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Title: Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses

Abstract

Ultrafast electron transfer in dissociating iodomethane and fluoromethane molecules was studied at the Linac Coherent Light Source free-electron laser using an ultraviolet pump, X-ray-probe scheme. The results for both molecules are discussed with respect to the nature of their UV excitation and different chemical properties. Signatures of long distance intramolecular charge transfer are observed for both species, and a quantitative analysis of its distance dependence in iodomethane is carried out for charge states up to I 21þ. The reconstructed critical distances for electron transfer are in good agreement with a classical over-the-barrier model and with an earlier experiment employing a near infrared pump pulse. VC 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http:// creativecommons.org/licenses/by/4.0/). [http://dx.doi.org/10.1063/1.4944344]

Authors:
 [1];  [2];  [3];  [4];  [2];  [3];  [5];  [3];  [3];  [6];  [7];  [8];  [9];  [10];  [3];  [11];  [8];  [11];  [12];  [13] more »;  [14];  [15];  [5] « less
+ Show Author Affiliations
  1. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Max Planck Inst. fuer Kernphysik, Heidelberg (Germany)
  2. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science; Univ. of Hamburg (Germany). Center for Ultrafast Imaging
  5. Kansas State Univ., Manhattan, KS (United States). J.R. Macdonald Lab.
  6. Max Planck Inst. for Medical Research, Heidelberg (Germany)
  7. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science; Univ. of Hamburg (Germany). Center for Ultrafast Imaging; Univ. of Hamburg (Germany). Dept. of Physics
  8. Sorbonne Univ., Paris (France). Laboratoire de Chimie Physique–Matiere et Rayonnement. CNRS
  9. Synchrotron SOLEIL, Gif-sur-Yvette Cedex (France). L'Orme des Merisiers; Horia Hulubei National Inst.for Physics and Nuclear Engineering, Ilfov (Romania). Extreme Light Infrastructure – Nuclear Physics
  10. Synchrotron SOLEIL, Gif-sur-Yvette Cedex (France). L'Orme des Merisiers; Univ. of Oulu (Finland). Molecular Materials Research Community
  11. SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  12. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Max Planck Inst. for Biophysical Chemistry, Göttingen (Germany); Univ. of Göttingen (Germany). Inst. of X-ray Physics
  13. Tohoku Univ., Sendai (Japan). IMRAM
  14. SLAC National Accelerator Lab., Menlo Park, CA (United States); Argonne National Lab. (ANL), Argonne, IL (United States); Northwestern Univ., Evanston, IL (United States). Dept. of Physics and Astronomy
  15. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Kansas State Univ., Manhattan, KS (United States). J.R. Macdonald Lab.
Publication Date:
Research Org.:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division
OSTI Identifier:
1624995
Grant/Contract Number:  
AC02-76SF00515; AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Structural Dynamics
Additional Journal Information:
Journal Volume: 3; Journal Issue: 4; Journal ID: ISSN 2329-7778
Publisher:
American Crystallographic Association/AIP
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Chemistry; Physics

Citation Formats

Boll, Rebecca, Erk, Benjamin, Coffee, Ryan, Kierspel, Thomas, Bomme, Cédric, Bozek, John D., Burkett, Mitchell, Carron, Sebastian, Ferguson, Ken R., Foucar, Lutz, Küpper, Jochen, Marchenko, Tatiana, Miron, Catalin, Patanen, Minna, Osipov, Timur, Schorb, Sebastian, Simon, Marc, Swiggers, Michelle, Techert, Simone, Ueda, Kiyoshi, Bostedt, Christoph, Rolles, Daniel, and Rudenko, Artem. Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses. United States: N. p., 2016. Web. doi:10.1063/1.4944344.
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Boll, Rebecca, Erk, Benjamin, Coffee, Ryan, Kierspel, Thomas, Bomme, Cédric, Bozek, John D., Burkett, Mitchell, Carron, Sebastian, Ferguson, Ken R., Foucar, Lutz, Küpper, Jochen, Marchenko, Tatiana, Miron, Catalin, Patanen, Minna, Osipov, Timur, Schorb, Sebastian, Simon, Marc, Swiggers, Michelle, Techert, Simone, Ueda, Kiyoshi, Bostedt, Christoph, Rolles, Daniel, & Rudenko, Artem. Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses. United States. https://doi.org/10.1063/1.4944344
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Boll, Rebecca, Erk, Benjamin, Coffee, Ryan, Kierspel, Thomas, Bomme, Cédric, Bozek, John D., Burkett, Mitchell, Carron, Sebastian, Ferguson, Ken R., Foucar, Lutz, Küpper, Jochen, Marchenko, Tatiana, Miron, Catalin, Patanen, Minna, Osipov, Timur, Schorb, Sebastian, Simon, Marc, Swiggers, Michelle, Techert, Simone, Ueda, Kiyoshi, Bostedt, Christoph, Rolles, Daniel, and Rudenko, Artem. Fri . "Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses". United States. https://doi.org/10.1063/1.4944344. https://www.osti.gov/servlets/purl/1624995.
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@article{osti_1624995,
title = {Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses},
author = {Boll, Rebecca and Erk, Benjamin and Coffee, Ryan and Kierspel, Thomas and Bomme, Cédric and Bozek, John D. and Burkett, Mitchell and Carron, Sebastian and Ferguson, Ken R. and Foucar, Lutz and Küpper, Jochen and Marchenko, Tatiana and Miron, Catalin and Patanen, Minna and Osipov, Timur and Schorb, Sebastian and Simon, Marc and Swiggers, Michelle and Techert, Simone and Ueda, Kiyoshi and Bostedt, Christoph and Rolles, Daniel and Rudenko, Artem},
abstractNote = {Ultrafast electron transfer in dissociating iodomethane and fluoromethane molecules was studied at the Linac Coherent Light Source free-electron laser using an ultraviolet pump, X-ray-probe scheme. The results for both molecules are discussed with respect to the nature of their UV excitation and different chemical properties. Signatures of long distance intramolecular charge transfer are observed for both species, and a quantitative analysis of its distance dependence in iodomethane is carried out for charge states up to I 21þ. The reconstructed critical distances for electron transfer are in good agreement with a classical over-the-barrier model and with an earlier experiment employing a near infrared pump pulse. VC 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http:// creativecommons.org/licenses/by/4.0/). [http://dx.doi.org/10.1063/1.4944344]},
doi = {10.1063/1.4944344},
journal = {Structural Dynamics},
number = 4,
volume = 3,
place = {United States},
year = {Fri Mar 25 00:00:00 EDT 2016},
month = {Fri Mar 25 00:00:00 EDT 2016}
}
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    journal, October 2018

    • Forbes, Ruaridh; De Fanis, Alberto; Bomme, Cédric
    • The Journal of Chemical Physics, Vol. 149, Issue 14
    • DOI: 10.1063/1.5035496

    Photoionization of the iodine 3d, 4s, and 4p orbitals in methyl iodide
    text, January 2018

    • Forbes, Ruaridh; De Fanis, Alberto; Bomme, Cedric
    • Deutsches Elektronen-Synchrotron, DESY, Hamburg
    • DOI: 10.3204/pubdb-2019-00088

    Theoretical evidence for the sensitivity of charge-rearrangement-enhanced x-ray ionization to molecular size
    journal, July 2019

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