Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr0.8Sn0.2O3

Yang, Junyi; Hao, Lin; Cui, Qi; Lin, Jiaqi; Horak, Lukas; Liu, Xuerong; Zhang, Lu; Yang, Huaixin; Karapetrova, Jenia; Kim, Jong-Woo; Ryan, Philip J.; Dean, Mark P. M.; Cheng, Jinguang; Liu, Jian

doi:10.1103/PhysRevMaterials.3.124411

Title: Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate $SrI r_{0.8} S n_{0.2} O_{3}$

Abstract

5d iridates have shown vast emergent phenomena due to a strong interplay among their lattice, charge, and spin degrees of freedom, because of which the potential in spintronic application of the thin-film form is highly leveraged. Here we have epitaxially stabilized perovskite SrIr_0.8Sn_0.2O₃ on [001] SrTiO₃ substrates through pulsed laser deposition and systematically characterized the structural, electronic, and magnetic properties. Physical property measurements unravel an insulating ground state with a weak ferromagnetism in the compressively strained epitaxial film. Here, the octahedral rotation pattern is identified by synchrotron x-ray diffraction, resolving a mix of a⁺b^–c^– and a^–b⁺c^– domains. X-ray magnetic resonant scattering directly demonstrates a G-type antiferromagnetic structure of the magnetic order and the spin canting nature of the weak ferromagnetism.

Authors:

^[1];

^[1]; Cui, Qi ^[2];

^[3]; Horak, Lukas ^[4]; Liu, Xuerong ^[5]; Zhang, Lu ^[6]; Yang, Huaixin ^[7]; Karapetrova, Jenia ^[8]; Kim, Jong-Woo ^[8]; Ryan, Philip J. ^[8];

^[3];

^[7]; Liu, Jian ^[1]

Univ. of Tennessee, Knoxville, TN (United States)
Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Charles Univ., Prague (Czech Republic)
ShanghaiTech Univ., Shanghai (China)
Chinese Academy of Sciences (CAS), Beijing (China)
Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China); Songshan Lake Materials Lab., Guangdong (China)
Argonne National Lab. (ANL), Argonne, IL (United States)

Publication Date:: Tue Dec 24 00:00:00 EST 2019

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: National Science Foundation (NSF); University of Tennessee; National Key Research and Development Program of China; European Regional Development Fund (ERDF); National Natural Science Foundation of China (NSFC); Chinese Academy of Sciences (CAS); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division

OSTI Identifier:: 1595261

Grant/Contract Number:: AC02-06CH11357; DMR-1848269; SC0012704; 2018YFA0305700; 11874400; QYZDB-SSW-SLH013; 112111KYSB20170059

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Materials

Additional Journal Information:: Journal Volume: 3; Journal Issue: 12; Journal ID: ISSN 2475-9953

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Yang, Junyi, Hao, Lin, Cui, Qi, Lin, Jiaqi, Horak, Lukas, Liu, Xuerong, Zhang, Lu, Yang, Huaixin, Karapetrova, Jenia, Kim, Jong-Woo, Ryan, Philip J., Dean, Mark P. M., Cheng, Jinguang, and Liu, Jian. Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr0.8Sn0.2O3.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevMaterials.3.124411.

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                    Yang, Junyi, Hao, Lin, Cui, Qi, Lin, Jiaqi, Horak, Lukas, Liu, Xuerong, Zhang, Lu, Yang, Huaixin, Karapetrova, Jenia, Kim, Jong-Woo, Ryan, Philip J., Dean, Mark P. M., Cheng, Jinguang, & Liu, Jian. Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr0.8Sn0.2O3.  United States.  https://doi.org/10.1103/PhysRevMaterials.3.124411

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                    Yang, Junyi, Hao, Lin, Cui, Qi, Lin, Jiaqi, Horak, Lukas, Liu, Xuerong, Zhang, Lu, Yang, Huaixin, Karapetrova, Jenia, Kim, Jong-Woo, Ryan, Philip J., Dean, Mark P. M., Cheng, Jinguang, and Liu, Jian. Tue .  
"Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr0.8Sn0.2O3".  United States.  https://doi.org/10.1103/PhysRevMaterials.3.124411.  https://www.osti.gov/servlets/purl/1595261.

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@article{osti_1595261,

  title        = {Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr0.8Sn0.2O3},

  author       = {Yang, Junyi and Hao, Lin and Cui, Qi and Lin, Jiaqi and Horak, Lukas and Liu, Xuerong and Zhang, Lu and Yang, Huaixin and Karapetrova, Jenia and Kim, Jong-Woo and Ryan, Philip J. and Dean, Mark P. M. and Cheng, Jinguang and Liu, Jian},

  abstractNote = {5d iridates have shown vast emergent phenomena due to a strong interplay among their lattice, charge, and spin degrees of freedom, because of which the potential in spintronic application of the thin-film form is highly leveraged. Here we have epitaxially stabilized perovskite SrIr0.8Sn0.2O3 on [001] SrTiO3 substrates through pulsed laser deposition and systematically characterized the structural, electronic, and magnetic properties. Physical property measurements unravel an insulating ground state with a weak ferromagnetism in the compressively strained epitaxial film. Here, the octahedral rotation pattern is identified by synchrotron x-ray diffraction, resolving a mix of a+b–c– and a–b+c– domains. X-ray magnetic resonant scattering directly demonstrates a G-type antiferromagnetic structure of the magnetic order and the spin canting nature of the weak ferromagnetism.},

  doi          = {10.1103/PhysRevMaterials.3.124411},

  journal      = {Physical Review Materials},

  number       = 12,

  volume       = 3,

  place        = {United States},

  year         = {Tue Dec 24 00:00:00 EST 2019},

  month        = {Tue Dec 24 00:00:00 EST 2019}

}

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Title: Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrI r 0.8 S n 0.2 O 3

Abstract

Citation Formats

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Interplay of Spin-Orbit Interactions, Dimensionality, and Octahedral Rotations in Semimetallic SrIrO 3 journal, January 2015

Correlated Dirac semimetallic state with unusual positive magnetoresistance in strain-free perovskite SrIrO 3 journal, March 2017

Non-Fermi-liquid behavior in nearly ferromagnetic SrIrO 3 single crystals journal, September 2007

Ultrafast energy- and momentum-resolved dynamics of magnetic correlations in the photo-doped Mott insulator Sr2IrO4 journal, May 2016

Spin-Orbit Physics Giving Rise to Novel Phases in Correlated Systems: Iridates and Related Materials journal, March 2016

Dimensionality Driven Spin-Flop Transition in Layered Iridates journal, July 2012

Square Lattice Iridates journal, March 2019

Origin of the Anomalous Magnetic Behavior in Single Crystal Fe 3 O 4 Films journal, December 1997

Interplay between spin-orbit coupling and Hubbard interaction in SrIrO 3 and related Pbnm perovskite oxides journal, August 2012

High-pressure synthesis and physical properties of perovskite and post-perovskite Ca 1 − x Sr x Ir O 3 journal, February 2011

Novel J eff = 1 / 2 Mott State Induced by Relativistic Spin-Orbit Coupling in Sr 2 IrO 4 journal, August 2008

Magnetic and crystal structures of Sr 2 IrO 4 : A neutron diffraction study journal, April 2013

Magnetism in iridate heterostructures leveraged by structural distortions journal, March 2019

Spintronics: A Spin-Based Electronics Vision for the Future journal, November 2001

Simple ways of determining perovskite structures journal, November 1975

Giant magnetic response of a two-dimensional antiferromagnet journal, June 2018

Charge Dynamics and Metal–Insulator Transition in Perovskite SrIr 1− x Sn x O 3 journal, December 2018

Topological nodal line semimetals with and without spin-orbital coupling journal, August 2015

Anisotropic magnetoresistance in an antiferromagnetic semiconductor journal, September 2014

First-Order Melting of a Weak Spin-Orbit Mott Insulator into a Correlated Metal journal, June 2015

The classification of tilted octahedra in perovskites journal, November 1972

Metal insulator transitions in perovskite SrIrO 3 thin films journal, December 2014

Compressive strain-induced metal–insulator transition in orthorhombic SrIrO 3 thin films journal, October 2014

Dimensionality-Controlled Insulator-Metal Transition and Correlated Metallic State in 5 d Transition Metal Oxides Sr n + 1 Ir n O 3 n + 1 ( n = 1 , 2, and ∞ ) journal, November 2008

The challenge of spin–orbit-tuned ground states in iridates: a key issues review journal, February 2018

Twisted Hubbard Model for Sr 2 IrO 4 : Magnetism and Possible High Temperature Superconductivity journal, March 2011

Locking of iridium magnetic moments to the correlated rotation of oxygen octahedra in Sr 2 IrO 4 revealed by x-ray resonant scattering journal, September 2013

Mott Insulators in the Strong Spin-Orbit Coupling Limit: From Heisenberg to a Quantum Compass and Kitaev Models journal, January 2009

Synthesis, structures and properties of transition metal doped SrIrO3 journal, January 2013

Antiferromagnet-Based Spintronic Functionality by Controlling Isospin Domains in a Layered Perovskite Iridate journal, October 2018

Semimetal and Topological Insulator in Perovskite Iridates text, January 2011

Correlated quantum phenomena in the strong spin-orbit regime text, January 2013

Metal insulator transitions in perovskite SrIrO3 thin films text, January 2013

Spin-Orbit Physics Giving Rise to Novel Phases in Correlated Systems: Iridates and Related Materials text, January 2015

Slater Insulator in Iridate Perovskites with Strong Spin-Orbit Coupling text, January 2017

Antiferromagnet-based spintronic functionality by controlling isospin domains in a layered perovskite iridate text, January 2018

Title: Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate $SrI r_{0.8} S n_{0.2} O_{3}$

Sr ₂ IrO ₄ : Gateway to cuprate superconductivity?
journal, June 2015

High-pressure synthesis of orthorhombic SrIrO3 perovskite and its positive magnetoresistance
journal, May 2008

Two-Dimensional $J_{eff} = 1 / 2$ Antiferromagnetic Insulator Unraveled from Interlayer Exchange Coupling in Artificial Perovskite Iridate Superlattices
journal, July 2017

Towards a Strong Spin–Orbit Coupling Magnetoelectric Transistor
journal, June 2018

Lattice-driven magnetoresistivity and metal-insulator transition in single-layered iridates
journal, September 2011

Correlated Quantum Phenomena in the Strong Spin-Orbit Regime
journal, March 2014

Mott physics and band topology in materials with strong spin–orbit interaction
journal, March 2010

Superparamagnetic behavior of structural domains in epitaxial ultrathin magnetite films
journal, April 1998

Novel spin-orbit coupling driven emergent states in iridate-based heterostructures
journal, May 2019

Strong ferromagnetism induced by canted antiferromagnetic order in double perovskite iridates $({La}_{1 - x} {Sr}_{x})_{2} {ZnIrO}_{6}$
journal, April 2015

Anisotropic Magnetoresistance in Antiferromagnetic ${Sr}_{2} {IrO}_{4}$
journal, November 2014

Direct observation of the Dirac nodes lifting in semimetallic perovskite SrIrO3 thin films
journal, July 2016

Magnetoelectric Devices for Spintronics
journal, July 2014

Structure and properties of the high and low pressure forms of SrIrO3
journal, May 1971

Ordered vs. disordered perovskites; structural studies of Fe-doped SrIrO3 and SrRuO3
journal, October 2013

Giant anisotropic magnetoresistance and nonvolatile memory in canted antiferromagnet Sr2IrO4
journal, May 2019

Phase-Sensitive Observation of a Spin-Orbital Mott State in Sr2IrO4
journal, March 2009

Slater Insulator in Iridate Perovskites with Strong Spin-Orbit Coupling
journal, October 2016

Semimetal and Topological Insulator in Perovskite Iridates
journal, March 2012

Structure of epitaxial SrIrO ₃ perovskite studied by interference between X-ray waves diffracted by the substrate and the thin film
journal, February 2017

Strain-induced nonsymmorphic symmetry breaking and removal of Dirac semimetallic nodal line in an orthoperovskite iridate
journal, February 2016

Interplay of Spin-Orbit Interactions, Dimensionality, and Octahedral Rotations in Semimetallic ${SrIrO}_{3}$
journal, January 2015

Correlated Dirac semimetallic state with unusual positive magnetoresistance in strain-free perovskite ${SrIrO}_{3}$
journal, March 2017

Non-Fermi-liquid behavior in nearly ferromagnetic ${SrIrO}_{3}$ single crystals
journal, September 2007

Ultrafast energy- and momentum-resolved dynamics of magnetic correlations in the photo-doped Mott insulator Sr2IrO4
journal, May 2016

Spin-Orbit Physics Giving Rise to Novel Phases in Correlated Systems: Iridates and Related Materials
journal, March 2016

Dimensionality Driven Spin-Flop Transition in Layered Iridates
journal, July 2012

Square Lattice Iridates
journal, March 2019

Origin of the Anomalous Magnetic Behavior in Single Crystal ${Fe}_{3} O_{4}$ Films
journal, December 1997

Interplay between spin-orbit coupling and Hubbard interaction in SrIrO $_{3}$ and related $Pbnm$ perovskite oxides
journal, August 2012

High-pressure synthesis and physical properties of perovskite and post-perovskite Ca $_{1 - x}$ Sr $_{x}$ Ir $O_{3}$
journal, February 2011

Novel $J_{eff} = 1 / 2$ Mott State Induced by Relativistic Spin-Orbit Coupling in ${Sr}_{2} {IrO}_{4}$
journal, August 2008

Magnetic and crystal structures of ${Sr}_{2} {IrO}_{4}$ : A neutron diffraction study
journal, April 2013

Magnetism in iridate heterostructures leveraged by structural distortions
journal, March 2019

Spintronics: A Spin-Based Electronics Vision for the Future
journal, November 2001

Simple ways of determining perovskite structures
journal, November 1975

Giant magnetic response of a two-dimensional antiferromagnet
journal, June 2018

Charge Dynamics and Metal–Insulator Transition in Perovskite SrIr ₁₋ _x Sn _x O ₃
journal, December 2018

Topological nodal line semimetals with and without spin-orbital coupling
journal, August 2015

Anisotropic magnetoresistance in an antiferromagnetic semiconductor
journal, September 2014

First-Order Melting of a Weak Spin-Orbit Mott Insulator into a Correlated Metal
journal, June 2015

The classification of tilted octahedra in perovskites
journal, November 1972

Metal insulator transitions in perovskite SrIrO ₃ thin films
journal, December 2014

Compressive strain-induced metal–insulator transition in orthorhombic SrIrO ₃ thin films
journal, October 2014

Dimensionality-Controlled Insulator-Metal Transition and Correlated Metallic State in $5 d$ Transition Metal Oxides ${Sr}_{n + 1} {Ir}_{n} O_{3 n + 1}$ ( $n = 1$ , 2, and $\infty$ )
journal, November 2008

The challenge of spin–orbit-tuned ground states in iridates: a key issues review
journal, February 2018

Twisted Hubbard Model for ${Sr}_{2} {IrO}_{4}$ : Magnetism and Possible High Temperature Superconductivity
journal, March 2011

Locking of iridium magnetic moments to the correlated rotation of oxygen octahedra in Sr ₂ IrO ₄ revealed by x-ray resonant scattering
journal, September 2013

Mott Insulators in the Strong Spin-Orbit Coupling Limit: From Heisenberg to a Quantum Compass and Kitaev Models
journal, January 2009

Synthesis, structures and properties of transition metal doped SrIrO3
journal, January 2013

Antiferromagnet-Based Spintronic Functionality by Controlling Isospin Domains in a Layered Perovskite Iridate
journal, October 2018

Semimetal and Topological Insulator in Perovskite Iridates
text, January 2011

Correlated quantum phenomena in the strong spin-orbit regime
text, January 2013

Metal insulator transitions in perovskite SrIrO3 thin films
text, January 2013

Spin-Orbit Physics Giving Rise to Novel Phases in Correlated Systems: Iridates and Related Materials
text, January 2015

Slater Insulator in Iridate Perovskites with Strong Spin-Orbit Coupling
text, January 2017

Antiferromagnet-based spintronic functionality by controlling isospin domains in a layered perovskite iridate
text, January 2018