Influence of air mass origin on aerosol properties at a remote Michigan forest site
- Washington State Univ., Pullman, WA (United States)
- Washington State Univ., Pullman, WA (United States); African Centre for Technology Studies, Nairobi (Kenya)
- Washington State Univ., Pullman, WA (United States); Rice Univ., Houston, TX (United States)
- Washington State Univ., Pullman, WA (United States); Houston Advanced Research Center, The Woodlands, TX (United States)
The northern Great Lakes region of North America is a large, relatively pristine area. To date, there has only been limited study of the atmospheric aerosol in this region. During summer 2009, a detailed characterization of the atmospheric aerosol was conducted at the University of Michigan Biological Station (UMBS) as part of the Community Atmosphere–Biosphere Interactions Experiment (CABINEX). Measurements included particle size distribution, water-soluble composition, and CCN activity. Aerosol properties were strongly dependent on the origin of the air masses reaching the site. For ~60% of the study period, air was transported from sparsely populated regions to the northwest. During these times aerosol loadings were low, with mean number and volume concentrations of 1630 cm-3 and 1.91 μm3 cm-3, respectively. The aerosol during clean periods was dominated by organics, and exhibited low hygroscopicities (mean κ = 0.18 at s = 0.3%). When air was from more populated regions to the east and south (~29% of the time), aerosol properties reflected a stronger anthropogenic influence, with 85% greater particle number concentrations, 2.5 times greater aerosol volume, six times more sulfate mass, and increased hygroscopicity (mean к = 0.24 at s = 0.3%). Furthermore, these trends are have the potential to influence forest–atmosphere interactions and should be targeted for future study.
- Research Organization:
- Washington State Univ., Pullman, WA (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC)
- Grant/Contract Number:
- SC0003899
- OSTI ID:
- 1353457
- Alternate ID(s):
- OSTI ID: 1250952
- Journal Information:
- Atmospheric Environment (1994), Vol. 107, Issue C; ISSN 1352-2310
- Publisher:
- ElsevierCopyright Statement
- Country of Publication:
- United States
- Language:
- English
Web of Science
Ubiquitous influence of wildfire emissions and secondary organic aerosol on summertime atmospheric aerosol in the forested Great Lakes region
|
journal | January 2018 |
Differences in BVOC oxidation and SOA formation above and below the forest canopy
|
journal | January 2017 |
Ubiquitous Influence of Wildfire Emissions and Secondary Organic Aerosol on Summertime Atmospheric Aerosol in the Forested Great Lakes Region
|
journal | March 2018 |
Similar Records
Long-term observations of cloud condensation nuclei over the Amazon rain forest - Part 2: Variability and characteristics of biomass burning, long-range transport, and pristine rain forest aerosols
CCN activity and organic hygroscopicity of aerosols downwind of an urban region in central Amazonia: seasonal and diel variations and impact of anthropogenic emissions