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Title: Characterization of Used Nuclear Fuel with Multivariate Analysis for Process Monitoring

The Multi-Isotope Process (MIP) Monitor combines gamma spectroscopy and multivariate analysis to detect anomalies in various process streams in a nuclear fuel reprocessing system. Measured spectra are compared to models of nominal behavior at each measurement location to detect unexpected changes in system behavior. In order to improve the accuracy and specificity of process monitoring, fuel characterization may be used to more accurately train subsequent models in a full analysis scheme. This paper presents initial development of a reactor-type classifier that is used to select a reactor-specific partial least squares model to predict fuel burnup. Nuclide activities for prototypic used fuel samples were generated in ORIGEN-ARP and used to investigate techniques to characterize used nuclear fuel in terms of reactor type (pressurized or boiling water reactor) and burnup. A variety of reactor type classification algorithms, including k-nearest neighbors, linear and quadratic discriminant analyses, and support vector machines, were evaluated to differentiate used fuel from pressurized and boiling water reactors. Then, reactor type-specific partial least squares models were developed to predict the burnup of the fuel. Using these reactor type-specific models instead of a model trained for all light water reactors improved the accuracy of burnup predictions. The developed classification andmore » prediction models were combined and applied to a large dataset that included eight fuel assembly designs, two of which were not used in training the models, and spanned the range of the initial 235U enrichment, cooling time, and burnup values expected of future commercial used fuel for reprocessing. Error rates were consistent across the range of considered enrichment, cooling time, and burnup values. Average absolute relative errors in burnup predictions for validation data both within and outside the training space were 0.0574% and 0.0597%, respectively. The errors seen in this work are artificially low, because the models were trained, optimized, and tested on simulated, noise-free data. However, these results indicate that the developed models may generalize well to new data and that the proposed approach constitutes a viable first step in developing a fuel characterization algorithm based on gamma spectra.« less
 [1] ;  [2] ;  [2] ;  [2]
  1. Univ. of Texas at Austin, TX (United States)
  2. Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Publication Date:
OSTI Identifier:
Report Number(s):
Journal ID: ISSN 0168-9002; 400904120; TRN: US1400362
DOE Contract Number:
Resource Type:
Journal Article
Resource Relation:
Journal Name: Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment; Journal Volume: 746
Research Org:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Org:
Country of Publication:
United States
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; Multi-Isotope Process Monitor; Safeguards; Fuel Reprocessing; Process Monitoring