Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells

Chen, Bo; Bai, Yang; Yu, Zhengshan; Li, Tao; Zheng, Xiaopeng; Dong, Qingfeng; Shen, Liang; Boccard, Mathieu; Gruverman, Alexei; Holman, Zachary; Huang, Jinsong

doi:10.1002/aenm.201601128

Title: Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells

Journal Article · Tue Jul 19 00:00:00 EDT 2016 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201601128· OSTI ID:1342622

Chen, Bo ^[1]; Bai, Yang ^[1]; Yu, Zhengshan ^[2]; Li, Tao ^[1]; Zheng, Xiaopeng ^[1]; Dong, Qingfeng ^[1]; Shen, Liang ^[1]; Boccard, Mathieu ^[2]; Gruverman, Alexei ^[1]; Holman, Zachary ^[2]; Huang, Jinsong ^[1]

Univ. of Nebraska-Lincoln, Lincoln, NE (United States)
Arizona State Univ., Tempe, AZ (United States)

Here, we have investigated semi-transparent perovskite solar cells and infrared enhanced silicon heterojunction cells for high-efficiency tandem devices. A semi-transparent metal electrode with good electrical conductivity and optical transparency has been fabricated by thermal evaporation of 7 nm of Au onto a 1-nm-thick Cu seed layer. For this electrode to reach its full potential, MAPbI3 thin films were formed by a modified one-step spin-coating method, resulting in a smooth layer that allowed the subsequent metal thin film to remain continuous. The fabricated semi-transparent perovskite solar cells demonstrated 16.5% efficiency under one-sun illumination, and were coupled with infrared-enhanced silicon heterojunction cells tuned specifically for perovskite/Si tandem devices. A double-layer antireflection coating at the front side and MgF2 reflector at rear side of the silicon heterojunction cells reduced parasitic absorption of near-infrared light, leading to 6.5% efficiency after filtering with a perovskite device and 23.0% summed efficiency for the perovskite/Si tandem device.

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Research Organization:: Univ. of Nebraska, Lincoln, NE (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office

Grant/Contract Number:: EE0006709; EE0006335; DE‐EE0006709

OSTI ID:: 1342622

Alternate ID(s):: OSTI ID: 1400993

Journal Information:: Advanced Energy Materials, Vol. 6, Issue 19; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 232 works

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Title: Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells

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