Using nonequilibrium dynamics to probe competing orders in a Mott-Peierls system

Wang, Y.; Moritz, B.; Chen, C. -C.; Jia, C. J.; van Veenendaal, M.; Devereaux, T. P.

doi:10.1103/PhysRevLett.116.086401

Title: Using nonequilibrium dynamics to probe competing orders in a Mott-Peierls system

Journal Article · Wed Feb 24 00:00:00 EST 2016 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.116.086401· OSTI ID:1245833

Wang, Y. ^[1]; Moritz, B. ^[2]; Chen, C. -C. ^[3]; Jia, C. J. ^[4]; van Veenendaal, M. ^[5]; Devereaux, T. P. ^[6]

Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. of North Dakota, Grand Forks, ND (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Argonne National Lab. (ANL), Argonne, IL (United States); Northern Illinois Univ., DeKalb, IL (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)

Competition between ordered phases, and their associated phase transitions, are significant in the study of strongly correlated systems. Here, we examine one aspect, the nonequilibrium dynamics of a photoexcited Mott-Peierls system, using an effective Peierls-Hubbard model and exact diagonalization. Near a transition where spin and charge become strongly intertwined, we observe antiphase dynamics and a coupling-strength-dependent suppression or enhancement in the static structure factors. The renormalized bosonic excitations coupled to a particular photoexcited electron can be extracted, which provides an approach for characterizing the underlying bosonic modes. The results from this analysis for different electronic momenta show an uneven softening due to a stronger coupling near k_F. As a result, this behavior reflects the strong link between the fermionic momenta, the coupling vertices, and ultimately, the bosonic susceptibilities when multiple phases compete for the ground state of the system.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; AC02-76SF00515; AC02-05CH11231; FG02-03ER46097; SC0007091

OSTI ID:: 1245833

Alternate ID(s):: OSTI ID: 1239440; OSTI ID: 1257729

Report Number(s):: SLAC-PUB-16569; 125920

Journal Information:: Physical Review Letters, Vol. 116, Issue 8; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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