Observations of Multiple Nuclear Reaction Histories and Fuel-Ion Species Dynamics in Shock-Driven Inertial Confinement Fusion Implosions
Abstract
Fuel-ion species dynamics in DT3He-gas-filled Inertial Confinement Fusion implosion is quantitatively assessed for the first time using simultaneously measured D3He and DT reaction histories. Here, these reaction histories are measured with the Particle X-ray Temporal Diagnostic, which captures the relative timing between different nuclear burns with unprecedented precision (~10 ps). The observed 50±10 ps earlier D3He reaction history timing (relative to DT) cannot be explained by average-ion hydrodynamic simulations, and is attributed to fuel-ion species separation between the D, T, and 3He ions during shock convergence and rebound. At the onset of the shock burn, inferred 3He/T fuel ratio in the burn region using the measured reaction histories is much higher as compared to the initial gas-fill ratio. As T and 3He have the same mass but different charge, these results indicate that the charge-to-mass ratio plays an important role in driving fuel-ion species separation during strong shock propagation.
- Authors:
-
more »
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Univ. of Rome (Italy)
- Univ. of Rochester, NY (United States). Lab. for Laser Energetics
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- Univ. of Nevada, Reno, NV (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1657124
- Alternate Identifier(s):
- OSTI ID: 1492108; OSTI ID: 1884638
- Report Number(s):
- LA-UR-18-30435; LLNL-JRNL-839254
Journal ID: ISSN 0031-9007; TRN: US2203228
- Grant/Contract Number:
- 89233218CNA000001; NA0001857; NA0002949; DENA0002905; FC52-08NA28752; AC52-07NA27344
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 122; Journal Issue: 3; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 22 GENERAL STUDIES OF NUCLEAR REACTORS; 70 PLASMA PHYSICS AND FUSION TECHNOLOGY
Citation Formats
Sio, Hong, Frenje, J. A., Le, Ari Yitzchak, Atzeni, S., Kwan, Thomas J. T, Gatu Johnson, M., Kagan, Grigory, Stoeckl, C., Li, C. K., Parker, C. E., Forrest, C. J., Glebov, V., Kabadi, N. V., Bose, A., Rinderknecht, H. G., Amendt, P., Casey, D. T., Mancini, R., Taitano, William, Keenan, Brett, Simakov, Andrei N., Chacon, Luis, Regan, S. P., Sangster, T. C., Campbell, E. M., Seguin, F. H., and Petrasso, R. D. Observations of Multiple Nuclear Reaction Histories and Fuel-Ion Species Dynamics in Shock-Driven Inertial Confinement Fusion Implosions. United States: N. p., 2019.
Web. doi:10.1103/physrevlett.122.035001.
Sio, Hong, Frenje, J. A., Le, Ari Yitzchak, Atzeni, S., Kwan, Thomas J. T, Gatu Johnson, M., Kagan, Grigory, Stoeckl, C., Li, C. K., Parker, C. E., Forrest, C. J., Glebov, V., Kabadi, N. V., Bose, A., Rinderknecht, H. G., Amendt, P., Casey, D. T., Mancini, R., Taitano, William, Keenan, Brett, Simakov, Andrei N., Chacon, Luis, Regan, S. P., Sangster, T. C., Campbell, E. M., Seguin, F. H., & Petrasso, R. D. Observations of Multiple Nuclear Reaction Histories and Fuel-Ion Species Dynamics in Shock-Driven Inertial Confinement Fusion Implosions. United States. https://doi.org/10.1103/physrevlett.122.035001
Sio, Hong, Frenje, J. A., Le, Ari Yitzchak, Atzeni, S., Kwan, Thomas J. T, Gatu Johnson, M., Kagan, Grigory, Stoeckl, C., Li, C. K., Parker, C. E., Forrest, C. J., Glebov, V., Kabadi, N. V., Bose, A., Rinderknecht, H. G., Amendt, P., Casey, D. T., Mancini, R., Taitano, William, Keenan, Brett, Simakov, Andrei N., Chacon, Luis, Regan, S. P., Sangster, T. C., Campbell, E. M., Seguin, F. H., and Petrasso, R. D. Fri .
"Observations of Multiple Nuclear Reaction Histories and Fuel-Ion Species Dynamics in Shock-Driven Inertial Confinement Fusion Implosions". United States. https://doi.org/10.1103/physrevlett.122.035001. https://www.osti.gov/servlets/purl/1657124.
@article{osti_1657124,
title = {Observations of Multiple Nuclear Reaction Histories and Fuel-Ion Species Dynamics in Shock-Driven Inertial Confinement Fusion Implosions},
author = {Sio, Hong and Frenje, J. A. and Le, Ari Yitzchak and Atzeni, S. and Kwan, Thomas J. T and Gatu Johnson, M. and Kagan, Grigory and Stoeckl, C. and Li, C. K. and Parker, C. E. and Forrest, C. J. and Glebov, V. and Kabadi, N. V. and Bose, A. and Rinderknecht, H. G. and Amendt, P. and Casey, D. T. and Mancini, R. and Taitano, William and Keenan, Brett and Simakov, Andrei N. and Chacon, Luis and Regan, S. P. and Sangster, T. C. and Campbell, E. M. and Seguin, F. H. and Petrasso, R. D.},
abstractNote = {Fuel-ion species dynamics in DT3He-gas-filled Inertial Confinement Fusion implosion is quantitatively assessed for the first time using simultaneously measured D3He and DT reaction histories. Here, these reaction histories are measured with the Particle X-ray Temporal Diagnostic, which captures the relative timing between different nuclear burns with unprecedented precision (~10 ps). The observed 50±10 ps earlier D3He reaction history timing (relative to DT) cannot be explained by average-ion hydrodynamic simulations, and is attributed to fuel-ion species separation between the D, T, and 3He ions during shock convergence and rebound. At the onset of the shock burn, inferred 3He/T fuel ratio in the burn region using the measured reaction histories is much higher as compared to the initial gas-fill ratio. As T and 3He have the same mass but different charge, these results indicate that the charge-to-mass ratio plays an important role in driving fuel-ion species separation during strong shock propagation.},
doi = {10.1103/physrevlett.122.035001},
journal = {Physical Review Letters},
number = 3,
volume = 122,
place = {United States},
year = {Fri Jan 25 00:00:00 EST 2019},
month = {Fri Jan 25 00:00:00 EST 2019}
}
Web of Science
Works referenced in this record:
Thermo-diffusion in inertially confined plasmas
journal, April 2014
- Kagan, Grigory; Tang, Xian-Zhu
- Physics Letters A, Vol. 378, Issue 21
Development and characterization of a pair of 30–40 ps x‐ray framing cameras
journal, January 1995
- Bradley, D. K.; Bell, P. M.; Landen, O. L.
- Review of Scientific Instruments, Vol. 66, Issue 1
Tests of the hydrodynamic equivalence of direct-drive implosions with different D2 and He3 mixtures
journal, May 2006
- Rygg, J. R.; Frenje, J. A.; Li, C. K.
- Physics of Plasmas, Vol. 13, Issue 5
Observations of the collapse of asymmetrically driven convergent shocks
journal, March 2008
- Rygg, J. R.; Frenje, J. A.; Li, C. K.
- Physics of Plasmas, Vol. 15, Issue 3
Direct-drive-implosion experiments with enhanced fluence balance on OMEGA
journal, January 2004
- Marshall, F. J.; Delettrez, J. A.; Epstein, R.
- Physics of Plasmas, Vol. 11, Issue 1
Assessment of ion kinetic effects in shock-driven inertial confinement fusion implosions using fusion burn imaging
journal, June 2015
- Rosenberg, M. J.; Séguin, F. H.; Amendt, P. A.
- Physics of Plasmas, Vol. 22, Issue 6
Ion-kinetic simulations of D- 3 He gas-filled inertial confinement fusion target implosions with moderate to large Knudsen number
journal, January 2016
- Larroche, O.; Rinderknecht, H. G.; Rosenberg, M. J.
- Physics of Plasmas, Vol. 23, Issue 1
Evidence for Stratification of Deuterium-Tritium Fuel in Inertial Confinement Fusion Implosions
journal, February 2012
- Casey, D. T.; Frenje, J. A.; Gatu Johnson, M.
- Physical Review Letters, Vol. 108, Issue 7
Fluid and kinetic simulation of inertial confinement fusion plasmas
journal, July 2005
- Atzeni, S.; Schiavi, A.; Califano, F.
- Computer Physics Communications, Vol. 169, Issue 1-3
A mass, momentum, and energy conserving, fully implicit, scalable algorithm for the multi-dimensional, multi-species Rosenbluth–Fokker–Planck equation
journal, September 2015
- Taitano, W. T.; Chacón, L.; Simakov, A. N.
- Journal of Computational Physics, Vol. 297
Hard x-ray detectors for OMEGA and NIF
journal, January 2001
- Stoeckl, C.; Glebov, V. Yu.; Meyerhofer, D. D.
- Review of Scientific Instruments, Vol. 72, Issue 1
Initial performance results of the OMEGA laser system
journal, January 1997
- Boehly, T. R.; Brown, D. L.; Craxton, R. S.
- Optics Communications, Vol. 133, Issue 1-6
Species separation and kinetic effects in collisional plasma shocks
journal, May 2014
- Bellei, C.; Rinderknecht, H.; Zylstra, A.
- Physics of Plasmas, Vol. 21, Issue 5
Thermonuclear reactions probed at stellar-core conditions with laser-based inertial-confinement fusion
journal, August 2017
- Casey, D. T.; Sayre, D. B.; Brune, C. R.
- Nature Physics, Vol. 13, Issue 12
Electro-diffusion in a plasma with two ion species
journal, August 2012
- Kagan, Grigory; Tang, Xian-Zhu
- Physics of Plasmas, Vol. 19, Issue 8
Species separation in inertial confinement fusion fuels
journal, January 2013
- Bellei, C.; Amendt, P. A.; Wilks, S. C.
- Physics of Plasmas, Vol. 20, Issue 1
Exploding pusher performance − A theoretical model
journal, January 1979
- Rosen, M. D.; Nuckolls, J. H.
- Physics of Fluids, Vol. 22, Issue 7
Observation of interspecies ion separation in inertial-confinement-fusion implosions
journal, September 2016
- Hsu, S. C.; Joshi, T. R.; Hakel, P.
- EPL (Europhysics Letters), Vol. 115, Issue 6
Effect of laser illumination nonuniformity on the analysis of time-resolved x-ray measurements in uv spherical transport experiments
journal, October 1987
- Delettrez, J.; Epstein, R.; Richardson, M. C.
- Physical Review A, Vol. 36, Issue 8
Development of the indirect‐drive approach to inertial confinement fusion and the target physics basis for ignition and gain
journal, November 1995
- Lindl, John
- Physics of Plasmas, Vol. 2, Issue 11
The physics basis for ignition using indirect-drive targets on the National Ignition Facility
journal, February 2004
- Lindl, John D.; Amendt, Peter; Berger, Richard L.
- Physics of Plasmas, Vol. 11, Issue 2
Anomalous yield reduction in direct-drive deuterium/tritium implosions due to H3e addition
journal, May 2009
- Herrmann, H. W.; Langenbrunner, J. R.; Mack, J. M.
- Physics of Plasmas, Vol. 16, Issue 5
Observation of a Reflected Shock in an Indirectly Driven Spherical Implosion at the National Ignition Facility
journal, June 2014
- Le Pape, S.; Divol, L.; Berzak Hopkins, L.
- Physical Review Letters, Vol. 112, Issue 22
Model equation-of-state for any material in conditions relevant to ICF and to stellar interiors
journal, August 1986
- Atzeni, S.; Caruso, A.; Pais, V. A.
- Laser and Particle Beams, Vol. 4, Issue 3-4
Ion Thermal Decoupling and Species Separation in Shock-Driven Implosions
journal, January 2015
- Rinderknecht, Hans G.; Rosenberg, M. J.; Li, C. K.
- Physical Review Letters, Vol. 114, Issue 2
A Chandra View of the Morphological and Spectral Evolution of Supernova Remnant 1987A
journal, July 2004
- Park, Sangwook; Zhekov, Svetozar A.; Burrows, David N.
- The Astrophysical Journal, Vol. 610, Issue 1
Implementation of an non-iterative implicit electromagnetic field solver for dense plasma simulation
journal, December 2004
- Welch, D. R.; Rose, D. V.; Clark, R. E.
- Computer Physics Communications, Vol. 164, Issue 1-3
First Measurements of Deuterium-Tritium and Deuterium-Deuterium Fusion Reaction Yields in Ignition-Scalable Direct-Drive Implosions
journal, March 2017
- Forrest, C. J.; Radha, P. B.; Knauer, J. P.
- Physical Review Letters, Vol. 118, Issue 9
Plasma Barodiffusion in Inertial-Confinement-Fusion Implosions: Application to Observed Yield Anomalies in Thermonuclear Fuel Mixtures
journal, September 2010
- Amendt, Peter; Landen, O. L.; Robey, H. F.
- Physical Review Letters, Vol. 105, Issue 11
Simulation and assessment of ion kinetic effects in a direct-drive capsule implosion experiment
journal, October 2016
- Le, A.; Kwan, T. J. T.; Schmitt, M. J.
- Physics of Plasmas, Vol. 23, Issue 10
Kinetic physics in ICF: present understanding and future directions
journal, April 2018
- Rinderknecht, Hans G.; Amendt, P. A.; Wilks, S. C.
- Plasma Physics and Controlled Fusion, Vol. 60, Issue 6
A Particle X-ray Temporal Diagnostic (PXTD) for studies of kinetic, multi-ion effects, and ion-electron equilibration rates in Inertial Confinement Fusion plasmas at OMEGA (invited)
journal, September 2016
- Sio, H.; Frenje, J. A.; Katz, J.
- Review of Scientific Instruments, Vol. 87, Issue 11
Approximate models for the ion-kinetic regime in inertial-confinement-fusion capsule implosions
journal, May 2015
- Hoffman, Nelson M.; Zimmerman, George B.; Molvig, Kim
- Physics of Plasmas, Vol. 22, Issue 5
Stability of imploding shocks in the CCW approximation
journal, January 1982
- Gardner, John H.; Book, David L.; Bernstein, Ira B.
- Journal of Fluid Mechanics, Vol. 114, Issue -1
HYADES—A plasma hydrodynamics code for dense plasma studies
journal, January 1994
- Larsen, Jon T.; Lane, Stephen M.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 51, Issue 1-2
Electro-diffusion in a plasma with two ion species
text, January 2012
- Kagan, Grigory; Tang, Xian-Zhu
- arXiv
Works referencing / citing this record:
Nuclear diagnostics for Inertial Confinement Fusion (ICF) plasmas
journal, January 2020
- Frenje, J. A.
- Plasma Physics and Controlled Fusion, Vol. 62, Issue 2
Kinetic simulations of fusion ignition with hot-spot ablator mix
journal, September 2019
- Sadler, James D.; Lu, Yingchao; Spiers, Benjamin
- Physical Review E, Vol. 100, Issue 3
Probing ion species separation and ion thermal decoupling in shock-driven implosions using multiple nuclear reaction histories
journal, July 2019
- Sio, H.; Larroche, O.; Atzeni, S.
- Physics of Plasmas, Vol. 26, Issue 7
Universal relationship of compression shocks in two-dimensional Yukawa systems
journal, January 2020
- Lin, Wei; Murillo, M. S.; Feng, Yan
- Physical Review E, Vol. 101, Issue 1