Imaging an aligned polyatomic molecule with laser-induced electron diffraction
Abstract
Laser-induced electron diffraction is an evolving tabletop method that aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-Ångstro¨m spatial and femtosecond temporal resolutions. Here we demonstrate the retrieval of multiple bond lengths from a polyatomic molecule by simultaneously measuring the C–C and C–H bond lengths in aligned acetylene. Our approach takes the method beyond the hitherto achieved imaging of simple diatomic molecules and is based on the combination of a 160 kHz mid-infrared few-cycle laser source with full three-dimensional electron–ion coincidence detection. Our technique provides an accessible and robust route towards imaging ultrafast processes in complex gas-phase molecules with atto- to femto-second temporal resolution.
- Authors:
-
[1];
- Inst. de Ciencies Fotoniques (ICFO), Barcelona (Spain)
- Kansas State Univ., Manhattan, KS (United States)
- Univ. Kassel (Germany)
- Max-Planck-Inst. für Kernphysik, Heidelberg (Germany)
- Max-Planck-Inst. für Kernphysik, Heidelberg (Germany); Physikalisch-Technische Bundesanstalt (PTB), Braunschweig (Germany)
- Inst. de Ciencies Fotoniques (ICFO), Barcelona (Spain); Univ. of New Mexico, Albuquerque, NM (United States); Inst. Catalana de Recerca i Estudis Avançats (ICREA), Barcelona (Spain)
- Publication Date:
- Research Org.:
- Kansas State Univ., Manhattan, KS (United States)
- Sponsoring Org.:
- Ministerio de Economía y Competitividad (MINECO); Catalan Agencia de Gestio´ d’Ajuts Universitaris i de Recerca (AGAUR); Fundació Cellex Barcelona; Laserlab-Europe; European Commission (EC); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division
- OSTI Identifier:
- 1623980
- Grant/Contract Number:
- FG02-86ER13491; 228334
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 6; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; science & technology - other topics; atomic and molecular physics; imaging and sensing; lasers, LEDS and light sources
Citation Formats
Pullen, Michael G., Wolter, Benjamin, Le, Anh-Thu, Baudisch, Matthias, Hemmer, Michaël, Senftleben, Arne, Schröter, Claus Dieter, Ullrich, Joachim, Moshammer, Robert, Lin, C. D., and Biegert, Jens. Imaging an aligned polyatomic molecule with laser-induced electron diffraction. United States: N. p., 2015.
Web. doi:10.1038/ncomms8262.
Pullen, Michael G., Wolter, Benjamin, Le, Anh-Thu, Baudisch, Matthias, Hemmer, Michaël, Senftleben, Arne, Schröter, Claus Dieter, Ullrich, Joachim, Moshammer, Robert, Lin, C. D., & Biegert, Jens. Imaging an aligned polyatomic molecule with laser-induced electron diffraction. United States. https://doi.org/10.1038/ncomms8262
Pullen, Michael G., Wolter, Benjamin, Le, Anh-Thu, Baudisch, Matthias, Hemmer, Michaël, Senftleben, Arne, Schröter, Claus Dieter, Ullrich, Joachim, Moshammer, Robert, Lin, C. D., and Biegert, Jens. Wed .
"Imaging an aligned polyatomic molecule with laser-induced electron diffraction". United States. https://doi.org/10.1038/ncomms8262. https://www.osti.gov/servlets/purl/1623980.
@article{osti_1623980,
title = {Imaging an aligned polyatomic molecule with laser-induced electron diffraction},
author = {Pullen, Michael G. and Wolter, Benjamin and Le, Anh-Thu and Baudisch, Matthias and Hemmer, Michaël and Senftleben, Arne and Schröter, Claus Dieter and Ullrich, Joachim and Moshammer, Robert and Lin, C. D. and Biegert, Jens},
abstractNote = {Laser-induced electron diffraction is an evolving tabletop method that aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-Ångstro¨m spatial and femtosecond temporal resolutions. Here we demonstrate the retrieval of multiple bond lengths from a polyatomic molecule by simultaneously measuring the C–C and C–H bond lengths in aligned acetylene. Our approach takes the method beyond the hitherto achieved imaging of simple diatomic molecules and is based on the combination of a 160 kHz mid-infrared few-cycle laser source with full three-dimensional electron–ion coincidence detection. Our technique provides an accessible and robust route towards imaging ultrafast processes in complex gas-phase molecules with atto- to femto-second temporal resolution.},
doi = {10.1038/ncomms8262},
journal = {Nature Communications},
number = 1,
volume = 6,
place = {United States},
year = {Wed Jun 24 00:00:00 EDT 2015},
month = {Wed Jun 24 00:00:00 EDT 2015}
}
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Figure 1: Laser-induced electron diffraction from aligned C2H2 molecules using a mid-infrared OPCPA source and a reaction microscope. The cartoon film shows the procedure. (a) The C2H2 molecules are pre-aligned by focusing the 1.7μm pump pulse (blue) into a molecular jet. (b) The 3.1 μm pulse (red) is used tomore »
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text, January 2018
- Chatterley, Adam S.; Schouder, Constant; Christiansen, Lars
- arXiv
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