Giant reversible barocaloric response of (MnNiSi)1-x (FeCoGe)x (x = 0.39, 0.40, 0.41)
Abstract
MnNiSi-based alloys and isostructural systems have traditionally demonstrated impressive magnetocaloric properties near room temperature associated with a highly tunable first-order magnetostructural transition that involves large latent heat. However, these materials are limited by a small field-sensitivity of the transition, preventing significant reversible effects usable for cooling applications. Instead, the concomitant large transition volume changes prompt a high pressure-sensitivity, and therefore, promise substantial barocaloric performances, but they have been sparsely studied in these materials. Here, we study the barocaloric response in a series of composition-related (MnNiSi)1-x(FeCoGe)x (x = 0.39, 0.40, 0.41) alloys that span continuously over a wide temperature range around ambient. We report on giant reversible effects of ~40 J K-1 kg-1 and up to ~4 K upon application of ~2 kbar and find a degradation of the first-order transition properties with pressure that limits the barocaloric effects at high pressures. Our results confirm the potential of this type of alloys for barocaloric applications, where multicaloric and composite possibilities, along with the high density and relatively high thermal conductivity, constructively add to the magnitude of the caloric effects.
- Authors:
-
[1];
[1];
[1];
- Univ. Politècnica de Catalunya, Barcelona, Catalonia (Spain). Campus Diagonal-Besòs, Barcelona Research Center in Multiscale Science and Engineering
- Louisiana State Univ., Baton Rouge, LA (United States)
- Southern Illinois Univ., Carbondale, IL (United States)
- Publication Date:
- Research Org.:
- Southern Illinois Univ., Carbondale, IL (United States); Louisiana State Univ., Baton Rouge, LA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Ministry of Economic Affairs and Digital Transformation of Spain (MINECO)
- OSTI Identifier:
- 1609723
- Alternate Identifier(s):
- OSTI ID: 1529409; OSTI ID: 1872897
- Grant/Contract Number:
- FG02-06ER46291; SC0010521; FG02-13ER46946
- Resource Type:
- Accepted Manuscript
- Journal Name:
- APL Materials
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 6; Journal ID: ISSN 2166-532X
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Thermodynamic properties; Thermodynamic measurements and instrumentation; Calorimetry; Alloys; Entropy; X-ray diffraction; Compressors; Refrigerators; Phase transitions; Magnetic ordering; 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATION; barocaloric effect; magnetocaloric effect; phase transitions
Citation Formats
Lloveras, Pol, Samanta, Tapas, Barrio, María, Dubenko, Igor, Ali, Naushad, Tamarit, Josep-Lluís, and Stadler, Shane. Giant reversible barocaloric response of (MnNiSi)1-x (FeCoGe)x (x = 0.39, 0.40, 0.41). United States: N. p., 2019.
Web. doi:10.1063/1.5097959.
Lloveras, Pol, Samanta, Tapas, Barrio, María, Dubenko, Igor, Ali, Naushad, Tamarit, Josep-Lluís, & Stadler, Shane. Giant reversible barocaloric response of (MnNiSi)1-x (FeCoGe)x (x = 0.39, 0.40, 0.41). United States. https://doi.org/10.1063/1.5097959
Lloveras, Pol, Samanta, Tapas, Barrio, María, Dubenko, Igor, Ali, Naushad, Tamarit, Josep-Lluís, and Stadler, Shane. Tue .
"Giant reversible barocaloric response of (MnNiSi)1-x (FeCoGe)x (x = 0.39, 0.40, 0.41)". United States. https://doi.org/10.1063/1.5097959. https://www.osti.gov/servlets/purl/1609723.
@article{osti_1609723,
title = {Giant reversible barocaloric response of (MnNiSi)1-x (FeCoGe)x (x = 0.39, 0.40, 0.41)},
author = {Lloveras, Pol and Samanta, Tapas and Barrio, María and Dubenko, Igor and Ali, Naushad and Tamarit, Josep-Lluís and Stadler, Shane},
abstractNote = {MnNiSi-based alloys and isostructural systems have traditionally demonstrated impressive magnetocaloric properties near room temperature associated with a highly tunable first-order magnetostructural transition that involves large latent heat. However, these materials are limited by a small field-sensitivity of the transition, preventing significant reversible effects usable for cooling applications. Instead, the concomitant large transition volume changes prompt a high pressure-sensitivity, and therefore, promise substantial barocaloric performances, but they have been sparsely studied in these materials. Here, we study the barocaloric response in a series of composition-related (MnNiSi)1-x(FeCoGe)x (x = 0.39, 0.40, 0.41) alloys that span continuously over a wide temperature range around ambient. We report on giant reversible effects of ~40 J K-1 kg-1 and up to ~4 K upon application of ~2 kbar and find a degradation of the first-order transition properties with pressure that limits the barocaloric effects at high pressures. Our results confirm the potential of this type of alloys for barocaloric applications, where multicaloric and composite possibilities, along with the high density and relatively high thermal conductivity, constructively add to the magnitude of the caloric effects.},
doi = {10.1063/1.5097959},
journal = {APL Materials},
number = 6,
volume = 7,
place = {United States},
year = {Tue Jun 25 00:00:00 EDT 2019},
month = {Tue Jun 25 00:00:00 EDT 2019}
}
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