Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks

Stroujkova, A.; Gorman, E.; Avendaño, S. T.; Horne, M.; Person, M. A.; Hubbard, P.; Salerno, J.; Carrigan, C. R.; Harp, Dylan Robert; Stauffer, Philip H.

doi:10.1029/2019jb018992

Title: Using SF₆ and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks

Authors:

^[1]; Gorman, E. ^[2]; Avendaño, S. T. ^[3]; Horne, M. ^[4];

^[4]; Hubbard, P. ^[1]; Salerno, J. ^[1];

^[5];

^[3];

^[3]

Applied Research Associates, Lexington MA (United States)
Columbia Univ., Palisades, NY (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
New Mexico Inst. of Mining and Technology, Socorro, NM (United States)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Publication Date:: Wed Apr 15 00:00:00 EDT 2020

Research Org.:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Org.:: Defense Threat Reduction Agency (DTRA); USDOE National Nuclear Security Administration (NNSA)

OSTI Identifier:: 1660592

Alternate Identifier(s):: OSTI ID: 1616486; OSTI ID: 1813696

Report Number(s):: LA-UR-19-24483; LLNL-JRNL-817844
Journal ID: ISSN 2169-9313

Grant/Contract Number:: 89233218CNA000001; HDTRA1‐17‐1‐0040; AC52-06NA25396; AC52-07NA27344

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Geophysical Research. Solid Earth

Additional Journal Information:: Journal Volume: 125; Journal Issue: 5; Journal ID: ISSN 2169-9313

Publisher:: American Geophysical Union

Country of Publication:: United States

Language:: English

Subject:: 58 GEOSCIENCES; underground explosion monitoring; gas transport; fractured rock; gas sampling; Geosciences, Environmental sciences

Citation Formats


                    Stroujkova, A., Gorman, E., Avendaño, S. T., Horne, M., Person, M. A., Hubbard, P., Salerno, J., Carrigan, C. R., Harp, Dylan Robert, and Stauffer, Philip H. Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks.  United States: N. p., 2020. 
Web.  doi:10.1029/2019jb018992.

Copy to clipboard


                    Stroujkova, A., Gorman, E., Avendaño, S. T., Horne, M., Person, M. A., Hubbard, P., Salerno, J., Carrigan, C. R., Harp, Dylan Robert, & Stauffer, Philip H. Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks.  United States.  https://doi.org/10.1029/2019jb018992

Copy to clipboard


                    Stroujkova, A., Gorman, E., Avendaño, S. T., Horne, M., Person, M. A., Hubbard, P., Salerno, J., Carrigan, C. R., Harp, Dylan Robert, and Stauffer, Philip H. Wed .  
"Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks".  United States.  https://doi.org/10.1029/2019jb018992.  https://www.osti.gov/servlets/purl/1660592.

Copy to clipboard


                    
@article{osti_1660592,

  title        = {Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks},

  author       = {Stroujkova, A. and Gorman, E. and Avendaño, S. T. and Horne, M. and Person, M. A. and Hubbard, P. and Salerno, J. and Carrigan, C. R. and Harp, Dylan Robert and Stauffer, Philip H.},

  abstractNote = {},

  doi          = {10.1029/2019jb018992},

  journal      = {Journal of Geophysical Research. Solid Earth},

  number       = 5,

  volume       = 125,

  place        = {United States},

  year         = {Wed Apr 15 00:00:00 EDT 2020},

  month        = {Wed Apr 15 00:00:00 EDT 2020}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (DOE)

Publisher's Version of Record

https://doi.org/10.1029/2019jb018992

Other availability

Search WorldCat to find libraries that may hold this journal

Citation Metrics:

Cited by: 3 works

Citation information provided by
Web of Science

Save / Share:

Export Metadata

Save to My Library

Works referenced in this record:

Characterization of Xe-133 global atmospheric background: Implications for the International Monitoring System of the Comprehensive Nuclear-Test-Ban Treaty: Xe-133 Global Atmospheric Background
journal, May 2016

Achim, Pascal; Generoso, Sylvia; Morin, Mireille
Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 9
DOI: 10.1002/2016JD024872

Radionuclide migration experiments under laboratory conditions
journal, June 1995

Vandergraaf, T. T.
Geophysical Research Letters, Vol. 22, Issue 11
DOI: 10.1029/95GL01492

Trace gas emissions on geological faults as indicators of underground nuclear testing
journal, August 1996

Carrigan, C. R.; Heinle, R. A.; Hudson, G. B.
Nature, Vol. 382, Issue 6591
DOI: 10.1038/382528a0

A New Experimental Field Study of the Effects of Explosive Detonation Products on Seismic Radiation
journal, June 2017

Stroujkova, Anastasia; Leidig, Mark; Lewkowicz, James
Seismological Research Letters, Vol. 88, Issue 5
DOI: 10.1785/0220170032

Atmospheric pumping: A mechanism causing vertical transport of contaminated gases through fractured permeable media
journal, December 1991

Nilson, R. H.; Peterson, E. W.; Lie, K. H.
Journal of Geophysical Research: Solid Earth, Vol. 96, Issue B13
DOI: 10.1029/91JB01836

Rock Damage and Seismic Radiation: A Case Study of the Chemical Explosions in New Hampshire
journal, October 2018

Stroujkova, Anastasia
Bulletin of the Seismological Society of America, Vol. 108, Issue 6
DOI: 10.1785/0120180117

Discrimination of Nuclear Explosions against Civilian Sources Based on Atmospheric Xenon Isotopic Activity Ratios
journal, January 2010

Kalinowski, Martin B.; Axelsson, Anders; Bean, Marc
Pure and Applied Geophysics, Vol. 167, Issue 4-5
DOI: 10.1007/s00024-009-0032-1

Evidence for High Rates of Gas Transport in the Deep Subsurface
journal, April 2019

Stauffer, P. H.; Rahn, T.; Ortiz, J. P.
Geophysical Research Letters, Vol. 46, Issue 7
DOI: 10.1029/2019GL082394

The solubility of certain gaseous fluorine compounds in water
journal, January 1968

Ashton, J. T.; Dawe, R. A.; Miller, K. W.
Journal of the Chemical Society A: Inorganic, Physical, Theoretical
DOI: 10.1039/j19680001793

Subsurface mass transport affects the radioxenon signatures that are used to identify clandestine nuclear tests: SUBSURFACE MASS TRANSPORT AFFECTS RADIOXENON SIGNATURES
journal, January 2013

Lowrey, J. D.; Biegalski, S. R.; Osborne, A. G.
Geophysical Research Letters, Vol. 40, Issue 1
DOI: 10.1029/2012GL053885

Uncertainty in Prediction of Radionuclide Gas Migration from Underground Nuclear Explosions
journal, January 2014

Jordan, Amy B.; Stauffer, Philip H.; Zyvoloski, George A.
Vadose Zone Journal, Vol. 13, Issue 10
DOI: 10.2136/vzj2014.06.0070

Xenon adsorption on geological media and implications for radionuclide signatures
journal, July 2018

Paul, M. J.; Biegalski, S. R.; Haas, D. A.
Journal of Environmental Radioactivity, Vol. 187
DOI: 10.1016/j.jenvrad.2018.01.029

Experimental determination of noble gases and SF6, as tracers of CO2 flow through porous sandstone
journal, March 2018

Kilgallon, R.; Gilfillan, S. M. V.; Edlmann, K.
Chemical Geology, Vol. 480
DOI: 10.1016/j.chemgeo.2017.09.022

Noble gas migration experiment to support the detection of underground nuclear explosions
journal, December 2015

Olsen, K. B.; Kirkham, R. R.; Woods, V. T.
Journal of Radioanalytical and Nuclear Chemistry, Vol. 307, Issue 3
DOI: 10.1007/s10967-015-4639-7

Similar Records in DOE PAGES and OSTI.GOV collections:

Radionuclide gas transport through nuclear explosion-generated fracture networks

Journal Article Jordan, Amy B. ; Stauffer, Philip H. ; Knight, Earl E. ; ... - Scientific Reports

Underground nuclear weapon testing produces radionuclide gases which may seep to the surface. Barometric pumping of gas through explosion-fractured rock is investigated using a new sequentially-coupled hydrodynamic rock damage/gas transport model. Fracture networks are produced for two rock types (granite and tuff) and three depths of burial. The fracture networks are integrated into a flow and transport numerical model driven by surface pressure signals of differing amplitude and variability. There are major differences between predictions using a realistic fracture network and prior results that used a simplified geometry. Matrix porosity and maximum fracture aperture have the greatest impact on gasmore »« less
Cited by 34
https://doi.org/10.1038/srep18383

Full Text Available
Detection of Spatiotemporal Prescription Opioid Hot Spots With Network Scan Statistics: Multistate Analysis

Journal Article Basak, Arinjoy ; Cadena, Jose ; Marathe, Achla ; ... - JMIR Public Health and Surveillance

Background: Overuse and misuse of prescription opioids have become significant public health burdens in the United States. About 11.5 million people are estimated to have misused prescription opioids for nonmedical purposes in 2016. This has led to a significant number of drug overdose deaths in the United States. Previous studies have examined spatiotemporal clusters of opioid misuse, but they have been restricted to circular shaped regions. Objective: The goal of this study was to identify spatiotemporal hot spots of opioid users and opioid prescription claims using Medicare data. Methods: We examined spatiotemporal clusters with significantly higher number of beneficiaries andmore »« less
https://doi.org/10.2196/12110

Full Text Available
Effectiveness of supercritical-CO₂ and N₂ huff-and-puff methods of enhanced oil recovery in shale fracture networks using microfluidic experiments

Journal Article Nguyen, Thanh Phong ; Carey, J. William ; Viswanathan, Hari S. ; ... - Applied Energy
https://doi.org/10.1016/j.apenergy.2018.08.098

Full Text Available
Measured and calculated SF{sub 6}{sup -} collision and swarm ion transport data in SF{sub 6}-Ar and SF{sub 6}-Xe mixtures

Journal Article Benhenni, M ; Yousfi, M ; Merbahi, N ; ... - Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics

The measurement of the mobility of SF{sub 6}{sup -} in the mixtures SF{sub 6}-Ar and SF{sub 6}-Xe is reported over the density-reduced electric field strength E/N 1-180 Td (1 Townsend=10{sup -17} V cm{sup 2}), from a time-resolved pulsed Townsend technique. Simultaneously, the mobility of SF{sub 6}{sup -} in the same binary mixtures has been calculated from a set of collision cross sections for SF{sub 6}{sup -}-Ar, SF{sub 6}{sup -}-Xe, and SF{sub 6}{sup -}-SF{sub 6} using a Monte Carlo simulation procedure for ion transport. The good agreement between measured and calculated mobilities in these gas mixtures has led us to concludemore »« less
https://doi.org/10.1103/PhysRevE.71.036405
Identification of corona discharge-induced SF/sub 6/ oxidation mechanisms using SF/sub 6///sup 18/O/sub 2//H/sub 2/ /sup 16/O and SF/sub 6///sup 16/O/sub 2//H/sub 2/ /sup 18/O gas mixtures

Journal Article Van Brunt, R J ; Siddagangappa, M C - Plasma Chem. Plasma Process.; (United States)

The absolute yields of gaseous oxyfluorides SOF/sub 2/, SO/sub 2/F/sub 2/, and SOF/sub 4/ from negative, point-plane corona discharges in pressurized gas mixtures of SF/sub 6/ with O/sub 2/ and H/sub 2/O enriched with /sup 18/O/sub 2/ and H/sub 2/ /sup 18/O have been measured using a gas chromatograph-mass spectrometer. The predominant SF/sub 6/ oxidation mechanisms have been revealed from a determination of the relative /sup 18/O and /sup 16/O isotope content of the observed oxy-fluoride by-products. The results are consistent with previously proposed production mechanisms and indicate that SOF/sub 2/ and SO/sub 2/F/sub 2/ derive oxygen predominantly from H/submore »« less
https://doi.org/10.1007/BF01016158

Similar Records

Title: Using SF6 and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks

Citation Formats

Characterization of Xe-133 global atmospheric background: Implications for the International Monitoring System of the Comprehensive Nuclear-Test-Ban Treaty: Xe-133 Global Atmospheric Background journal, May 2016

Radionuclide migration experiments under laboratory conditions journal, June 1995

Trace gas emissions on geological faults as indicators of underground nuclear testing journal, August 1996

A New Experimental Field Study of the Effects of Explosive Detonation Products on Seismic Radiation journal, June 2017

Atmospheric pumping: A mechanism causing vertical transport of contaminated gases through fractured permeable media journal, December 1991

Rock Damage and Seismic Radiation: A Case Study of the Chemical Explosions in New Hampshire journal, October 2018

Discrimination of Nuclear Explosions against Civilian Sources Based on Atmospheric Xenon Isotopic Activity Ratios journal, January 2010

Evidence for High Rates of Gas Transport in the Deep Subsurface journal, April 2019

The solubility of certain gaseous fluorine compounds in water journal, January 1968

Subsurface mass transport affects the radioxenon signatures that are used to identify clandestine nuclear tests: SUBSURFACE MASS TRANSPORT AFFECTS RADIOXENON SIGNATURES journal, January 2013

Uncertainty in Prediction of Radionuclide Gas Migration from Underground Nuclear Explosions journal, January 2014

Xenon adsorption on geological media and implications for radionuclide signatures journal, July 2018

Experimental determination of noble gases and SF6, as tracers of CO2 flow through porous sandstone journal, March 2018

Noble gas migration experiment to support the detection of underground nuclear explosions journal, December 2015

Title: Using SF₆ and Xe to Monitor Gas Migration Through Explosion-Generated Fracture Networks

Characterization of Xe-133 global atmospheric background: Implications for the International Monitoring System of the Comprehensive Nuclear-Test-Ban Treaty: Xe-133 Global Atmospheric Background
journal, May 2016

Radionuclide migration experiments under laboratory conditions
journal, June 1995

Trace gas emissions on geological faults as indicators of underground nuclear testing
journal, August 1996

A New Experimental Field Study of the Effects of Explosive Detonation Products on Seismic Radiation
journal, June 2017

Atmospheric pumping: A mechanism causing vertical transport of contaminated gases through fractured permeable media
journal, December 1991

Rock Damage and Seismic Radiation: A Case Study of the Chemical Explosions in New Hampshire
journal, October 2018

Discrimination of Nuclear Explosions against Civilian Sources Based on Atmospheric Xenon Isotopic Activity Ratios
journal, January 2010

Evidence for High Rates of Gas Transport in the Deep Subsurface
journal, April 2019

The solubility of certain gaseous fluorine compounds in water
journal, January 1968

Subsurface mass transport affects the radioxenon signatures that are used to identify clandestine nuclear tests: SUBSURFACE MASS TRANSPORT AFFECTS RADIOXENON SIGNATURES
journal, January 2013

Uncertainty in Prediction of Radionuclide Gas Migration from Underground Nuclear Explosions
journal, January 2014

Xenon adsorption on geological media and implications for radionuclide signatures
journal, July 2018

Experimental determination of noble gases and SF6, as tracers of CO2 flow through porous sandstone
journal, March 2018

Noble gas migration experiment to support the detection of underground nuclear explosions
journal, December 2015