Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations
Abstract
The interplay between crystal and solvent structure, interparticle forces and ensemble particle response dynamics governs the process of crystallization by oriented attachment (OA), yet a quantitative understanding is lacking. Using as a model system ZnO, we combine in situ TEM observations of single particle and ensemble assembly dynamics with simulations of interparticle forces and responses to relate experimentally derived interparticle potentials to the underlying interactions. We show that OA is driven by forces and torques due to a combination of electrostatic ion-solvent correlations and dipolar interactions that act at separations well beyond 5 nm. Importantly, coalignment is achieved before particles reach separations at which strong attractions drive the final jump to contact. The observed barrier to attachment is negligible, while dissipative factors in the quasi-2D confinement of the TEM fluid cell lead to abnormal diffusivities with timescales for rotation much less than for translation, thus enabling OA to dominate.
- Authors:
-
[1];
[1];
[3];
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Univ. of Washington, Seattle, WA (United States)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States); City Univ. of New York (CUNY), NY (United States)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1604768
- Report Number(s):
- PNNL-SA-148131
Journal ID: ISSN 2041-1723
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 11; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Liu, Lili, Nakouzi, Elias, Sushko, Maria L., Schenter, Gregory K., Mundy, Christopher J., Chun, Jaehun, and De Yoreo, James J. Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations. United States: N. p., 2020.
Web. doi:10.1038/s41467-020-14719-w.
Liu, Lili, Nakouzi, Elias, Sushko, Maria L., Schenter, Gregory K., Mundy, Christopher J., Chun, Jaehun, & De Yoreo, James J. Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations. United States. https://doi.org/10.1038/s41467-020-14719-w
Liu, Lili, Nakouzi, Elias, Sushko, Maria L., Schenter, Gregory K., Mundy, Christopher J., Chun, Jaehun, and De Yoreo, James J. Tue .
"Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations". United States. https://doi.org/10.1038/s41467-020-14719-w. https://www.osti.gov/servlets/purl/1604768.
@article{osti_1604768,
title = {Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations},
author = {Liu, Lili and Nakouzi, Elias and Sushko, Maria L. and Schenter, Gregory K. and Mundy, Christopher J. and Chun, Jaehun and De Yoreo, James J.},
abstractNote = {The interplay between crystal and solvent structure, interparticle forces and ensemble particle response dynamics governs the process of crystallization by oriented attachment (OA), yet a quantitative understanding is lacking. Using as a model system ZnO, we combine in situ TEM observations of single particle and ensemble assembly dynamics with simulations of interparticle forces and responses to relate experimentally derived interparticle potentials to the underlying interactions. We show that OA is driven by forces and torques due to a combination of electrostatic ion-solvent correlations and dipolar interactions that act at separations well beyond 5 nm. Importantly, coalignment is achieved before particles reach separations at which strong attractions drive the final jump to contact. The observed barrier to attachment is negligible, while dissipative factors in the quasi-2D confinement of the TEM fluid cell lead to abnormal diffusivities with timescales for rotation much less than for translation, thus enabling OA to dominate.},
doi = {10.1038/s41467-020-14719-w},
journal = {Nature Communications},
number = 1,
volume = 11,
place = {United States},
year = {Tue Feb 25 00:00:00 EST 2020},
month = {Tue Feb 25 00:00:00 EST 2020}
}
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ZnO Nanorods with Tunable Aspect Ratios Deriving from Oriented-attachment for Enhanced Performance in Quantum-dot Sensitized Solar Cells
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In Situ Liquid Cell TEM Reveals Bridge-Induced Contact and Fusion of Au Nanocrystals in Aqueous Solution
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Effect of Ionic Strength on the Kinetics of Crystal Growth by Oriented Aggregation
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Silver Nanorice Structures: Oriented Attachment-Dominated Growth, High Environmental Sensitivity, and Real-Space Visualization of Multipolar Resonances
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Synthesis of Quantum-Sized Cubic ZnS Nanorods by the Oriented Attachment Mechanism
journal, April 2005
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Designing PbSe Nanowires and Nanorings through Oriented Attachment of Nanoparticles
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- Cho, Kyung-Sang; Talapin, Dmitri V.; Gaschler, Wolfgang
- Journal of the American Chemical Society, Vol. 127, Issue 19
Defects and Disorder: Probing the Surface Chemistry of Heterogenite (CoOOH) by Dissolution Using Hydroquinone and Iminodiacetic Acid
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Orientated Attachment Assisted Self-Assembly of Sb 2 O 3 Nanorods and Nanowires: End-to-End versus Side-by-Side
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The Role of Solvent Heterogeneity in Determining the Dispersion Interaction between Nanoassemblies
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Oriented Attachment Growth of Quantum-Sized CdS Nanorods by Direct Thermolysis of Single-Source Precursor
journal, March 2011
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DLVO Interaction between Rough Surfaces
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Bonding Pathways of Gold Nanocrystals in Solution
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- Aabdin, Zainul; Lu, Jingyu; Zhu, Xi
- Nano Letters, Vol. 14, Issue 11
Nanocrystal Diffusion in a Liquid Thin Film Observed by in Situ Transmission Electron Microscopy
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- Zheng, Haimei; Claridge, Shelley A.; Minor, Andrew M.
- Nano Letters, Vol. 9, Issue 6
Direction-specific interaction forces underlying zinc oxide crystal growth by oriented attachment
journal, October 2017
- Zhang, X.; Shen, Z.; Liu, J.
- Nature Communications, Vol. 8, Issue 1
In-situ liquid cell transmission electron microscopy investigation on oriented attachment of gold nanoparticles
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- Zhu, Chao; Liang, Suxia; Song, Erhong
- Nature Communications, Vol. 9, Issue 1
Accessing crystal–crystal interaction forces with oriented nanocrystal atomic force microscopy probes
journal, September 2018
- Zhang, Xin; He, Yang; Liu, Jia
- Nature Protocols, Vol. 13, Issue 9
Anomalous oriented attachment growth behavior on SnO2 nanocrystals
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- Stroppa, Daniel G.; Montoro, Luciano A.; Beltrán, Armando
- Chemical Communications, Vol. 47, Issue 11
Colloidal gelation of oppositely charged particles
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Aqueous citrate: a first-principles and force-field molecular dynamics study
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Nanocrystal growth via oriented attachment
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- Zhang, Hengzhong; Penn, R. Lee; Lin, Zhang
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Probing interaction forces in colloidal monolayers: Inversion of structural data
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- Quesada-Pérez, M.; Moncho-Jordá, A.; Martı́nez-López, F.
- The Journal of Chemical Physics, Vol. 115, Issue 23
Electrolytes between dielectric charged surfaces: Simulations and theory
journal, May 2015
- dos Santos, Alexandre P.; Levin, Yan
- The Journal of Chemical Physics, Vol. 142, Issue 19
Ionic size effects on the Poisson-Boltzmann theory
journal, July 2017
- Colla, Thiago; Nunes Lopes, Lucas; dos Santos, Alexandre P.
- The Journal of Chemical Physics, Vol. 147, Issue 1
Trends in mica–mica adhesion reflect the influence of molecular details on long-range dispersion forces underlying aggregation and coalignment
journal, July 2017
- Li, Dongsheng; Chun, Jaehun; Xiao, Dongdong
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 29
Van der Waals forces between an atom and a surface
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Enhanced Dispersion Interaction in Confined Geometry
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Repulsion between Oppositely Charged Surfaces in Multivalent Electrolytes
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- Physical Review Letters, Vol. 97, Issue 6
Real-Time Imaging of Pt3Fe Nanorod Growth in Solution
journal, May 2012
- Liao, H. -G.; Cui, L.; Whitelam, S.
- Science, Vol. 336, Issue 6084
Direction-Specific Interactions Control Crystal Growth by Oriented Attachment
journal, May 2012
- Li, D.; Nielsen, M. H.; Lee, J. R. I.
- Science, Vol. 336, Issue 6084
Imperfect Oriented Attachment: Dislocation Generation in Defect-Free Nanocrystals
journal, August 1998
- Penn, R. Lee; Banfield, Jillian F.
- Science, Vol. 281, Issue 5379, p. 969-971
Direction-specific van der Waals attraction between rutile TiO 2 nanocrystals
journal, April 2017
- Zhang, Xin; He, Yang; Sushko, Maria L.
- Science, Vol. 356, Issue 6336
Repulsion between Oppositely Charged Planar Macroions
journal, August 2013
- Jho, YongSeok; Brown, Frank L. H.; Kim, MahnWon
- PLoS ONE, Vol. 8, Issue 8
Efficient simulation method for nano-patterned charged surfaces in an electrolyte solution
text, January 2018
- Bakhshandeh, Amin; Dos Santos, Alexandre P.; Levin, Yan
- Freie Universität Berlin
Oriented Attachment of ZnO Nanocrystals
text, January 2013
- Hapiuk, Dimitri; Masenelli, Bruno; Masenelli-Varlot, Karine
- arXiv
The role of correlation and solvation in ion interactions with B-DNA
text, January 2015
- Sushko, Maria L.; Thomas, Dennis G.; Pabit, Suzette A.
- arXiv
Simulations of Coulomb systems confined by polarizable surfaces using periodic Green functions
text, January 2017
- Santos, Alexandre P. dos; Girotto, Matheus; Levin, Yan
- arXiv