Gas phase heterogeneous catalytic oxidation of alkanes to aliphatic ketones and/or other oxygenates

Lin, Manhua; Wang, Xiang; Yeom, Younghoon

Title: Gas phase heterogeneous catalytic oxidation of alkanes to aliphatic ketones and/or other oxygenates

Patent · Tue Mar 17 00:00:00 EDT 2015

OSTI ID:1172752

Lin, Manhua; Wang, Xiang; Yeom, Younghoon

A catalyst, its method of preparation and its use for producing aliphatic ketones by subjecting alkanes C.sub.3 to C.sub.9 to a gas phase catalytic oxidation in the presence of air or oxygen, and, optionally, steam and/or one or more diluting gases. The catalyst comprises a catalytically active mixed metal oxide phase and a suitable support material onto and/or into which the active catalytic phase id dispersed.

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Research Organization:: Ever Nu Technology, LLC, Warminster, PA (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: FG02-03ER83652

Assignee:: Ever Nu Technology, LLC (Warminster, PA)

Patent Number(s):: 8,981,157

Application Number:: 14/116,424

OSTI ID:: 1172752

Resource Relation:: Patent File Date: 2012 May 09

Country of Publication:: United States

Language:: English

References (13)

Cyclohexane oxidation continues to be a challenge Schuchardt, Ulf; Cardoso, Dilson; Sercheli, Ricardo Applied Catalysis A: General, Vol. 211, Issue 1, p. 1-17 https://doi.org/10.1016/S0926-860X(01)00472-0	journal	March 2001
VPO catalyst for n-butane oxidation to maleic anhydride: A goal achieved, or a still open challenge? Ballarini, N.; Cavani, F.; Cortelli, C. Topics in Catalysis, Vol. 38, Issue 1-3 https://doi.org/10.1007/s11244-006-0080-z	journal	July 2006
Cyclohexane oxidation and carbon deposition over metal oxide catalysts Hettige, C.; Mahanama, K. R. R.; Dissanayake, D. P. Chemosphere, Vol. 43, Issue 8, p. 1079-1083 https://doi.org/10.1016/S0045-6535(00)00195-8	journal	June 2001
Vapor-Phase Air Oxidation of Cyclohexane Hoot, William F.; Kobe, Kenneth A. Industrial & Engineering Chemistry, Vol. 47, Issue 4 https://doi.org/10.1021/ie50544a037	journal	April 1955
Cyclohexane oxidation over Cu₂O–CuO and CuO thin films deposited by CVD process on fiberglass Medina-Valtierra, Jorge; Ramı́rez-Ortiz, Jorge; Arroyo-Rojas, Victor M Applied Catalysis A: General, Vol. 238, Issue 1, p. 1-9 https://doi.org/10.1016/S0926-860X(02)00074-1	journal	January 2003
Why is it Interesting to Study Cyclohexane Oxidation? Schuchardt, Ulf; Carvalho, Wagner Alves; Spinacé, Estevam Vitorio Synlett, Vol. 1993, Issue 10 https://doi.org/10.1055/s-1993-22583	journal	January 1993
Aerobic oxidation of cyclohexane by gold nanoparticles immobilized upon mesoporous silica Zhu, Kake; Hu, Juncheng; Richards, Ryan Catalysis Letters, Vol. 100, Issue 3-4 https://doi.org/10.1007/s10562-004-3454-5	journal	April 2005
Method for producing an unsaturated carboxylic acid Ushikubo, Takashi; Nakamura, Hiroya; Koyasu, Yukio https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/5380933 US Patent Document 5,380,933	patent	January 1995
Molybdenum promoted vanadium-antimony-oxide based catalyst for selective paraffin ammoxidation Brazdil, James F.; Toft, Mark A. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6156920 US Patent Document 6,156,920	patent	December 2000
Method for producing an oxide catalyst for use in producing acrylonitrile or methacrylonitrile from propane or isobutane Inoue, Tomoya; Ishida, Hiroshi https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6514902 US Patent Document 6,514,902	patent	February 2003
Process for preparing a catalyst Lin, Manhua; Linsen, Michael https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6514903 US Patent Document 6,514,903	patent	February 2003
Selective oxidation of alkanes and/or alkenes to valuable oxygenates Lin, Manhua; Pillai, Krishnan S. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7888281 US Patent Document 7,888,281	patent	February 2011
Selective Oxidation of Alkanes and/or Alkenes to Valuable Oxygenates Lin, Manjua; Pillai, Krishnan S. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20080177106 US Patent Application 12/016264; 20080177106	patent-application	July 2008

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