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Title: Conversion of Biomass-Derived Small Oxygenates over HZSM-5 and its Deactivation Mechanism

HZSM-5 catalyst deactivation was studied using aqueous feed mixtures containing ethanol, ethanol+ acetic acid, ethanol+ethyl acetate, or ethanol+acetaldehyde in a fixed bed reactor at 360°C and 300psig. Compared to ethanol alone experiment, addition of other oxygenates reduced catalyst life in the order of: ethyl acetate
Authors:
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Publication Date:
OSTI Identifier:
1126329
Report Number(s):
PNNL-SA-97838
BM0101010
DOE Contract Number:
AC05-76RL01830
Resource Type:
Journal Article
Resource Relation:
Journal Name: Green Chemistry, 16(2):748-760
Research Org:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English