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Title: In situ TEM investigation of self-ion irradiation of nanoporous gold

Abstract

The ability of nanoporous metals to avoid accumulation of damage under ion beam irradiation has been the focus of several studies in recent years. The width of the interconnected ligaments forming the network structure typically is on the order of tens of nanometers. In such confined volumes with high amounts of surface area, the accumulation of damage (defects such as stacking-fault tetrahedra and dislocation loops) can be mitigated via migration and annihilation of these defects at the free surfaces. Here, in situ characterization of radiation damage in nanoporous gold (np-Au) was performed in the transmission electron microscope. Several samples with varying average ligament size were subjected to gold ion beams having three different energies (10 MeV, 1.7 MeV and 46 keV). The inherent radiation tolerance of np-Au was directly observed in real time, for all ion beam conditions, and the degree of ion-induced damage accumulation in np-Au ligaments is discussed here.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [2]; ORCiD logo [1]
+ Show Author Affiliations
  1. Univ. of Kentucky, Lexington, KY (United States). Dept. of Chemical and Materials Engineering
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA); National Science Foundation (NSF)
OSTI Identifier:
1650171
Report Number(s):
SAND-2020-8427J
Journal ID: ISSN 0022-2461; 689937
Grant/Contract Number:  
AC04-94AL85000; NA-0003525; 1355438
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Materials Science
Additional Journal Information:
Journal Volume: 54; Journal Issue: 9; Journal ID: ISSN 0022-2461
Publisher:
Springer
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Briot, Nicolas J., Kosmidou, Maria, Dingreville, Rémi, Hattar, Khalid, and Balk, T. John. In situ TEM investigation of self-ion irradiation of nanoporous gold. United States: N. p., 2019. Web. doi:10.1007/s10853-019-03385-z.
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Briot, Nicolas J., Kosmidou, Maria, Dingreville, Rémi, Hattar, Khalid, & Balk, T. John. In situ TEM investigation of self-ion irradiation of nanoporous gold. United States. https://doi.org/10.1007/s10853-019-03385-z
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Briot, Nicolas J., Kosmidou, Maria, Dingreville, Rémi, Hattar, Khalid, and Balk, T. John. Wed . "In situ TEM investigation of self-ion irradiation of nanoporous gold". United States. https://doi.org/10.1007/s10853-019-03385-z. https://www.osti.gov/servlets/purl/1650171.
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@article{osti_1650171,
title = {In situ TEM investigation of self-ion irradiation of nanoporous gold},
author = {Briot, Nicolas J. and Kosmidou, Maria and Dingreville, Rémi and Hattar, Khalid and Balk, T. John},
abstractNote = {The ability of nanoporous metals to avoid accumulation of damage under ion beam irradiation has been the focus of several studies in recent years. The width of the interconnected ligaments forming the network structure typically is on the order of tens of nanometers. In such confined volumes with high amounts of surface area, the accumulation of damage (defects such as stacking-fault tetrahedra and dislocation loops) can be mitigated via migration and annihilation of these defects at the free surfaces. Here, in situ characterization of radiation damage in nanoporous gold (np-Au) was performed in the transmission electron microscope. Several samples with varying average ligament size were subjected to gold ion beams having three different energies (10 MeV, 1.7 MeV and 46 keV). The inherent radiation tolerance of np-Au was directly observed in real time, for all ion beam conditions, and the degree of ion-induced damage accumulation in np-Au ligaments is discussed here.},
doi = {10.1007/s10853-019-03385-z},
journal = {Journal of Materials Science},
number = 9,
volume = 54,
place = {United States},
year = {Wed Jan 30 00:00:00 EST 2019},
month = {Wed Jan 30 00:00:00 EST 2019}
}
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Publisher's Version of Record
https://doi.org/10.1007/s10853-019-03385-z
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    Works referencing / citing this record:

    Electronic heat transport versus atomic heating in irradiated short metallic nanowires
    journal, October 2019

    Amorphous intergranular films mitigate radiation damage in nanocrystalline Cu-Zr
    journal, March 2020

    Amorphous intergranular films mitigate radiation damage in nanocrystalline Cu-Zr
    preprint, January 2019

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