Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11

Rau, J. G.; Wu, L. S.; May, A. F.; Poudel, L.; Winn, B.; Garlea, V. O.; Huq, A.; Whitfield, P.; Taylor, A. E.; Lumsden, M. D.; Gingras, M. J.  P.; Christianson, A. D.

doi:10.1103/PhysRevLett.116.257204

Title: Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$

Journal Article · Fri Jun 24 00:00:00 EDT 2016 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.116.257204· OSTI ID:1260086

Rau, J. G. ^[1]; Wu, L. S. ^[2]; May, A. F. ^[3]; Poudel, L. ^[4]; Winn, B. ^[2]; Garlea, V. O. ^[2]; Huq, A. ^[5]; Whitfield, P. ^[5]; Taylor, A. E. ^[2]; Lumsden, M. D. ^[2]; Gingras, M. J. P. ^[6]; Christianson, A. D. ^[4]

Univ. of Waterloo, ON (Canada)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division; Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical and Engineering Materials Division
Univ. of Waterloo, ON (Canada); Perimeter Inst. for Theoretical Physics, Waterloo, ON (Canada)

The low energy spin excitation spectrum of the breathing pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$ has been investigated with inelastic neutron scattering. Several nearly resolution limited modes with no observable dispersion are observed at 250 mK while, at elevated temperatures, transitions between excited levels become visible. To gain deeper insight, a theoretical model of isolated Yb³⁺ tetrahedra parametrized by four anisotropic exchange constants is constructed. The model reproduces the inelastic neutron scattering data, specific heat, and magnetic susceptibility with high fidelity. The fitted exchange parameters reveal a Heisenberg antiferromagnet with a very large Dzyaloshinskii-Moriya interaction. Ultimately, using this model, we predict the appearance of an unusual octupolar paramagnet at low temperatures and speculate on the development of inter-tetrahedron correlations.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1260086

Alternate ID(s):: OSTI ID: 1259338

Journal Information:: Physical Review Letters, Vol. 116, Issue 25; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment Tarjus, G.; Kivelson, S. A.; Nussinov, Z. arXiv https://doi.org/10.48550/arxiv.cond-mat/0509127	text	January 2005

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Title: Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$