Field-induced spin density wave and spiral phases in a layered antiferromagnet

Stone, Matthew B.; Lumsden, Mark D.; Garlea, Vasile O.; Grenier, B.; Ressouche, E.; Samulon, Eric C.; Fisher, Ian R.

doi:10.1103/PhysRevB.92.020415

Title: Field-induced spin density wave and spiral phases in a layered antiferromagnet

Journal Article · Tue Jul 28 00:00:00 EDT 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.92.020415· OSTI ID:1210151

Stone, Matthew B. ^[1]; Lumsden, Mark D. ^[1]; Garlea, Vasile O. ^[1]; Grenier, B. ^[2]; Ressouche, E. ^[2]; Samulon, Eric C. ^[3]; Fisher, Ian R. ^[3]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
Alternative Energies and Atomic Energy Commission (CEA), Grenoble (France). Inst. on Nanoscience and Cryogenics (INAC) and Statistical Physics, Magnetism and Superconductivity (SPSMS)
Stanford Univ., CA (United States). Dept. of Applied Physics and Geballe Lab. for Advanced Materials

In this study, we determine the low-field ordered magnetic phases of the S=1 dimerized antiferromagnet Ba₃Mn₂O₈ using single-crystal neutron diffraction. We find that for magnetic fields between μ₀H=8.80T and 10.56T applied along the [110] direction the system exhibits spin density wave order with incommensurate wave vectors of type (η,η,ε). For μ₀H>10.56T, the magnetic order changes to a spiral phase with incommensurate wave vectors only along the [hh0] direction. For both field-induced ordered phases, the magnetic moments are lying in the plane perpendicular to the field direction. The nature of these two transitions is fundamentally different: the low-field transition is a second-order transition to a spin density wave ground state, while the one at higher field, toward the spiral phase, is of first order.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: AC05-00OR22725; DMR-1205165; DMR-0454672

OSTI ID:: 1210151

Alternate ID(s):: OSTI ID: 1203817; OSTI ID: 1327631

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 92, Issue 2; ISSN 1098-0121

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1 work

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