Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries
Abstract
Society’s long-standing energy demands have fuelled for centuries the quest for power-dense, portable and economically viable energy carriers. Since the birth of the first rechargeable battery in 1860, emerging battery technologies have provided both answers to these demands as well as additional obstacles. One ubiquitous energy storage device, the metal or metalion battery, offers quintessential examples of both. The strongly reducing nature of Group 1 and 2 metal ions qualifies these elements as viable energy-dense anode materials: standard reduction potentials several volts below that of the standard hydrogen electrode (SHE) allow a thermodynamically favourable oxidation of these metals to readily release electrons that shuttle through an external circuit, generating the electric current that serves as the power supply during battery discharge. Integration of energy-dense materials into devices allows power sources to be compact and portable, by maximizing energy output per unit mass of material. Further, the reversibility of these oxidation events makes possible extensive battery cycling, thus providing a rechargeable power source. Indeed, current Li-ion batteries boast an energy density of 265 Wh kg-1, with the potential of a 20% improvement, and are operable for over 1000 charge–discharge cycles.
- Publication Date:
- Research Org.:
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1601987
- Grant/Contract Number:
- SC0018235
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences
- Additional Journal Information:
- Journal Volume: 377; Journal Issue: 2149; Journal ID: ISSN 1364-503X
- Publisher:
- The Royal Society Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; MOF; COF; metal-ion batteries; solid-state electrolyte
Citation Formats
Miner, Elise M., and Dincă, Mircea. Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries. United States: N. p., 2019.
Web. doi:10.1098/rsta.2018.0225.
Miner, Elise M., & Dincă, Mircea. Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries. United States. https://doi.org/10.1098/rsta.2018.0225
Miner, Elise M., and Dincă, Mircea. Mon .
"Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries". United States. https://doi.org/10.1098/rsta.2018.0225. https://www.osti.gov/servlets/purl/1601987.
@article{osti_1601987,
title = {Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries},
author = {Miner, Elise M. and Dincă, Mircea},
abstractNote = {Society’s long-standing energy demands have fuelled for centuries the quest for power-dense, portable and economically viable energy carriers. Since the birth of the first rechargeable battery in 1860, emerging battery technologies have provided both answers to these demands as well as additional obstacles. One ubiquitous energy storage device, the metal or metalion battery, offers quintessential examples of both. The strongly reducing nature of Group 1 and 2 metal ions qualifies these elements as viable energy-dense anode materials: standard reduction potentials several volts below that of the standard hydrogen electrode (SHE) allow a thermodynamically favourable oxidation of these metals to readily release electrons that shuttle through an external circuit, generating the electric current that serves as the power supply during battery discharge. Integration of energy-dense materials into devices allows power sources to be compact and portable, by maximizing energy output per unit mass of material. Further, the reversibility of these oxidation events makes possible extensive battery cycling, thus providing a rechargeable power source. Indeed, current Li-ion batteries boast an energy density of 265 Wh kg-1, with the potential of a 20% improvement, and are operable for over 1000 charge–discharge cycles.},
doi = {10.1098/rsta.2018.0225},
journal = {Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences},
number = 2149,
volume = 377,
place = {United States},
year = {Mon May 27 00:00:00 EDT 2019},
month = {Mon May 27 00:00:00 EDT 2019}
}
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Mechanically Shaped Two-Dimensional Covalent Organic Frameworks Reveal Crystallographic Alignment and Fast Li-Ion Conductivity
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A pre-synthetic strategy to construct single ion conductive covalent organic frameworks
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