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Title: Nanoscale control of LaAlO 3 /SrTiO 3 metal–insulator transition using ultra-low-voltage electron-beam lithography

Abstract

In this work, we describe a method to control the insulator–metal transition at the LaAlO3/SrTiO3 interface using ultra-low-voltage electron beam lithography. Compared to previous reports that utilize conductive atomic force microscope (c-AFM) lithography, this approach can provide comparable resolution (~10 nm) at write speeds (10 mm/s) that are up to 10 000× faster than c-AFM. The writing technique is nondestructive, and the conductive state is reversible via prolonged exposure to air. Transport properties of representative devices are measured at milli-Kelvin temperatures, where superconducting behavior is observed. We also demonstrate the ability to create conducting devices on graphene/LaAlO3/SrTiO3 heterostructures. The underlying mechanism is believed to be closely related to the same mechanism regulating c-AFM-based methods.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2];  [1]; ORCiD logo [1];  [1]; ORCiD logo [3];  [3];  [3]; ORCiD logo [1]; ORCiD logo [1]
  1. University of Pittsburgh, Pittsburgh, PA (United States). Department of Physics and Astronomy; Pittsburgh Quantum Institute, Pittsburgh, PA (United States)
  2. Univ. of Pittsburgh, PA (United States). Department of Electrical and Computer Engineering and Peterson Institute of Nanoscience and Engineering
  3. University of Wisconsin-Madison, Madison, WI (United States). Department of Materials Science and Engineering
Publication Date:
Research Org.:
Univ. of Wisconsin, Madison, WI (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); US Office of Naval Research (ONR)
OSTI Identifier:
1849704
Alternate Identifier(s):
OSTI ID: 1737864
Grant/Contract Number:  
FG02-06ER46327; N00014-20-1-2481; N00014-15-2847
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 117; Journal Issue: 25; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Physics

Citation Formats

Yang, Dengyu, Hao, Shan, Chen, Jun, Guo, Qing, Yu, Muqing, Hu, Yang, Eom, Kitae, Lee, Jung-Woo, Eom, Chang-Beom, Irvin, Patrick, and Levy, Jeremy. Nanoscale control of LaAlO 3 /SrTiO 3 metal–insulator transition using ultra-low-voltage electron-beam lithography. United States: N. p., 2020. Web. doi:10.1063/5.0027480.
Yang, Dengyu, Hao, Shan, Chen, Jun, Guo, Qing, Yu, Muqing, Hu, Yang, Eom, Kitae, Lee, Jung-Woo, Eom, Chang-Beom, Irvin, Patrick, & Levy, Jeremy. Nanoscale control of LaAlO 3 /SrTiO 3 metal–insulator transition using ultra-low-voltage electron-beam lithography. United States. https://doi.org/10.1063/5.0027480
Yang, Dengyu, Hao, Shan, Chen, Jun, Guo, Qing, Yu, Muqing, Hu, Yang, Eom, Kitae, Lee, Jung-Woo, Eom, Chang-Beom, Irvin, Patrick, and Levy, Jeremy. Mon . "Nanoscale control of LaAlO 3 /SrTiO 3 metal–insulator transition using ultra-low-voltage electron-beam lithography". United States. https://doi.org/10.1063/5.0027480. https://www.osti.gov/servlets/purl/1849704.
@article{osti_1849704,
title = {Nanoscale control of LaAlO 3 /SrTiO 3 metal–insulator transition using ultra-low-voltage electron-beam lithography},
author = {Yang, Dengyu and Hao, Shan and Chen, Jun and Guo, Qing and Yu, Muqing and Hu, Yang and Eom, Kitae and Lee, Jung-Woo and Eom, Chang-Beom and Irvin, Patrick and Levy, Jeremy},
abstractNote = {In this work, we describe a method to control the insulator–metal transition at the LaAlO3/SrTiO3 interface using ultra-low-voltage electron beam lithography. Compared to previous reports that utilize conductive atomic force microscope (c-AFM) lithography, this approach can provide comparable resolution (~10 nm) at write speeds (10 mm/s) that are up to 10 000× faster than c-AFM. The writing technique is nondestructive, and the conductive state is reversible via prolonged exposure to air. Transport properties of representative devices are measured at milli-Kelvin temperatures, where superconducting behavior is observed. We also demonstrate the ability to create conducting devices on graphene/LaAlO3/SrTiO3 heterostructures. The underlying mechanism is believed to be closely related to the same mechanism regulating c-AFM-based methods.},
doi = {10.1063/5.0027480},
journal = {Applied Physics Letters},
number = 25,
volume = 117,
place = {United States},
year = {Mon Dec 21 00:00:00 EST 2020},
month = {Mon Dec 21 00:00:00 EST 2020}
}

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