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Title: Distribution of neptunium and plutonium in New Mexico lichen samples ( Usnea arizonica) contaminated by atmospheric fallout

In this study, the concentrations of 237Np, 239Pu and 240Pu were determined in lichen samples ( Usnea arizonica) that were collected from ten locations in New Mexico between 2011 and 2013 using isotope dilution inductively-coupled plasma mass spectrometry (ID-ICP-MS). The observed isotopic ratios for 237Np/ 239Pu and 240Pu/ 239Pu indicate trace contamination from global and regional fallout (e.g. Trinity test and atmospheric testing at the Nevada Test Site). The fact that actinide contamination is detected in recent lichen collections suggests continuous re-suspension of fallout radionuclides even 50 years after ratification of the Limited Test Ban Treaty.
 [1] ;  [1] ;  [2] ;  [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Univ. of Cincinnati, Cincinnati, OH (United States)
Publication Date:
OSTI Identifier:
Report Number(s):
Journal ID: ISSN 0236-5731; PII: 4402
Grant/Contract Number:
20120459ER; AC52-06NA25396
Accepted Manuscript
Journal Name:
Journal of Radioanalytical and Nuclear Chemistry
Additional Journal Information:
Journal Name: Journal of Radioanalytical and Nuclear Chemistry; Journal ID: ISSN 0236-5731
Research Org:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org:
Country of Publication:
United States
54 ENVIRONMENTAL SCIENCES; Neptunium-237; Plutonium isotopes; atmospheric fallout; ICP-MS lichen