Long-Term Measurements Show Little Evidence for Large Increases in Total U.S. Methane Emissions Over the Past Decade
Abstract
Recent studies show conflicting estimates of trends in methane (CH4) emissions from oil and natural gas (ONG) operations in the United States. We analyze atmospheric CH4 measurements from 20 North American sites in the National Oceanic and Atmospheric Administration Global Greenhouse Gas Reference Network and determined trends for 2006–2015. Using CH4 vertical gradients as an indicator of regional surface emissions, we find no significant increase in emissions at most sites and modest increases at three sites heavily influenced by ONG activities. Our estimated increases in North American ONG CH4 emissions (on average approximately 3.4 ± 1.4 %/year for 2006–2015, ±σ) are much smaller than estimates from some previous studies and below our detection threshold for total emissions increases at the east coast sites that are sensitive to U.S. outflows. We also find an increasing trend in ethane/methane emission ratios, which has resulted in major overestimation of oil and gas emissions trends in some previous studies.
- Authors:
-
- Univ. of Colorado, Boulder, CO (United States); National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States)
- National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Biological and Environmental Research (BER)
- OSTI Identifier:
- 1572010
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Geophysical Research Letters
- Additional Journal Information:
- Journal Volume: 46; Journal Issue: 9; Journal ID: ISSN 0094-8276
- Publisher:
- American Geophysical Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; atmospheric composition; methane; oil and natural gas emissions
Citation Formats
Lan, Xin, Tans, Pieter, Sweeney, Colm, Andrews, Arlyn, Dlugokencky, Edward, Schwietzke, Stefan, Kofler, Jonathan, McKain, Kathryn, Thoning, Kirk, Crotwell, Molly, Montzka, Stephen, Miller, Benjamin R., and Biraud, Sébastien C. Long-Term Measurements Show Little Evidence for Large Increases in Total U.S. Methane Emissions Over the Past Decade. United States: N. p., 2019.
Web. doi:10.1029/2018gl081731.
Lan, Xin, Tans, Pieter, Sweeney, Colm, Andrews, Arlyn, Dlugokencky, Edward, Schwietzke, Stefan, Kofler, Jonathan, McKain, Kathryn, Thoning, Kirk, Crotwell, Molly, Montzka, Stephen, Miller, Benjamin R., & Biraud, Sébastien C. Long-Term Measurements Show Little Evidence for Large Increases in Total U.S. Methane Emissions Over the Past Decade. United States. https://doi.org/10.1029/2018gl081731
Lan, Xin, Tans, Pieter, Sweeney, Colm, Andrews, Arlyn, Dlugokencky, Edward, Schwietzke, Stefan, Kofler, Jonathan, McKain, Kathryn, Thoning, Kirk, Crotwell, Molly, Montzka, Stephen, Miller, Benjamin R., and Biraud, Sébastien C. Thu .
"Long-Term Measurements Show Little Evidence for Large Increases in Total U.S. Methane Emissions Over the Past Decade". United States. https://doi.org/10.1029/2018gl081731. https://www.osti.gov/servlets/purl/1572010.
@article{osti_1572010,
title = {Long-Term Measurements Show Little Evidence for Large Increases in Total U.S. Methane Emissions Over the Past Decade},
author = {Lan, Xin and Tans, Pieter and Sweeney, Colm and Andrews, Arlyn and Dlugokencky, Edward and Schwietzke, Stefan and Kofler, Jonathan and McKain, Kathryn and Thoning, Kirk and Crotwell, Molly and Montzka, Stephen and Miller, Benjamin R. and Biraud, Sébastien C.},
abstractNote = {Recent studies show conflicting estimates of trends in methane (CH4) emissions from oil and natural gas (ONG) operations in the United States. We analyze atmospheric CH4 measurements from 20 North American sites in the National Oceanic and Atmospheric Administration Global Greenhouse Gas Reference Network and determined trends for 2006–2015. Using CH4 vertical gradients as an indicator of regional surface emissions, we find no significant increase in emissions at most sites and modest increases at three sites heavily influenced by ONG activities. Our estimated increases in North American ONG CH4 emissions (on average approximately 3.4 ± 1.4 %/year for 2006–2015, ±σ) are much smaller than estimates from some previous studies and below our detection threshold for total emissions increases at the east coast sites that are sensitive to U.S. outflows. We also find an increasing trend in ethane/methane emission ratios, which has resulted in major overestimation of oil and gas emissions trends in some previous studies.},
doi = {10.1029/2018gl081731},
journal = {Geophysical Research Letters},
number = 9,
volume = 46,
place = {United States},
year = {Thu Apr 25 00:00:00 EDT 2019},
month = {Thu Apr 25 00:00:00 EDT 2019}
}
Web of Science
Works referenced in this record:
Anthropogenic emissions of methane in the United States
journal, November 2013
- Miller, S. M.; Wofsy, S. C.; Michalak, A. M.
- Proceedings of the National Academy of Sciences, Vol. 110, Issue 50
Evaluation of wetland methane emissions across North America using atmospheric data and inverse modeling
journal, January 2016
- Miller, Scot M.; Commane, Roisin; Melton, Joe R.
- Biogeosciences, Vol. 13, Issue 4
Development and validation of a global database of lakes, reservoirs and wetlands
journal, August 2004
- Lehner, Bernhard; Döll, Petra
- Journal of Hydrology, Vol. 296, Issue 1-4
Seasonal climatology of CO 2 across North America from aircraft measurements in the NOAA/ESRL Global Greenhouse Gas Reference Network : VERTICAL CLIMATOLOGY OF CO
journal, May 2015
- Sweeney, Colm; Karion, Anna; Wolter, Sonja
- Journal of Geophysical Research: Atmospheres, Vol. 120, Issue 10
Revised methane emissions factors and spatially distributed annual carbon fluxes for global livestock
journal, September 2017
- Wolf, Julie; Asrar, Ghassem R.; West, Tristram O.
- Carbon Balance and Management, Vol. 12, Issue 1
Computer-Intensive Methods in Statistics
journal, May 1983
- Diaconis, Persi; Efron, Bradley
- Scientific American, Vol. 248, Issue 5
Contribution of oil and natural gas production to renewed increase in atmospheric methane (2007–2014): top–down estimate from ethane and methane column observations
journal, January 2016
- Hausmann, Petra; Sussmann, Ralf; Smale, Dan
- Atmospheric Chemistry and Physics, Vol. 16, Issue 5
Evaluation of solid adsorbent materials for cryogen-free trapping—gas chromatographic analysis of atmospheric C2–C6 non-methane hydrocarbons
journal, November 2006
- Pollmann, Jan; Helmig, Detlev; Hueber, Jacques
- Journal of Chromatography A, Vol. 1134, Issue 1-2, p. 1-15
Evaluating ethane and methane emissions associated with the development of oil and natural gas extraction in North America
journal, April 2016
- Franco, B.; Mahieu, E.; Emmons, L. K.
- Environmental Research Letters, Vol. 11, Issue 4
Upward revision of global fossil fuel methane emissions based on isotope database
journal, October 2016
- Schwietzke, Stefan; Sherwood, Owen A.; Bruhwiler, Lori M. P.
- Nature, Vol. 538, Issue 7623
Coupled weather research and forecasting–stochastic time-inverted lagrangian transport (WRF–STILT) model
journal, May 2010
- Nehrkorn, Thomas; Eluszkiewicz, Janusz; Wofsy, Steven C.
- Meteorology and Atmospheric Physics, Vol. 107, Issue 1-2
Observational constraints on recent increases in the atmospheric CH 4 burden
journal, January 2009
- Dlugokencky, E. J.; Bruhwiler, L.; White, J. W. C.
- Geophysical Research Letters, Vol. 36, Issue 18
The global methane budget 2000–2012
journal, January 2016
- Saunois, Marielle; Bousquet, Philippe; Poulter, Ben
- Earth System Science Data, Vol. 8, Issue 2
Linking emissions of fossil fuel CO 2 and other anthropogenic trace gases using atmospheric 14 CO 2 : THE
journal, April 2012
- Miller, John B.; Lehman, Scott J.; Montzka, Stephen A.
- Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D8
Atmospheric methane levels off: Temporary pause or a new steady-state?
journal, January 2003
- Dlugokencky, E. J.
- Geophysical Research Letters, Vol. 30, Issue 19
Airborne Ethane Observations in the Barnett Shale: Quantification of Ethane Flux and Attribution of Methane Emissions
journal, June 2015
- Smith, Mackenzie L.; Kort, Eric A.; Karion, Anna
- Environmental Science & Technology, Vol. 49, Issue 13
A 21st-century shift from fossil-fuel to biogenic methane emissions indicated by 13CH4
journal, March 2016
- Schaefer, H.; Fletcher, S. E. M.; Veidt, C.
- Science, Vol. 352, Issue 6281
Contribution of anthropogenic and natural sources to atmospheric methane variability
journal, September 2006
- Bousquet, P.; Ciais, P.; Miller, J. B.
- Nature, Vol. 443, Issue 7110
U.S. CH 4 emissions from oil and gas production: Have recent large increases been detected? : U.S. Emissions From Oil and Gas Production
journal, April 2017
- Bruhwiler, L. M.; Basu, S.; Bergamaschi, P.
- Journal of Geophysical Research: Atmospheres, Vol. 122, Issue 7
Methane Leaks from North American Natural Gas Systems
journal, February 2014
- Brandt, A. R.; Heath, G. A.; Kort, E. A.
- Science, Vol. 343, Issue 6172
Quantifying atmospheric methane emissions from oil and natural gas production in the Bakken shale region of North Dakota: CH
journal, May 2016
- Peischl, J.; Karion, A.; Sweeney, C.
- Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 10
The tropospheric distribution and budget of ethane
journal, January 1995
- Rudolph, J.
- Journal of Geophysical Research, Vol. 100, Issue D6
Apparent seasonal cycle in isotopic discrimination of carbon in the atmosphere and biosphere due to vapor pressure deficit: SEASONAL ISOTOPIC DISCRIMINATION OF CO2
journal, September 2010
- Ballantyne, A. P.; Miller, J. B.; Tans, P. P.
- Global Biogeochemical Cycles, Vol. 24, Issue 3
Atmospheric carbon dioxide at Mauna Loa Observatory: 2. Analysis of the NOAA GMCC data, 1974-1985
journal, June 1989
- Thoning, Kirk W.; Tans, Pieter P.; Komhyr, Walter D.
- Journal of Geophysical Research: Atmospheres, Vol. 94, Issue D6
A near-field tool for simulating the upstream influence of atmospheric observations: The Stochastic Time-Inverted Lagrangian Transport (STILT) model
journal, January 2003
- Lin, J. C.
- Journal of Geophysical Research, Vol. 108, Issue D16
Seasonal variations of nonmethane hydrocarbons in rural New England: Constraints on OH concentrations in northern midlatitudes
journal, January 1995
- Goldstein, A. H.; Wofsy, S. C.; Spivakovsky, C. M.
- Journal of Geophysical Research, Vol. 100, Issue D10
CO 2 , CO, and CH 4 measurements from tall towers in the NOAA Earth System Research Laboratory's Global Greenhouse Gas Reference Network: instrumentation, uncertainty analysis, and recommendations for future high-accuracy greenhouse gas monitoring efforts
journal, January 2014
- Andrews, A. E.; Kofler, J. D.; Trudeau, M. E.
- Atmospheric Measurement Techniques, Vol. 7, Issue 2
Highly Elevated Atmospheric Levels of Volatile Organic Compounds in the Uintah Basin, Utah
journal, April 2014
- Helmig, D.; Thompson, C. R.; Evans, J.
- Environmental Science & Technology, Vol. 48, Issue 9
Global tropospheric distribution and calibration scale of HCFC-22
journal, April 1993
- Montzka, S. A.; Myers, R. C.; Butler, J. H.
- Geophysical Research Letters, Vol. 20, Issue 8
Sampling, storage, and analysis of C2–C7 non-methane hydrocarbons from the US National Oceanic and Atmospheric Administration Cooperative Air Sampling Network glass flasks
journal, April 2008
- Pollmann, Jan; Helmig, Detlev; Hueber, Jacques
- Journal of Chromatography A, Vol. 1188, Issue 2
Rising atmospheric methane: 2007-2014 growth and isotopic shift: RISING METHANE 2007-2014
journal, September 2016
- Nisbet, E. G.; Dlugokencky, E. J.; Manning, M. R.
- Global Biogeochemical Cycles, Vol. 30, Issue 9
Regional-scale measurements of CH4 exchange from a tall tower over a mixed temperate/boreal lowland and wetland forest
journal, September 2003
- Werner, Cindy; Davis, Kenneth; Bakwin, Peter
- Global Change Biology, Vol. 9, Issue 9
The NCEP/NCAR 40-Year Reanalysis Project
journal, March 1996
- Kalnay, E.; Kanamitsu, M.; Kistler, R.
- Bulletin of the American Meteorological Society, Vol. 77, Issue 3
Conversion of NOAA atmospheric dry air CH 4 mole fractions to a gravimetrically prepared standard scale
journal, January 2005
- Dlugokencky, E. J.
- Journal of Geophysical Research, Vol. 110, Issue D18
Fugitive emissions from the Bakken shale illustrate role of shale production in global ethane shift: Ethane Emissions From the Bakken Shale
journal, May 2016
- Kort, E. A.; Smith, M. L.; Murray, L. T.
- Geophysical Research Letters, Vol. 43, Issue 9
A multi-year record of airborne CO 2 observations in the US Southern Great Plains
journal, January 2013
- Biraud, S. C.; Torn, M. S.; Smith, J. R.
- Atmospheric Measurement Techniques, Vol. 6, Issue 3
Discrepancies and Uncertainties in Bottom-up Gridded Inventories of Livestock Methane Emissions for the Contiguous United States
journal, November 2017
- Hristov, Alexander N.; Harper, Michael; Meinen, Robert
- Environmental Science & Technology, Vol. 51, Issue 23
Gridded National Inventory of U.S. Methane Emissions
journal, November 2016
- Maasakkers, Joannes D.; Jacob, Daniel J.; Sulprizio, Melissa P.
- Environmental Science & Technology, Vol. 50, Issue 23
On the global distribution, seasonality, and budget of atmospheric carbonyl sulfide (COS) and some similarities to CO 2
journal, January 2007
- Montzka, S. A.; Calvert, P.; Hall, B. D.
- Journal of Geophysical Research, Vol. 112, Issue D9
Rising atmospheric methane: 2007-2014 growth and isotopic shift
text, January 2016
- Nisbet, Eg; Dlugokencky, Ej; Manning, Mr
- Apollo - University of Cambridge Repository
Contribution of oil and natural gas production to renewed increase of atmospheric methane (2007-2014): top-down estimate from ethane and methane column observations
text, January 2015
- Hausmann, P.; Sussmann, R.; Smale, D.
- Karlsruhe
The global methane budget 2000--2012
text, January 2016
- Saunois, Marielle; Bousquet, Philippe; Poulter, Ben
- Copernicus Publications
Works referencing / citing this record:
On the Causes and Consequences of Recent Trends in Atmospheric Methane
journal, August 2019
- Schaefer, Hinrich
- Current Climate Change Reports, Vol. 5, Issue 4
Daily Satellite Observations of Methane from Oil and Gas Production Regions in the United States
journal, January 2020
- de Gouw, Joost A.; Veefkind, J. Pepijn; Roosenbrand, Esther
- Scientific Reports, Vol. 10, Issue 1
Evaluating the carbon inventory, carbon fluxes and carbon cycles for a long-term sustainable world
journal, January 2019
- Tomkins, P.; Müller, T. E.
- Green Chemistry, Vol. 21, Issue 15
Rising methane: A new climate challenge
journal, June 2019
- Fletcher, Sara E. Mikaloff; Schaefer, Hinrich
- Science, Vol. 364, Issue 6444