Configurable topological textures in strain graded ferroelectric nanoplates
Abstract
Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much as 105m-1) associated with misfit strain relaxation enables five discrete levels for the ferroelectric topological invariant of the entire system because of its peculiar radial quadrant domain texture and its inherent domain wall chirality. The total winding number of the topological texture can be configured from-1 to 3 by selective non-local electric switching of the quadrant domains. By using angle-resolved piezoresponse force microscopy in conjunction with local winding number analysis, we directly identify the existence of vortices and anti-vortices, observe pair creation and annihilation and manipulate the net number of vortices. Our findings offer a useful concept for multi-level topological defect memory.
- Authors:
-
- Korea Advanced Institute of Science and Technology (KAIST), Dept. of Physics, Yuseong-gu, Daejeon, 34141, Republic of Korea
- Korea Inst. of Materials Science, Dept. of Materials Modelling and Characterization, Changwon, Gyeongnam, 51508, Republic of Korea; Pusan National Univ., Dept. of Materials Science and Engineering, Geumjeong-gu, Busan, 46241, Republic of Korea
- The Pennsylvania State Univ., Department of Materials Science and Engineering, University Park, PA, 16802, (United States)
- Pohang Accelerator Laboratory, POSTECH, Pohang, Gyeongbuk, 37673, Republic of Korea
- Korea Inst. of Materials Science, Dept. of Materials Modelling and Characterization, Changwon, Gyeongnam, 51508, Republic of Korea; POSTECH, Dept. of Materials Science and Engineering, Pohang, Gyeongbuk, 37673, Republic of Korea
- Univ. of California, Dept. of Materials Science and Engineering/Dept. of Physics, Berkeley, CA, 94720, (United States); Lawrence Berkeley National Lab (LBNL), Berkeley, CA 94720 (United States)
- Korea Advanced Institute of Science and Technology (KAIST), Dept. of Physics, Yuseong-gu, Daejeon, 34141, Republic of Korea; KAIST Institute for the NanoCentury, KAIST, Yuseong-gu, Daejeon, 34141, Republic of Korea
- Publication Date:
- Research Org.:
- Pennsylvania State Univ., University Park, PA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Research Foundation (NRF), Korean Government; Creative Research Initiative Center for Lattice Defectronics; Center for Quantum Coherence in Condensed Matter; Global Frontier R&D Program on Center for Hybrid Interface Materials (HIM), Ministry of Science, ICT & Future Planning; National Science Foundation (NSF); Penn State MRSEC, Center for Nanoscale Science
- OSTI Identifier:
- 1624072
- Grant/Contract Number:
- FG02-07ER46417
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- Science & Technology - Other Topics
Citation Formats
Kim, Kwang-Eun, Jeong, Seuri, Chu, Kanghyun, Lee, Jin Hong, Kim, Gi-Yeop, Xue, Fei, Koo, Tae Yeong, Chen, Long-Qing, Choi, Si-Young, Ramesh, Ramamoorthy, and Yang, Chan-Ho. Configurable topological textures in strain graded ferroelectric nanoplates. United States: N. p., 2018.
Web. doi:10.1038/s41467-017-02813-5.
Kim, Kwang-Eun, Jeong, Seuri, Chu, Kanghyun, Lee, Jin Hong, Kim, Gi-Yeop, Xue, Fei, Koo, Tae Yeong, Chen, Long-Qing, Choi, Si-Young, Ramesh, Ramamoorthy, & Yang, Chan-Ho. Configurable topological textures in strain graded ferroelectric nanoplates. United States. https://doi.org/10.1038/s41467-017-02813-5
Kim, Kwang-Eun, Jeong, Seuri, Chu, Kanghyun, Lee, Jin Hong, Kim, Gi-Yeop, Xue, Fei, Koo, Tae Yeong, Chen, Long-Qing, Choi, Si-Young, Ramesh, Ramamoorthy, and Yang, Chan-Ho. Fri .
"Configurable topological textures in strain graded ferroelectric nanoplates". United States. https://doi.org/10.1038/s41467-017-02813-5. https://www.osti.gov/servlets/purl/1624072.
@article{osti_1624072,
title = {Configurable topological textures in strain graded ferroelectric nanoplates},
author = {Kim, Kwang-Eun and Jeong, Seuri and Chu, Kanghyun and Lee, Jin Hong and Kim, Gi-Yeop and Xue, Fei and Koo, Tae Yeong and Chen, Long-Qing and Choi, Si-Young and Ramesh, Ramamoorthy and Yang, Chan-Ho},
abstractNote = {Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much as 105m-1) associated with misfit strain relaxation enables five discrete levels for the ferroelectric topological invariant of the entire system because of its peculiar radial quadrant domain texture and its inherent domain wall chirality. The total winding number of the topological texture can be configured from-1 to 3 by selective non-local electric switching of the quadrant domains. By using angle-resolved piezoresponse force microscopy in conjunction with local winding number analysis, we directly identify the existence of vortices and anti-vortices, observe pair creation and annihilation and manipulate the net number of vortices. Our findings offer a useful concept for multi-level topological defect memory.},
doi = {10.1038/s41467-017-02813-5},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Fri Jan 26 00:00:00 EST 2018},
month = {Fri Jan 26 00:00:00 EST 2018}
}
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