Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays

Knudson, Michael P.; Li, Ran; Wang, Danqing; Wang, Weijia; Schaller, Richard D.; Odom, Teri W.

doi:10.1021/acsnano.9b01142

Title: Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays

Abstract

In this paper, we report how geometric effects in low-symmetry plasmonic nanoparticle arrays can produce polarization-dependent lasing responses. We developed a scalable fabrication procedure to pattern rhombohedral arrays of aluminum anisotropic nanoparticles that support lattice plasmon modes from both first-order and second-order diffraction coupling. We found that nanoparticle shape can be used to engineer the spatial overlap between electromagnetic hot spots of different lattice modes and dye gain to support plasmonic lasing. The lasing behavior revealed that plasmon–exciton energy transfer depends on polarization, with stronger coupling and faster dynamics when the transition dipole moments of the excited gain are aligned with the electric field of the plasmon modes.

Authors:

Knudson, Michael P. ^[1]; Li, Ran ^[1]; Wang, Danqing ^[1]; Wang, Weijia ^[1];

^[2];

^[1]

Northwestern Univ., Evanston, IL (United States)
Northwestern Univ., Evanston, IL (United States); Argonne National Lab. (ANL), Lemont, IL (United States)

Publication Date:: Tue Apr 02 00:00:00 EDT 2019

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; U.S. Department of Defense (DOD) - Vannevar Bush Faculty Fellowship; National Science Foundation (NSF) - Directorate for Mathematical and Physical Sciences Division of Materials Research (MPS-DMR)

OSTI Identifier:: 1571632

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: ACS Nano

Additional Journal Information:: Journal Volume: 13; Journal Issue: 7; Journal ID: ISSN 1936-0851

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; symmetry; aluminum plasmonics; anisotropic nanoparticles; lasing; lattice plasmons; polarization

Citation Formats


                    Knudson, Michael P., Li, Ran, Wang, Danqing, Wang, Weijia, Schaller, Richard D., and Odom, Teri W. Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays.  United States: N. p., 2019. 
Web.  doi:10.1021/acsnano.9b01142.

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                    Knudson, Michael P., Li, Ran, Wang, Danqing, Wang, Weijia, Schaller, Richard D., & Odom, Teri W. Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays.  United States.  https://doi.org/10.1021/acsnano.9b01142

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                    Knudson, Michael P., Li, Ran, Wang, Danqing, Wang, Weijia, Schaller, Richard D., and Odom, Teri W. Tue .  
"Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays".  United States.  https://doi.org/10.1021/acsnano.9b01142.  https://www.osti.gov/servlets/purl/1571632.

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@article{osti_1571632,

  title        = {Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays},

  author       = {Knudson, Michael P. and Li, Ran and Wang, Danqing and Wang, Weijia and Schaller, Richard D. and Odom, Teri W.},

  abstractNote = {In this paper, we report how geometric effects in low-symmetry plasmonic nanoparticle arrays can produce polarization-dependent lasing responses. We developed a scalable fabrication procedure to pattern rhombohedral arrays of aluminum anisotropic nanoparticles that support lattice plasmon modes from both first-order and second-order diffraction coupling. We found that nanoparticle shape can be used to engineer the spatial overlap between electromagnetic hot spots of different lattice modes and dye gain to support plasmonic lasing. The lasing behavior revealed that plasmon–exciton energy transfer depends on polarization, with stronger coupling and faster dynamics when the transition dipole moments of the excited gain are aligned with the electric field of the plasmon modes.},

  doi          = {10.1021/acsnano.9b01142},

  journal      = {ACS Nano},

  number       = 7,

  volume       = 13,

  place        = {United States},

  year         = {Tue Apr 02 00:00:00 EDT 2019},

  month        = {Tue Apr 02 00:00:00 EDT 2019}

}

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Title: Polarization-Dependent Lasing Behavior from Low-Symmetry Nanocavity Arrays

Abstract

Citation Formats

Nanophotonics: Shrinking light-based technology journal, April 2015

Structural Engineering in Plasmon Nanolasers journal, October 2017

Symmetry Breaking in Tetrahedral Chiral Plasmonic Nanoparticle Assemblies journal, October 2014

Circular Differential Scattering of Single Chiral Self-Assembled Gold Nanorod Dimers journal, October 2015

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Quasiperiodic Moiré Plasmonic Crystals journal, November 2013

Optics of photonic quasicrystals journal, February 2013

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Quasicrystals enter third dimension journal, February 2007

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Theoretical studies of plasmon resonances in one-dimensional nanoparticle chains: narrow lineshapes with tunable widths journal, May 2006

Experimental observation of narrow surface plasmon resonances in gold nanoparticle arrays journal, November 2008

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