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Title: Influence of interfacial coherency on ferroelectric switching of superlattice BaTiO3/SrTiO3

Switching behavior of (BaTiO3)8/ (SrTiO3)4 heterostructure superlattice grown on SrTiO3 substrate was studied by employing the phase field method. To investigate the constraint effect of the substrate on switching, three types of superlattice/substrate interface mechanical relaxation conditions were considered, i.e. the fully ommensurate, partially relaxed and fully relaxed. Our simulation results demonstrated that the hysteresis loops under the three types of constraints were very different. The interfacial coherency affects dramatically the coercivity and remanence of the superlattice films. The mechanism of the hysteresis loop varying with interfacial coherency was analyzed by the ferroelectric domain configuration and its evolution during the switching process. The hysteresis loop of fully relaxed superlattice shows application potential on ferroelectric energy storage materials.
Authors:
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Publication Date:
OSTI Identifier:
1274891
Report Number(s):
PNNL-SA-106498
Journal ID: ISSN 0003-6951
DOE Contract Number:
AC05-76RL01830
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 107; Journal Issue: 12
Publisher:
American Institute of Physics (AIP)
Research Org:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
superlattice; Switching; Constraint effect; Phase field method