahedron journal March 2012
Upper critical field of K Fe 2 As 2 under pressure: A test for the change in the superconducting gap structure journal June 2014
Pauli-Limited Multiband Superconductivity in KFe 2 As 2 journal August 2013
Self-consistent d x 2 - y 2 pairing in a two-dimensional Hubbard model journal March 1994
Spin fluctuations and high temperature superconductivity journal July 2000
Chemical Pressure and Physical Pressure in BaFe 2 (As 1- x P x ) 2 journal December 2010
Selective Mott Physics as a Key to Iron Superconductors journal April 2014
Superconductivity-induced re-entrance of the orthorhombic distortion in Ba1−xKxFe2As2 journal July 2015
Electronic structure in a one-Fe Brillouin zone of the iron pnictide superconductors CsFe 2 As 2 and RbFe 2 As 2 journal November 2015
Universally Diverging Grüneisen Parameter and the Magnetocaloric Effect Close to Quantum Critical Points journal August 2003
U ( 1 ) slave-spin theory and its application to Mott transition in a multiorbital model for iron pnictides journal August 2012
Site specific spin dynamics in BaFe2As2: tuning the ground state by orbital differentiation journal October 2014
Wien2wannier: From linearized augmented plane waves to maximally localized Wannier functions journal November 2010
Fermi surface in KFe 2 As 2 determined via de Haas–van Alphen oscillation measurements journal June 2013
Measurement of Anomalous Phonon Dispersion of CaFe 2 As 2 Single Crystals Using Inelastic Neutron Scattering journal May 2009
Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides journal September 2011
High-temperature superconductivity stabilized by electron-hole interband coupling in collapsed tetragonal phase of KFe 2 As 2 under high pressure journal February 2015
Quasiparticle Mass Enhancement Close to the Quantum Critical Point in BaFe 2 ( As 1 x P x ) 2 journal June 2013
Pressure versus Concentration Tuning of the Superconductivity in Ba(Fe 1- x Co x ) 2 As 2 journal December 2010
Single 20 meV boson mode in KFe 2 As 2 detected by point-contact spectroscopy journal September 2014
Strong Correlations from Hund’s Coupling journal April 2013
Strong Pauli-limiting behavior of H c 2 and uniaxial pressure dependencies in KFe 2 As 2 journal July 2013
Evidence of Strong Correlations and Coherence-Incoherence Crossover in the Iron Pnictide Superconductor KFe 2 As 2 journal July 2013
Linear response in a density-functional mixed-basis approach journal August 1999
Microscopic nature of correlations in multiorbital A Fe 2 As 2 ( A = K , Rb , Cs ) : Hund's coupling versus Coulomb repulsion journal November 2015
Maximally localized Wannier functions for entangled energy bands journal December 2001
Sudden reversal in the pressure dependence of T c in the iron-based superconductor CsFe 2 As 2 : A possible link between inelastic scattering and pairing symmetry journal April 2014
Octet-Line Node Structure of Superconducting Order Parameter in KFe2As2 journal September 2012
Chemical Pressure and Physical Pressure in BaFe_2(As_{1-x}P_{x})_2 text January 2010
Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides text January 2011
U(1) Slave-spin theory and its application to Mott transition in a multi-orbital model for iron pnictides text January 2012
Quantum critical point lying beneath the superconducting dome in iron-pnictides text January 2013
Orbital-dependent effects of electron correlations in microscopic models for iron-based superconductors text January 2013
Site specific spin dynamics in BaFe2As2: tuning the ground state by orbital differentiation preprint January 2014
Maximally-localized Wannier functions for entangled energy bands text January 2001
Sign change of the Grueneisen parameter and magnetocaloric effect near quantum critical points text January 2005

Cited By (8)

Evidence of nematic order and nodal superconducting gap along [110] direction in RbFe2As2 journal March 2019
Reciprocity between local moments and collective magnetic excitations in the phase diagram of BaFe2(As1−xPx)2 journal November 2019
Novel electronic nematicity in heavily hole-doped iron pnictide superconductors journal March 2020
Putative hybridization gap in CaMn 2 Bi 2 under applied pressure journal July 2019
Broken mirror symmetry, incommensurate spin correlations, and B 2 g nematic order in iron pnictides journal September 2019
Strong correlations, strong coupling, and s -wave superconductivity in hole-doped BaFe 2 As 2 single crystals journal November 2016
Non-trivial role of interlayer cation states in iron-based superconductors text January 2016
Evidence of nematic order and nodal superconducting gap along [110] direction in RbFe2As2 text January 2018

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