A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory
Abstract
Abstract Atmospheric supply of iron can modulate ocean biogeochemistry, due to its key role in global nitrogen and carbon cycles. Current estimates predict up to 20% of global ocean net primary productivity depends on an atmospheric iron source. Using a technology‐based methodology, we revise total and soluble anthropogenic iron emissions and resolve iron into its mineral components, which allows modeling mineral‐specific atmospheric reactions. We compare different methodologies for representing anthropogenic iron solubility: measured in mild and strong leaches and estimated using a mineralogy basis and identify the emissions that are most affected by such assumptions. The inclusion of metal smelting as an iron source increases iron emissions by up to 10 times higher in the fine aerosol fraction (smaller than 1 μm) than most previous inventories. Different solubility assumptions alter anthropogenic soluble iron emissions and deposition by a factor of 20 and 10, respectively. Using solubilities measured in mild leaches and calculated by mineralogy give 20–30 Gg/yr anthropogenic emissions and 40–50 Gg/yr deposition, while those measured in strong leaches give 80–440 Gg/yr emissions and 200–450 Gg/yr deposition. This range of anthropogenic soluble iron deposition leads to global soluble iron deposition of 1,900–2,300 Gg/yr when dust, wildfires, and atmospheric processing are included, indicating such assumptions can affectmore »
- Authors:
-
- Univ. of Illinois at Urbana-Champaign, IL (United States); Colorado State Univ., Fort Collins, CO (United States)
- Cornell Univ., Ithaca, NY (United States)
- International Inst. for Applied Systems Analysis (IIASA), Laxenburg (Austria)
- Univ. of Delaware, Newark, DE (United States)
- Publication Date:
- Research Org.:
- Univ. of Illinois at Urbana-Champaign, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Biological and Environmental Research (BER). Earth and Environmental Systems Science Division; USDOE
- OSTI Identifier:
- 1734785
- Alternate Identifier(s):
- OSTI ID: 1782269
- Grant/Contract Number:
- SC0016321; DE‐Sc0016362
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Additional Journal Information:
- Journal Volume: 125; Journal Issue: 17; Journal ID: ISSN 2169-897X
- Publisher:
- American Geophysical Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 58 GEOSCIENCES; 54 ENVIRONMENTAL SCIENCES; aerosol; emission inventory; biogeochemical cycles; iron; solubility; anthropogenic; biogeochemistry; mineralogy; emissions
Citation Formats
Rathod, Sagar D., Hamilton, Douglas S., Mahowald, Natalie M., Klimont, Zbigniew, Corbett, James J., and Bond, Tami C. A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory. United States: N. p., 2020.
Web. doi:10.1029/2019jd032114.
Rathod, Sagar D., Hamilton, Douglas S., Mahowald, Natalie M., Klimont, Zbigniew, Corbett, James J., & Bond, Tami C. A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory. United States. https://doi.org/10.1029/2019jd032114
Rathod, Sagar D., Hamilton, Douglas S., Mahowald, Natalie M., Klimont, Zbigniew, Corbett, James J., and Bond, Tami C. Mon .
"A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory". United States. https://doi.org/10.1029/2019jd032114. https://www.osti.gov/servlets/purl/1734785.
@article{osti_1734785,
title = {A Mineralogy–Based Anthropogenic Combustion–Iron Emission Inventory},
author = {Rathod, Sagar D. and Hamilton, Douglas S. and Mahowald, Natalie M. and Klimont, Zbigniew and Corbett, James J. and Bond, Tami C.},
abstractNote = {Abstract Atmospheric supply of iron can modulate ocean biogeochemistry, due to its key role in global nitrogen and carbon cycles. Current estimates predict up to 20% of global ocean net primary productivity depends on an atmospheric iron source. Using a technology‐based methodology, we revise total and soluble anthropogenic iron emissions and resolve iron into its mineral components, which allows modeling mineral‐specific atmospheric reactions. We compare different methodologies for representing anthropogenic iron solubility: measured in mild and strong leaches and estimated using a mineralogy basis and identify the emissions that are most affected by such assumptions. The inclusion of metal smelting as an iron source increases iron emissions by up to 10 times higher in the fine aerosol fraction (smaller than 1 μm) than most previous inventories. Different solubility assumptions alter anthropogenic soluble iron emissions and deposition by a factor of 20 and 10, respectively. Using solubilities measured in mild leaches and calculated by mineralogy give 20–30 Gg/yr anthropogenic emissions and 40–50 Gg/yr deposition, while those measured in strong leaches give 80–440 Gg/yr emissions and 200–450 Gg/yr deposition. This range of anthropogenic soluble iron deposition leads to global soluble iron deposition of 1,900–2,300 Gg/yr when dust, wildfires, and atmospheric processing are included, indicating such assumptions can affect global soluble iron supply by about 30%. In regions where marine primary productivity is iron limited, anthropogenic combustion‐iron contributes up to half of the atmospheric soluble iron flux to the North Pacific Ocean but supplies less than 5% to the Southern Ocean.},
doi = {10.1029/2019jd032114},
journal = {Journal of Geophysical Research: Atmospheres},
number = 17,
volume = 125,
place = {United States},
year = {Mon Aug 03 00:00:00 EDT 2020},
month = {Mon Aug 03 00:00:00 EDT 2020}
}
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