Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials
Abstract
Topologically nontrivial two-dimensional materials hold great promise for next-generation optoelectronic applications. However, measuring the Hall or spin-Hall response is often a challenge and practically limited to the ground state. An experimental technique for tracing the topological character in a differential fashion would provide useful insights. In this work, we show that circular dichroism angle-resolved photoelectron spectroscopy provides a powerful tool that can resolve the topological and quantum-geometrical character in momentum space. In particular, we investigate how to map out the signatures of the momentum-resolved Berry curvature in two-dimensional materials by exploiting its intimate connection to the orbital polarization. A spin-resolved detection of the photoelectrons allows one to extend the approach to spin-Chern insulators. The present proposal can be extended to address topological properties in materials out of equilibrium in a time-resolved fashion.
- Authors:
-
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. of Fribourg (Switzerland)
- Max Planck Inst. for the Structure and Dynamics of Matter, Hamburg (Germany)
- Max Planck Inst. for the Structure and Dynamics of Matter, Hamburg (Germany); The Flatiron Inst., New York, NY (United States)
- Univ. of Fribourg (Switzerland)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE; Swiss National Science Foundation (SNSF)
- OSTI Identifier:
- 1608948
- Grant/Contract Number:
- AC02-76SF00515; 724103; ERC-2015-AdG-694097
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Science Advances
- Additional Journal Information:
- Journal Volume: 6; Journal Issue: 9; Journal ID: ISSN 2375-2548
- Publisher:
- AAAS
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Schüler, Michael, De Giovannini, Umberto, Hübener, Hannes, Rubio, Angel, Sentef, Michael A., and Werner, Philipp. Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials. United States: N. p., 2020.
Web. doi:10.1126/sciadv.aay2730.
Schüler, Michael, De Giovannini, Umberto, Hübener, Hannes, Rubio, Angel, Sentef, Michael A., & Werner, Philipp. Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials. United States. https://doi.org/10.1126/sciadv.aay2730
Schüler, Michael, De Giovannini, Umberto, Hübener, Hannes, Rubio, Angel, Sentef, Michael A., and Werner, Philipp. Fri .
"Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials". United States. https://doi.org/10.1126/sciadv.aay2730. https://www.osti.gov/servlets/purl/1608948.
@article{osti_1608948,
title = {Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials},
author = {Schüler, Michael and De Giovannini, Umberto and Hübener, Hannes and Rubio, Angel and Sentef, Michael A. and Werner, Philipp},
abstractNote = {Topologically nontrivial two-dimensional materials hold great promise for next-generation optoelectronic applications. However, measuring the Hall or spin-Hall response is often a challenge and practically limited to the ground state. An experimental technique for tracing the topological character in a differential fashion would provide useful insights. In this work, we show that circular dichroism angle-resolved photoelectron spectroscopy provides a powerful tool that can resolve the topological and quantum-geometrical character in momentum space. In particular, we investigate how to map out the signatures of the momentum-resolved Berry curvature in two-dimensional materials by exploiting its intimate connection to the orbital polarization. A spin-resolved detection of the photoelectrons allows one to extend the approach to spin-Chern insulators. The present proposal can be extended to address topological properties in materials out of equilibrium in a time-resolved fashion.},
doi = {10.1126/sciadv.aay2730},
journal = {Science Advances},
number = 9,
volume = 6,
place = {United States},
year = {Fri Feb 28 00:00:00 EST 2020},
month = {Fri Feb 28 00:00:00 EST 2020}
}
Web of Science
Works referenced in this record:
Bismuthene on a SiC substrate: A candidate for a high-temperature quantum spin Hall material
journal, June 2017
- Reis, F.; Li, G.; Dudy, L.
- Science, Vol. 357, Issue 6348
Direct measurement of quantum phases in graphene via photoemission spectroscopy
journal, September 2011
- Hwang, Choongyu; Park, Cheol-Hwan; Siegel, David A.
- Physical Review B, Vol. 84, Issue 12
Topological insulators and superconductors
journal, October 2011
- Qi, Xiao-Liang; Zhang, Shou-Cheng
- Reviews of Modern Physics, Vol. 83, Issue 4
Theoretical paradigm for the quantum spin Hall effect at high temperatures
journal, October 2018
- Li, Gang; Hanke, Werner; Hankiewicz, Ewelina M.
- Physical Review B, Vol. 98, Issue 16
Hidden orbital polarization in diamond, silicon, germanium, gallium arsenide and layered materials
journal, May 2017
- Ryoo, Ji Hoon; Park, Cheol-Hwan
- NPG Asia Materials, Vol. 9, Issue 5
Two-Dimensional Topological Insulators: Progress and Prospects
journal, April 2017
- Kou, Liangzhi; Ma, Yandong; Sun, Ziqi
- The Journal of Physical Chemistry Letters, Vol. 8, Issue 8
Geometric Origin of Superfluidity in the Lieb-Lattice Flat Band
journal, July 2016
- Julku, Aleksi; Peotta, Sebastiano; Vanhala, Tuomas I.
- Physical Review Letters, Vol. 117, Issue 4
Unifying Optical Selection Rules for Excitons in Two Dimensions: Band Topology and Winding Numbers
journal, February 2018
- Cao, Ting; Wu, Meng; Louie, Steven G.
- Physical Review Letters, Vol. 120, Issue 8
Monitoring Electron-Photon Dressing in WSe 2
journal, November 2016
- De Giovannini, Umberto; Hübener, Hannes; Rubio, Angel
- Nano Letters, Vol. 16, Issue 12
Recent trends in spin-resolved photoelectron spectroscopy
journal, November 2017
- Okuda, Taichi
- Journal of Physics: Condensed Matter, Vol. 29, Issue 48
Dichroic -sum rule and the orbital magnetization of crystals
journal, February 2008
- Souza, Ivo; Vanderbilt, David
- Physical Review B, Vol. 77, Issue 5
Experimental reconstruction of the Berry curvature in a Floquet Bloch band
journal, May 2016
- Flaschner, N.; Rem, B. S.; Tarnowski, M.
- Science, Vol. 352, Issue 6289
Prediction of a Large-Gap and Switchable Kane-Mele Quantum Spin Hall Insulator
journal, March 2018
- Marrazzo, Antimo; Gibertini, Marco; Campi, Davide
- Physical Review Letters, Vol. 120, Issue 11
Measuring quantized circular dichroism in ultracold topological matter
journal, February 2019
- Asteria, Luca; Tran, Duc Thanh; Ozawa, Tomoki
- Nature Physics, Vol. 15, Issue 5
Phonon Driven Floquet Matter
journal, January 2018
- Hübener, Hannes; De Giovannini, Umberto; Rubio, Angel
- Nano Letters, Vol. 18, Issue 2
Experimental Observation of Hidden Berry Curvature in Inversion-Symmetric Bulk
journal, October 2018
- Cho, Soohyun; Park, Jin-Hong; Hong, Jisook
- Physical Review Letters, Vol. 121, Issue 18
octopus: a tool for the application of time-dependent density functional theory
journal, September 2006
- Castro, Alberto; Appel, Heiko; Oliveira, Micael
- physica status solidi (b), Vol. 243, Issue 11
Valley-dependent optoelectronics from inversion symmetry breaking
journal, June 2008
- Yao, Wang; Xiao, Di; Niu, Qian
- Physical Review B, Vol. 77, Issue 23
Universal optical control of chiral superconductors and Majorana modes
journal, May 2019
- Claassen, M.; Kennes, D. M.; Zingl, M.
- Nature Physics, Vol. 15, Issue 8
All-optical nonequilibrium pathway to stabilising magnetic Weyl semimetals in pyrochlore iridates
journal, October 2018
- Topp, Gabriel E.; Tancogne-Dejean, Nicolas; Kemper, Alexander F.
- Nature Communications, Vol. 9, Issue 1
Selective Probing of Hidden Spin-Polarized States in Inversion-Symmetric Bulk
journal, February 2017
- Razzoli, E.; Jaouen, T.; Mottas, M. -L.
- Physical Review Letters, Vol. 118, Issue 8
Simulating Pump-Probe Photoelectron and Absorption Spectroscopy on the Attosecond Timescale with Time-Dependent Density Functional Theory
journal, March 2013
- De Giovannini, Umberto; Brunetto, Gustavo; Castro, Alberto
- ChemPhysChem, Vol. 14, Issue 7
Quantum Nonlinear Hall Effect Induced by Berry Curvature Dipole in Time-Reversal Invariant Materials
journal, November 2015
- Sodemann, Inti; Fu, Liang
- Physical Review Letters, Vol. 115, Issue 21
Chiral Orbital-Angular Momentum in the Surface States of
journal, January 2012
- Park, Seung Ryong; Han, Jinhee; Kim, Chul
- Physical Review Letters, Vol. 108, Issue 4
Geometrical Description of the Fractional Quantum Hall Effect
journal, September 2011
- Haldane, F. D. M.
- Physical Review Letters, Vol. 107, Issue 11
All-optical materials design of chiral edge modes in transition-metal dichalcogenides
journal, October 2016
- Claassen, Martin; Jia, Chunjing; Moritz, Brian
- Nature Communications, Vol. 7, Issue 1
A First-Principles Time-Dependent Density Functional Theory Framework for Spin and Time-Resolved Angular-Resolved Photoelectron Spectroscopy in Periodic Systems
journal, December 2016
- De Giovannini, Umberto; Hübener, Hannes; Rubio, Angel
- Journal of Chemical Theory and Computation, Vol. 13, Issue 1
Light-induced anomalous Hall effect in graphene
journal, November 2019
- McIver, J. W.; Schulte, B.; Stein, F. -U.
- Nature Physics, Vol. 16, Issue 1
Tracing the nonequilibrium topological state of Chern insulators
journal, October 2017
- Schüler, Michael; Werner, Philipp
- Physical Review B, Vol. 96, Issue 15
Electrically switchable Berry curvature dipole in the monolayer topological insulator WTe2
journal, July 2018
- Xu, Su-Yang; Ma, Qiong; Shen, Huitao
- Nature Physics, Vol. 14, Issue 9
Hidden spin polarization in inversion-symmetric bulk crystals
journal, April 2014
- Zhang, Xiuwen; Liu, Qihang; Luo, Jun-Wei
- Nature Physics, Vol. 10, Issue 5
Probing Symmetry Properties of Few-Layer MoS 2 and h-BN by Optical Second-Harmonic Generation
journal, June 2013
- Li, Yilei; Rao, Yi; Mak, Kin Fai
- Nano Letters, Vol. 13, Issue 7
Atomic-like high-harmonic generation from two-dimensional materials
journal, February 2018
- Tancogne-Dejean, Nicolas; Rubio, Angel
- Science Advances, Vol. 4, Issue 2
Measuring the quantum geometry of Bloch bands with current noise
journal, June 2013
- Neupert, Titus; Chamon, Claudio; Mudry, Christopher
- Physical Review B, Vol. 87, Issue 24
Hall Effect in Ferromagnetics
journal, September 1954
- Karplus, Robert; Luttinger, J. M.
- Physical Review, Vol. 95, Issue 5
Fundamentals of Time-Dependent Density Functional Theory
book, January 2012
- Marques, Miguel A. L.; Maitra, Neepa T.; Nogueira, Fernando M. S.
- Lecture Notes in Physics
Quench dynamics and Hall response of interacting Chern insulators
journal, July 2019
- Schüler, Michael; Budich, Jan Carl; Werner, Philipp
- Physical Review B, Vol. 100, Issue 4
Observation of the nonlinear Hall effect under time-reversal-symmetric conditions
journal, December 2018
- Ma, Qiong; Xu, Su-Yang; Shen, Huitao
- Nature, Vol. 565, Issue 7739
Topological Order and the Quantum Spin Hall Effect
journal, September 2005
- Kane, C. L.; Mele, E. J.
- Physical Review Letters, Vol. 95, Issue 14, Article No. 146802
Relativistic separable dual-space Gaussian pseudopotentials from H to Rn
journal, August 1998
- Hartwigsen, C.; Goedecker, S.; Hutter, J.
- Physical Review B, Vol. 58, Issue 7
Colloquium: Topological insulators
journal, November 2010
- Hasan, M. Z.; Kane, C. L.
- Reviews of Modern Physics, Vol. 82, Issue 4, p. 3045-3067
Quantum Spin Hall Effect in Graphene
journal, November 2005
- Kane, C. L.; Mele, E. J.
- Physical Review Letters, Vol. 95, Issue 22
Creating stable Floquet–Weyl semimetals by laser-driving of 3D Dirac materials
journal, January 2017
- Hübener, Hannes; Sentef, Michael A.; De Giovannini, Umberto
- Nature Communications, Vol. 8, Issue 1
Spatial Separation of Carrier Spin by the Valley Hall Effect in Monolayer WSe 2 Transistors
journal, January 2019
- Barré, Elyse; Incorvia, Jean Anne C.; Kim, Suk Hyun
- Nano Letters, Vol. 19, Issue 2
Tight-binding theory of the spin-orbit coupling in graphene
journal, December 2010
- Konschuh, Sergej; Gmitra, Martin; Fabian, Jaroslav
- Physical Review B, Vol. 82, Issue 24
Chiral magnetic effect and natural optical activity in metals with or without Weyl points
journal, December 2015
- Ma, Jing; Pesin, D. A.
- Physical Review B, Vol. 92, Issue 23
Theory of Floquet band formation and local pseudospin textures in pump-probe photoemission of graphene
journal, May 2015
- Sentef, M. A.; Claassen, M.; Kemper, A. F.
- Nature Communications, Vol. 6, Issue 1
Model for a Quantum Hall Effect without Landau Levels: Condensed-Matter Realization of the "Parity Anomaly"
journal, October 1988
- Haldane, F. D. M.
- Physical Review Letters, Vol. 61, Issue 18
t -SURFF: fully differential two-electron photo-emission spectra
journal, August 2012
- Scrinzi, Armin
- New Journal of Physics, Vol. 14, Issue 8
Probing topology by “heating”: Quantized circular dichroism in ultracold atoms
journal, August 2017
- Tran, Duc Thanh; Dauphin, Alexandre; Grushin, Adolfo G.
- Science Advances, Vol. 3, Issue 8
Graphene Sublattice Symmetry and Isospin Determined by Circular Dichroism in Angle-Resolved Photoemission Spectroscopy
journal, July 2012
- Gierz, Isabella; Lindroos, Matti; Höchst, Hartmut
- Nano Letters, Vol. 12, Issue 8
Berry Curvature on the Fermi Surface: Anomalous Hall Effect as a Topological Fermi-Liquid Property
journal, November 2004
- Haldane, F. D. M.
- Physical Review Letters, Vol. 93, Issue 20
Ab initio tight-binding Hamiltonian for transition metal dichalcogenides
journal, November 2015
- Fang, Shiang; Kuate Defo, Rodrick; Shirodkar, Sharmila N.
- Physical Review B, Vol. 92, Issue 20
Circular dichroism in angle-resolved photoemission spectroscopy of topological insulators
journal, January 2013
- Wang, Yihua; Gedik, Nuh
- physica status solidi (RRL) - Rapid Research Letters, Vol. 7, Issue 1-2
Berry phase effects on electronic properties
journal, July 2010
- Xiao, Di; Chang, Ming-Che; Niu, Qian
- Reviews of Modern Physics, Vol. 82, Issue 3
Visualizing Electronic Chirality and Berry Phases in Graphene Systems Using Photoemission with Circularly Polarized Light
journal, October 2011
- Liu, Y.; Bian, G.; Miller, T.
- Physical Review Letters, Vol. 107, Issue 16
octopus: a tool for the application of time-dependent density functional theory
journal, September 2006
- Castro, Alberto; Appel, Heiko; Oliveira, Micael
- physica status solidi (b), Vol. 243, Issue 11
A First-Principles Time-Dependent Density Functional Theory Framework for Spin and Time-Resolved Angular-Resolved Photoelectron Spectroscopy in Periodic Systems
journal, December 2016
- De Giovannini, Umberto; Hübener, Hannes; Rubio, Angel
- Journal of Chemical Theory and Computation, Vol. 13, Issue 1
Two-Dimensional Topological Insulators: Progress and Prospects
journal, April 2017
- Kou, Liangzhi; Ma, Yandong; Sun, Ziqi
- The Journal of Physical Chemistry Letters, Vol. 8, Issue 8
Phonon Driven Floquet Matter
journal, January 2018
- Hübener, Hannes; De Giovannini, Umberto; Rubio, Angel
- Nano Letters, Vol. 18, Issue 2
Graphene Sublattice Symmetry and Isospin Determined by Circular Dichroism in Angle-Resolved Photoemission Spectroscopy
journal, July 2012
- Gierz, Isabella; Lindroos, Matti; Höchst, Hartmut
- Nano Letters, Vol. 12, Issue 8
Probing Symmetry Properties of Few-Layer MoS 2 and h-BN by Optical Second-Harmonic Generation
journal, June 2013
- Li, Yilei; Rao, Yi; Mak, Kin Fai
- Nano Letters, Vol. 13, Issue 7
Creating stable Floquet–Weyl semimetals by laser-driving of 3D Dirac materials
journal, January 2017
- Hübener, Hannes; Sentef, Michael A.; De Giovannini, Umberto
- Nature Communications, Vol. 8, Issue 1
Theory of Floquet band formation and local pseudospin textures in pump-probe photoemission of graphene
journal, May 2015
- Sentef, M. A.; Claassen, M.; Kemper, A. F.
- Nature Communications, Vol. 6, Issue 1
t -SURFF: fully differential two-electron photo-emission spectra
journal, August 2012
- Scrinzi, Armin
- New Journal of Physics, Vol. 14, Issue 8
Ab initio angle- and energy-resolved photoelectron spectroscopy with time-dependent density-functional theory
journal, June 2012
- De Giovannini, U.; Varsano, D.; Marques, M. A. L.
- Physical Review A, Vol. 85, Issue 6
Probing topology by “heating”: Quantized circular dichroism in ultracold atoms
journal, August 2017
- Tran, Duc Thanh; Dauphin, Alexandre; Grushin, Adolfo G.
- Science Advances, Vol. 3, Issue 8
Atomic-like high-harmonic generation from two-dimensional materials
journal, February 2018
- Tancogne-Dejean, Nicolas; Rubio, Angel
- Science Advances, Vol. 4, Issue 2
Experimental reconstruction of the Berry curvature in a Floquet Bloch band
journal, May 2016
- Flaschner, N.; Rem, B. S.; Tarnowski, M.
- Science, Vol. 352, Issue 6289
Examining electron-boson coupling using time-resolved spectroscopy
text, January 2012
- Sentef, Michael; Kemper, Alexander F.; Moritz, Brian
- arXiv
Simulating pump-probe photo-electron and absorption spectroscopy on the attosecond time-scale with time-dependent density-functional theory
text, January 2013
- De Giovannini, Umberto; Brunetto, Gustavo; Castro, Alberto
- arXiv
Chiral magnetic effect and natural optical activity in (Weyl) metals
text, January 2015
- Ma, Jing; Pesin, D. A.
- arXiv
Geometric origin of superfluidity in the Lieb lattice flat band
text, January 2016
- Julku, Aleksi; Peotta, Sebastiano; Vanhala, Tuomas
- arXiv
All-Optical Materials Design of Chiral Edge Modes in Transition-Metal Dichalcogenides
text, January 2016
- Claassen, Martin; Jia, Chunjing; Moritz, Brian
- arXiv
All-optical nonequilibrium pathway to stabilizing magnetic Weyl semimetals in pyrochlore iridates
text, January 2018
- Topp, Gabriel E.; Tancogne-Dejean, Nicolas; Kemper, Alexander F.
- arXiv
A new paradigm for the quantum spin Hall effect at high temperatures
text, January 2018
- Li, Gang; Hanke, Werner; Hankiewicz, Ewelina M.
- arXiv
Observation of the nonlinear Hall effect under time reversal symmetric conditions
text, January 2018
- Ma, Qiong; Xu, Su-Yang; Shen, Huitao
- arXiv
Universal Optical Control of Chiral Superconductors and Majorana Modes
text, January 2018
- Claassen, Martin; Kennes, Dante M.; Zingl, Manuel
- arXiv
Quench Dynamics and Hall Response of Interacting Chern Insulators
text, January 2018
- Schüler, Michael; Budich, Jan Carl; Werner, Philipp
- arXiv
Berry Curvature on the Fermi Surface: Anomalous Hall Effect as a Topological Fermi-Liquid Property
text, January 2004
- Haldane, F. D. M.
- arXiv
Tight-binding theory of the spin-orbit coupling in graphene
text, January 2010
- Konschuh, Sergej; Gmitra, Martin; Fabian, Jaroslav
- Universität Regensburg