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Title: High sensitivity hexagonal boron nitride lateral neutron detectors

Abstract

Hexagonal boron nitride (h-BN) thermal neutron detectors have demonstrated the highest detection efficiency among all solid-state detectors (at 58% for a detection area of 1 mm2 and 53% for a detection area of 9 mm2). However, scaling up the detector size of vertical h-BN detectors is challenging due to increased dark current, capacitance, and surface recombination with the increasing detection area. Here, we report the demonstration of a 29 mm2 thermal neutron detector fabricated from a freestanding 10B enriched h-BN epilayer of 90 μm in thickness with a detection efficiency of 50% by employing a lateral device geometry. The lateral detector geometry takes advantage of the unique layered structure of h-BN which naturally provides higher in-plane carrier mobilities than those in the vertical direction. Moreover, due to the reduced area of metals in contact with the h-BN material, the detrimental effects associated with the surface recombination at the metal contacts and device capacitance were reduced, which resulted in improved charge collection efficiency and signal to noise ratios. Furthermore, this work laid the ground work for scaling up to large size neutron detectors based on h-BN.

Authors:
 [1];  [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
  1. Texas Tech Univ., Lubbock, TX (United States). Dept. of Electrical and Computer Engineering
Publication Date:
Research Org.:
Texas Tech Univ., Lubbock, TX (United States)
Sponsoring Org.:
USDOE Advanced Research Projects Agency - Energy (ARPA-E)
OSTI Identifier:
1571783
Alternate Identifier(s):
OSTI ID: 1524460
Grant/Contract Number:  
AR0000964; NA0002927
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 114; Journal Issue: 22; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Maity, A., Grenadier, S. J., Li, J., Lin, J. Y., and Jiang, H. X. High sensitivity hexagonal boron nitride lateral neutron detectors. United States: N. p., 2019. Web. doi:10.1063/1.5098331.
Maity, A., Grenadier, S. J., Li, J., Lin, J. Y., & Jiang, H. X. High sensitivity hexagonal boron nitride lateral neutron detectors. United States. https://doi.org/10.1063/1.5098331
Maity, A., Grenadier, S. J., Li, J., Lin, J. Y., and Jiang, H. X. Mon . "High sensitivity hexagonal boron nitride lateral neutron detectors". United States. https://doi.org/10.1063/1.5098331. https://www.osti.gov/servlets/purl/1571783.
@article{osti_1571783,
title = {High sensitivity hexagonal boron nitride lateral neutron detectors},
author = {Maity, A. and Grenadier, S. J. and Li, J. and Lin, J. Y. and Jiang, H. X.},
abstractNote = {Hexagonal boron nitride (h-BN) thermal neutron detectors have demonstrated the highest detection efficiency among all solid-state detectors (at 58% for a detection area of 1 mm2 and 53% for a detection area of 9 mm2). However, scaling up the detector size of vertical h-BN detectors is challenging due to increased dark current, capacitance, and surface recombination with the increasing detection area. Here, we report the demonstration of a 29 mm2 thermal neutron detector fabricated from a freestanding 10B enriched h-BN epilayer of 90 μm in thickness with a detection efficiency of 50% by employing a lateral device geometry. The lateral detector geometry takes advantage of the unique layered structure of h-BN which naturally provides higher in-plane carrier mobilities than those in the vertical direction. Moreover, due to the reduced area of metals in contact with the h-BN material, the detrimental effects associated with the surface recombination at the metal contacts and device capacitance were reduced, which resulted in improved charge collection efficiency and signal to noise ratios. Furthermore, this work laid the ground work for scaling up to large size neutron detectors based on h-BN.},
doi = {10.1063/1.5098331},
journal = {Applied Physics Letters},
number = 22,
volume = 114,
place = {United States},
year = {Mon Jun 03 00:00:00 EDT 2019},
month = {Mon Jun 03 00:00:00 EDT 2019}
}

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Works referenced in this record:

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Works referencing / citing this record:

Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers
journal, August 2019

  • Grenadier, S.; Maity, A.; Li, J.
  • Applied Physics Letters, Vol. 115, Issue 7
  • DOI: 10.1063/1.5097984

Anisotropic index of refraction and structural properties of hexagonal boron nitride epilayers probed by spectroscopic ellipsometry
journal, February 2020

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  • Journal of Applied Physics, Vol. 127, Issue 5
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