Chemistry of Atmospheric Brown Carbon

Laskin, Alexander; Laskin, Julia; Nizkorodov, Sergey A.

doi:10.1021/cr5006167

Title: Chemistry of Atmospheric Brown Carbon

Journal Article · Thu Feb 26 00:00:00 EST 2015 · Chemical Reviews

DOI:https://doi.org/10.1021/cr5006167· OSTI ID:1240470

Laskin, Alexander; Laskin, Julia; Nizkorodov, Sergey A. ^[1]

Department of Chemistry, University of California, Irvine, Irvine, California 92697, United States

Organic carbon (OC) accounts for a large fraction of atmospheric aerosol and has profound effects on air quality, atmospheric chemistry and climate forcing. Molecular composition of the OC and its evolution during common processes of atmospheric aging have been a subject of extensive research over the last decade (see reviews of Ervens et al.,1 Hallquist et al.,2 Herckes et al.,3 Carlton et al.,4 Kroll and Seinfeld,5 Rudich et al.,6 and Kanakidou et al.7). Even though many fundamental advances have been reported in these studies, our understanding of the climate-related properties of atmospheric OC is still incomplete and the specific ways in which OC impacts atmospheric environment and climate forcing are just beginning to be understood. This review covers one topic of particular interest in this area –environmental chemistry of light-absorbing aerosol OC and its impact on radiative forcing.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States). Environmental Molecular Sciences Laboratory (EMSL)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1240470

Alternate ID(s):: OSTI ID: 1184286

Report Number(s):: PNNL-SA-106070

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Vol. 115 Journal Issue: 10; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 927 works

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Long term measurements of aerosol optical properties at a primary forest site in Amazonia Rizzo, L. V.; Artaxo, P.; Müller, T. Atmospheric Chemistry and Physics, Vol. 13, Issue 5 https://doi.org/10.5194/acp-13-2391-2013	journal	January 2013
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Characterizing an Extractive Electrospray Ionization (EESI) Source for the Online Mass Spectrometry Analysis of Organic Aerosols Gallimore, Peter J.; Kalberer, Markus Environmental Science & Technology, Vol. 47, Issue 13, p. 7324-7331 https://doi.org/10.1021/es305199h	journal	June 2013
Yellow Beads and Missing Particles: Trouble Ahead for Filter-Based Absorption Measurements Subramanian, R.; Roden, Christoph A.; Boparai, Poonam Aerosol Science and Technology, Vol. 41, Issue 6 https://doi.org/10.1080/02786820701344589	journal	May 2007
Brown Carbon Formation by Aqueous-Phase Carbonyl Compound Reactions with Amines and Ammonium Sulfate Powelson, Michelle H.; Espelien, Brenna M.; Hawkins, Lelia N. Environmental Science & Technology, Vol. 48, Issue 2 https://doi.org/10.1021/es4038325	journal	December 2013
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Organic aerosol formation photo-enhanced by the formation of secondary photosensitizers in aerosols Aregahegn, Kifle Z.; Nozière, Barbara; George, Christian Faraday Discussions, Vol. 165 https://doi.org/10.1039/c3fd00044c	journal	January 2013
Speciation of Gas-Phase and Fine Particle Emissions from Burning of Foliar Fuels Hays, Michael D.; Geron, Christopher D.; Linna, Kara J. Environmental Science & Technology, Vol. 36, Issue 11 https://doi.org/10.1021/es0111683	journal	June 2002
Chemical characterisation of semi-volatile and aerosol compounds from the photooxidation of toluene and NOx White, Stephen J.; Jamie, Ian M.; Angove, Dennys E. Atmospheric Environment, Vol. 83 https://doi.org/10.1016/j.atmosenv.2013.11.023	journal	February 2014
Characterization of a humic acid-like brown substance in airborne particulate matter and tentative identification of its origin Mukai, Hitoshi; Ambe, Yoshinari Atmospheric Environment (1967), Vol. 20, Issue 5 https://doi.org/10.1016/0004-6981(86)90265-9	journal	January 1986
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Light-absorbing carbon in Europe – measurement and modelling, with a focus on residential wood combustion emissions Genberg, J.; Denier van der Gon, H. A. C.; Simpson, D. Atmospheric Chemistry and Physics, Vol. 13, Issue 17 https://doi.org/10.5194/acp-13-8719-2013	journal	January 2013
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