DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Cryogenic Operation of Planar Ultrananocrystalline Diamond Field Emission Source in SRF Injector

Abstract

In this work, we report a demonstration of electron beam generation in a superconducting radio frequency (SRF) Teraelectronvolt Energy Superconducting Linear Accelerator 1.3 GHz gun equipped with a field emission cathode and operated at 2 K. The cathode is a submicrometer film of nitrogen-incorporated ultrananocrystalline diamond [(N)UNCD] deposited atop a Nb RRR300 cathode plug that is 4 mm in diameter. Measurements of the output current showed that it increased exponentially as a function of the gun gradient. Our results demonstrate a feasible path toward simplified fully cryogenic SRF injector technology. At a maximal gradient of 0.9 MV/m, a current density of 22 μA/cm2 was obtained [calculated as a 2.75 μA current over the total cathode surface area of π(2 mm)2]. One important finding is that the electron emitter made of (N)UNCD, a material long been known as a highly efficient field emission material, demonstrated a record low turn-on gradient of 0.6 MV/m. A hypothesis explaining this behavior is proposed.

Authors:
 [1];  [2];  [3];  [3];  [4];  [3];  [5];  [2];  [6];  [2];  [7];  [7]
  1. Michigan State Univ., East Lansing, MI (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Euclid TechLabs, Bolingbrook, IL (United States)
  4. Euclid TechLabs, Bolingbrook, IL (United States); Leidos, Reston, VA (United States)
  5. Brookhaven National Lab. (BNL), Upton, NY (United States); Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States)
  6. Brookhaven National Lab. (BNL), Upton, NY (United States); Central Academy of Drama of China, Beijing (China)
  7. Argonne National Lab. (ANL), Lemont, IL (United States). Center for Nanoscale Materials
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP); USDOE Office of Technology Transitions (OTT)
OSTI Identifier:
1764006
Alternate Identifier(s):
OSTI ID: 1823267
Report Number(s):
BNL-220965-2021-JAAM
Journal ID: ISSN 0003-6951; TRN: US2206128
Grant/Contract Number:  
SC0012704; AC02-06CH11357; SC0013145; ED2701000-05450-1009209
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 118; Journal Issue: 5; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
43 PARTICLE ACCELERATORS; Carbon based materials; Diamond; Particle accelerators; Field emitter arrays; Raman spectroscopy

Citation Formats

Baryshev, Sergey V., Wang, Erdong, Jing, Chunguang, Jabotinski, Vadim, Antipov, Sergey, Kanareykin, Alexei, Belomestnykh, Sergey, Ben-Zvi, Ilan, Chen, Lizhi, Wu, Qiong, Li, Hao, and Sumant, Anirudha V. Cryogenic Operation of Planar Ultrananocrystalline Diamond Field Emission Source in SRF Injector. United States: N. p., 2021. Web. doi:10.1063/5.0013172.
Baryshev, Sergey V., Wang, Erdong, Jing, Chunguang, Jabotinski, Vadim, Antipov, Sergey, Kanareykin, Alexei, Belomestnykh, Sergey, Ben-Zvi, Ilan, Chen, Lizhi, Wu, Qiong, Li, Hao, & Sumant, Anirudha V. Cryogenic Operation of Planar Ultrananocrystalline Diamond Field Emission Source in SRF Injector. United States. https://doi.org/10.1063/5.0013172
Baryshev, Sergey V., Wang, Erdong, Jing, Chunguang, Jabotinski, Vadim, Antipov, Sergey, Kanareykin, Alexei, Belomestnykh, Sergey, Ben-Zvi, Ilan, Chen, Lizhi, Wu, Qiong, Li, Hao, and Sumant, Anirudha V. Fri . "Cryogenic Operation of Planar Ultrananocrystalline Diamond Field Emission Source in SRF Injector". United States. https://doi.org/10.1063/5.0013172. https://www.osti.gov/servlets/purl/1764006.
@article{osti_1764006,
title = {Cryogenic Operation of Planar Ultrananocrystalline Diamond Field Emission Source in SRF Injector},
author = {Baryshev, Sergey V. and Wang, Erdong and Jing, Chunguang and Jabotinski, Vadim and Antipov, Sergey and Kanareykin, Alexei and Belomestnykh, Sergey and Ben-Zvi, Ilan and Chen, Lizhi and Wu, Qiong and Li, Hao and Sumant, Anirudha V.},
abstractNote = {In this work, we report a demonstration of electron beam generation in a superconducting radio frequency (SRF) Teraelectronvolt Energy Superconducting Linear Accelerator 1.3 GHz gun equipped with a field emission cathode and operated at 2 K. The cathode is a submicrometer film of nitrogen-incorporated ultrananocrystalline diamond [(N)UNCD] deposited atop a Nb RRR300 cathode plug that is 4 mm in diameter. Measurements of the output current showed that it increased exponentially as a function of the gun gradient. Our results demonstrate a feasible path toward simplified fully cryogenic SRF injector technology. At a maximal gradient of 0.9 MV/m, a current density of 22 μA/cm2 was obtained [calculated as a 2.75 μA current over the total cathode surface area of π(2 mm)2]. One important finding is that the electron emitter made of (N)UNCD, a material long been known as a highly efficient field emission material, demonstrated a record low turn-on gradient of 0.6 MV/m. A hypothesis explaining this behavior is proposed.},
doi = {10.1063/5.0013172},
journal = {Applied Physics Letters},
number = 5,
volume = 118,
place = {United States},
year = {Fri Jan 29 00:00:00 EST 2021},
month = {Fri Jan 29 00:00:00 EST 2021}
}

Works referenced in this record:

Planar ultrananocrystalline diamond field emitter in accelerator radio frequency electron injector: Performance metrics
journal, November 2014

  • Baryshev, Sergey V.; Antipov, Sergey; Shao, Jiahang
  • Applied Physics Letters, Vol. 105, Issue 20, Article No. 203505
  • DOI: 10.1063/1.4901723

Investigation of the dc vacuum breakdown mechanism
journal, September 2009

  • Descoeudres, A.; Levinsen, Y.; Calatroni, S.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 12, Issue 9
  • DOI: 10.1103/PhysRevSTAB.12.092001

The effect of nitrogen addition to Ar/CH4 plasmas on the growth, morphology and field emission of ultrananocrystalline diamond
journal, January 2002


Origin of a needle-like granular structure for ultrananocrystalline diamond films grown in a N 2 /CH 4 plasma
journal, August 2012


Heat load of a GaAs photocathode in an SRF electron gun
journal, April 2011


Field-emission cathode gating for rf electron guns
journal, March 2005


Mean transverse energy of ultrananocrystalline diamond photocathode
journal, March 2019

  • Chen, Gongxiaohui; Adhikari, Gowri; Spentzouris, Linda
  • Applied Physics Letters, Vol. 114, Issue 9
  • DOI: 10.1063/1.5084167

Origin of low threshold field emission from nitrogen-incorporated nanocrystalline diamond films
journal, April 2009

  • Ikeda, Tomohiro; Teii, Kungen
  • Applied Physics Letters, Vol. 94, Issue 14
  • DOI: 10.1063/1.3115767

Nanodiamond Thin Film Field Emitter Cartridge for Miniature High-Gradient Radio Frequency ${X}$ -Band Electron Injector
journal, March 2018

  • Qiu, Jiaqi; Baturin, Stanislav S.; Kovi, Kiran Kumar
  • IEEE Transactions on Electron Devices, Vol. 65, Issue 3
  • DOI: 10.1109/TED.2017.2788822

Higher-order mode-based cavity misalignment measurements at the free-electron laser FLASH
journal, December 2017


Strain engineering the work function in monolayer metal dichalcogenides
journal, April 2015

  • Lanzillo, Nicholas A.; Simbeck, Adam J.; Nayak, Saroj K.
  • Journal of Physics: Condensed Matter, Vol. 27, Issue 17
  • DOI: 10.1088/0953-8984/27/17/175501

High-brightness electron beams – small free-electron lasers
journal, April 1998

  • Brau, C. A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 407, Issue 1-3
  • DOI: 10.1016/S0168-9002(97)01356-9

Low-threshold cold cathodes made of nitrogen-doped chemical-vapour-deposited diamond
journal, May 1996

  • Okano, Ken; Koizumi, Satoshi; Silva, S. Ravi P.
  • Nature, Vol. 381, Issue 6578
  • DOI: 10.1038/381140a0

Work Function Modulation of Molybdenum Disulfide Nanosheets by Introducing Systematic Lattice Strain
journal, August 2017


High-Brightness Continuous-Wave Electron Beams from Superconducting Radio-Frequency Photoemission Gun
journal, June 2020


Locally Resolved Electron Emission Area and Unified View of Field Emission from Ultrananocrystalline Diamond Films
journal, September 2017

  • Chubenko, Oksana; Baturin, Stanislav S.; Kovi, Kiran K.
  • ACS Applied Materials & Interfaces, Vol. 9, Issue 38
  • DOI: 10.1021/acsami.7b07062

High quantum efficiency ultrananocrystalline diamond photocathode for photoinjector applications
journal, September 2014

  • Pérez Quintero, Kenneth J.; Antipov, Sergey; Sumant, Anirudha V.
  • Applied Physics Letters, Vol. 105, Issue 12, Article No. 123103
  • DOI: 10.1063/1.4896418

Superconducting TESLA cavities
journal, September 2000

  • Aune, B.; Bandelmann, R.; Bloess, D.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 3, Issue 9
  • DOI: 10.1103/PhysRevSTAB.3.092001

Dynamic graphitization of ultra-nano-crystalline diamond and its effects on material resistivity
journal, December 2020

  • Nikhar, Tanvi; Rechenberg, Robert; Becker, Michael F.
  • Journal of Applied Physics, Vol. 128, Issue 23
  • DOI: 10.1063/5.0029132