Scalable Two–Step Production of High–Efficiency Perovskite Solar Cells and Modules
Abstract
Perovskite solar cells (PSCs) fabricated in laboratories have already achieved a power conversion efficiency (PCE) comparable to market‐dominant crystalline silicon solar cells. However, this promising photovoltaic technology suffers from severe loss of PCE during scaling up, limiting its progress toward commercialization. One critical question is to develop scalable, low‐cost, high throughput, and well‐controlled production methods to deposit high‐quality perovskite films. Among various approaches, two‐step sequential deposition methods have their unique advantages but have been long overlooked. This review provides an overview of two‐step methods for fabricating efficient and stable perovskite solar modules (PSMs). The mechanisms of two‐step perovskite conversion and advanced engineering approaches to modulate the perovskite formation process are discussed first. The progress of efficient PSCs prepared by different two‐step methods is surveyed and the advantages and disadvantages of each method for the scalable production of PSMs are compared. Particularly, it is highlighted that the vapor‐based two‐step methods are promising for high‐throughput in‐line production of PSMs. Finally, insights into the challenges and outlook of the industrialization of two‐step processes for producing PSMs are provided.
- Authors:
-
- Univ. of Toledo, OH (United States)
- Publication Date:
- Research Org.:
- Univ. of Toledo, OH (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office
- OSTI Identifier:
- 1898049
- Alternate Identifier(s):
- OSTI ID: 1907503
- Grant/Contract Number:
- EE0008790
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Solar RRL
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 2367-198X
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; perovskite solar cells and modules; sequential deposition; formation mechanism; vapor deposition; scalable production
Citation Formats
Wu, Zhifang, Bi, Enbing, Li, Chongwen, Chen, Lei, Song, Zhaoning, and Yan, Yanfa. Scalable Two–Step Production of High–Efficiency Perovskite Solar Cells and Modules. United States: N. p., 2022.
Web. doi:10.1002/solr.202200571.
Wu, Zhifang, Bi, Enbing, Li, Chongwen, Chen, Lei, Song, Zhaoning, & Yan, Yanfa. Scalable Two–Step Production of High–Efficiency Perovskite Solar Cells and Modules. United States. https://doi.org/10.1002/solr.202200571
Wu, Zhifang, Bi, Enbing, Li, Chongwen, Chen, Lei, Song, Zhaoning, and Yan, Yanfa. Thu .
"Scalable Two–Step Production of High–Efficiency Perovskite Solar Cells and Modules". United States. https://doi.org/10.1002/solr.202200571. https://www.osti.gov/servlets/purl/1898049.
@article{osti_1898049,
title = {Scalable Two–Step Production of High–Efficiency Perovskite Solar Cells and Modules},
author = {Wu, Zhifang and Bi, Enbing and Li, Chongwen and Chen, Lei and Song, Zhaoning and Yan, Yanfa},
abstractNote = {Perovskite solar cells (PSCs) fabricated in laboratories have already achieved a power conversion efficiency (PCE) comparable to market‐dominant crystalline silicon solar cells. However, this promising photovoltaic technology suffers from severe loss of PCE during scaling up, limiting its progress toward commercialization. One critical question is to develop scalable, low‐cost, high throughput, and well‐controlled production methods to deposit high‐quality perovskite films. Among various approaches, two‐step sequential deposition methods have their unique advantages but have been long overlooked. This review provides an overview of two‐step methods for fabricating efficient and stable perovskite solar modules (PSMs). The mechanisms of two‐step perovskite conversion and advanced engineering approaches to modulate the perovskite formation process are discussed first. The progress of efficient PSCs prepared by different two‐step methods is surveyed and the advantages and disadvantages of each method for the scalable production of PSMs are compared. Particularly, it is highlighted that the vapor‐based two‐step methods are promising for high‐throughput in‐line production of PSMs. Finally, insights into the challenges and outlook of the industrialization of two‐step processes for producing PSMs are provided.},
doi = {10.1002/solr.202200571},
journal = {Solar RRL},
number = 1,
volume = 7,
place = {United States},
year = {Thu Oct 06 00:00:00 EDT 2022},
month = {Thu Oct 06 00:00:00 EDT 2022}
}
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- ACS Energy Letters, Vol. 5, Issue 9
Iodine reduction for reproducible and high-performance perovskite solar cells and modules
journal, March 2021
- Chen, Shangshang; Xiao, Xun; Gu, Hangyu
- Science Advances, Vol. 7, Issue 10
High‐Pressure Nitrogen‐Extraction and Effective Passivation to Attain Highest Large‐Area Perovskite Solar Module Efficiency
journal, October 2020
- Du, Minyong; Zhu, Xuejie; Wang, Likun
- Advanced Materials, Vol. 32, Issue 47
Stabilizing perovskite-substrate interfaces for high-performance perovskite modules
journal, August 2021
- Chen, Shangshang; Dai, Xuezeng; Xu, Shuang
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Fully slot-die-coated perovskite solar cells in ambient condition
journal, May 2020
- Gao, Luoyi; Huang, Keqing; Long, Caoyu
- Applied Physics A, Vol. 126, Issue 6
Large-area perovskite solar cells employing spiro-Naph hole transport material
journal, January 2022
- Jeong, Mingyu; Choi, In Woo; Yim, Kanghoon
- Nature Photonics, Vol. 16, Issue 2
Interfacial Modification for High-Efficiency Vapor-Phase-Deposited Perovskite Solar Cells Based on a Metal Oxide Buffer Layer
journal, February 2018
- Pérez-del-Rey, Daniel; Boix, Pablo P.; Sessolo, Michele
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Vapor-Deposited Perovskites: The Route to High-Performance Solar Cell Production?
journal, November 2017
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Annealing-free efficient vacuum-deposited planar perovskite solar cells with evaporated fullerenes as electron-selective layers
journal, January 2016
- Zhao, Dewei; Ke, Weijun; Grice, Corey R.
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Highly Efficient and Stable Perovskite Solar Cells via Modification of Energy Levels at the Perovskite/Carbon Electrode Interface
journal, January 2019
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Low-bandgap mixed tin–lead iodide perovskites with reduced methylammonium for simultaneous enhancement of solar cell efficiency and stability
journal, October 2020
- Li, Chongwen; Song, Zhaoning; Chen, Cong
- Nature Energy, Vol. 5, Issue 10
Thermal degradation of CH 3 NH 3 PbI 3 perovskite into NH 3 and CH 3 I gases observed by coupled thermogravimetry–mass spectrometry analysis
journal, January 2016
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- Energy & Environmental Science, Vol. 9, Issue 11
Deposition of methylammonium iodideviaevaporation – combined kinetic and mass spectrometric study
journal, January 2018
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Thermal degradation of formamidinium based lead halide perovskites into sym -triazine and hydrogen cyanide observed by coupled thermogravimetry-mass spectrometry analysis
journal, January 2019
- Juarez-Perez, Emilio J.; Ono, Luis K.; Qi, Yabing
- Journal of Materials Chemistry A, Vol. 7, Issue 28
Chemical Reduction of Intrinsic Defects in Thicker Heterojunction Planar Perovskite Solar Cells
journal, April 2017
- Liu, Zonghao; Hu, Junnan; Jiao, Haoyang
- Advanced Materials, Vol. 29, Issue 23
Modeling the Interaction of Molecular Iodine with MAPbI 3 : A Probe of Lead-Halide Perovskites Defect Chemistry
journal, January 2018
- Meggiolaro, Daniele; Mosconi, Edoardo; De Angelis, Filippo
- ACS Energy Letters, Vol. 3, Issue 2
Iodine interstitials as a cause of nonradiative recombination in hybrid perovskites
journal, April 2020
- Zhang, Xie; Turiansky, Mark E.; Shen, Jimmy-Xuan
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Accelerated degradation of methylammonium lead iodide perovskites induced by exposure to iodine vapour
journal, December 2016
- Wang, Shenghao; Jiang, Yan; Juarez-Perez, Emilio J.
- Nature Energy, Vol. 2, Issue 1
Roles of MACl in Sequentially Deposited Bromine‐Free Perovskite Absorbers for Efficient Solar Cells
journal, December 2020
- Ye, Feihong; Ma, Junjie; Chen, Cong
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Unravelling the Effects of Grain Boundary and Chemical Doping on Electron–Hole Recombination in CH 3 NH 3 PbI 3 Perovskite by Time-Domain Atomistic Simulation
journal, March 2016
- Long, Run; Liu, Jin; Prezhdo, Oleg V.
- Journal of the American Chemical Society, Vol. 138, Issue 11
Impact of grain boundaries on efficiency and stability of organic-inorganic trihalide perovskites
journal, December 2017
- Chu, Zhaodong; Yang, Mengjin; Schulz, Philip
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Enhanced optoelectronic quality of perovskite thin films with hypophosphorous acid for planar heterojunction solar cells
journal, November 2015
- Zhang, Wei; Pathak, Sandeep; Sakai, Nobuya
- Nature Communications, Vol. 6, Issue 1
A Eu 3+ -Eu 2+ ion redox shuttle imparts operational durability to Pb-I perovskite solar cells
journal, January 2019
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Manipulation of facet orientation in hybrid perovskite polycrystalline films by cation cascade
journal, July 2018
- Zheng, Guanhaojie; Zhu, Cheng; Ma, Jingyuan
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A piperidinium salt stabilizes efficient metal-halide perovskite solar cells
journal, July 2020
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Air-Stable Hybrid Perovskite Solar Cell by Sequential Vapor Deposition in a Single Reactor
journal, February 2020
- Ngqoloda, Siphelo; Arendse, Christopher J.; Muller, Theophillus F.
- ACS Applied Energy Materials, Vol. 3, Issue 3