Temperature-induced amorphization in CaCO3 at high pressure and implications for recycled CaCO3 in subduction zones
Abstract
Calcium carbonate (CaCO3) significantly affects the properties of upper mantle and plays a key role in deep carbon recycling. However, its phase relations above 3 GPa and 1000 K are controversial. Here we report a reversible temperature-induced aragonite-amorphization transition in CaCO3 at 3.9-7.5 GPa and temperature above 1000 K. Amorphous CaCO3 shares a similar structure as liquid CaCO3 but with much larger C-O and Ca-Ca bond lengths, indicating a lower density and a mechanism of lattice collapse for the temperature-induced amorphous phase. The less dense amorphous phase compared with the liquid provides an explanation for the observed CaCO3 melting curve overturn at about 6 GPa. Amorphous CaCO3 is stable at subduction zone conditions and could aid the recycling of carbon to the surface.
- Authors:
-
[5];
- Center for High Pressure Science and Technology Advanced Research, Shanghai (China); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Center for High Pressure Science and Technology Advanced Research, Shanghai (China)
- Carnegie Inst. of Washington, Washington, DC (United States)
- CEA Key Laboratory of Earthquake Prediction, Institute of Earthquake Science, Beijing (China)
- Carnegie Inst. of Washington, Argonne, IL (United States)
- Center for High Pressure Science and Technology Advanced Research, Shanghai (China); Carnegie Inst. of Washington, Washington, DC (United States)
- Carnegie Inst. of Washington, Washington, DC (United States); Ehime Univ., Matsuyama (Japan)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1559210
- Grant/Contract Number:
- AC02-05CH11231; NA0001974; AC02-06CH11357; FG02-99ER45775
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 58 GEOSCIENCES
Citation Formats
Hou, Mingqiang, Zhang, Qian, Tao, Renbiao, Liu, Hong, Kono, Yoshio, Mao, Ho-kwang, Yang, Wenge, Chen, Bin, and Fei, Yingwei. Temperature-induced amorphization in CaCO3 at high pressure and implications for recycled CaCO3 in subduction zones. United States: N. p., 2019.
Web. doi:10.1038/s41467-019-09742-5.
Hou, Mingqiang, Zhang, Qian, Tao, Renbiao, Liu, Hong, Kono, Yoshio, Mao, Ho-kwang, Yang, Wenge, Chen, Bin, & Fei, Yingwei. Temperature-induced amorphization in CaCO3 at high pressure and implications for recycled CaCO3 in subduction zones. United States. https://doi.org/10.1038/s41467-019-09742-5
Hou, Mingqiang, Zhang, Qian, Tao, Renbiao, Liu, Hong, Kono, Yoshio, Mao, Ho-kwang, Yang, Wenge, Chen, Bin, and Fei, Yingwei. Mon .
"Temperature-induced amorphization in CaCO3 at high pressure and implications for recycled CaCO3 in subduction zones". United States. https://doi.org/10.1038/s41467-019-09742-5. https://www.osti.gov/servlets/purl/1559210.
@article{osti_1559210,
title = {Temperature-induced amorphization in CaCO3 at high pressure and implications for recycled CaCO3 in subduction zones},
author = {Hou, Mingqiang and Zhang, Qian and Tao, Renbiao and Liu, Hong and Kono, Yoshio and Mao, Ho-kwang and Yang, Wenge and Chen, Bin and Fei, Yingwei},
abstractNote = {Calcium carbonate (CaCO3) significantly affects the properties of upper mantle and plays a key role in deep carbon recycling. However, its phase relations above 3 GPa and 1000 K are controversial. Here we report a reversible temperature-induced aragonite-amorphization transition in CaCO3 at 3.9-7.5 GPa and temperature above 1000 K. Amorphous CaCO3 shares a similar structure as liquid CaCO3 but with much larger C-O and Ca-Ca bond lengths, indicating a lower density and a mechanism of lattice collapse for the temperature-induced amorphous phase. The less dense amorphous phase compared with the liquid provides an explanation for the observed CaCO3 melting curve overturn at about 6 GPa. Amorphous CaCO3 is stable at subduction zone conditions and could aid the recycling of carbon to the surface.},
doi = {10.1038/s41467-019-09742-5},
journal = {Nature Communications},
number = 1,
volume = 10,
place = {United States},
year = {Mon Apr 29 00:00:00 EDT 2019},
month = {Mon Apr 29 00:00:00 EDT 2019}
}
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CaSiO3 perovskite in diamond indicates the recycling of oceanic crust into the lower mantle
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Reversible switching between pressure-induced amorphization and thermal-driven recrystallization in VO2(B) nanosheets
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Ultralow viscosity of carbonate melts at high pressures
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Ponded melt at the boundary between the lithosphere and asthenosphere
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Carbon dioxide released from subduction zones by fluid-mediated reactions
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Structural evolution of calcite at high temperatures: Phase V unveiled
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General 2.5 power law of metallic glasses
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Temperature-induced amorphization of Na-zeolite A: A view from multi-nuclear high-resolution solid-state NMR
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- Foustoukos, D. I.; Mysen, B. O.
- American Mineralogist, Vol. 100, Issue 1
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journal, July 2007
- Ono, S.; Kikegawa, T.; Ohishi, Y.
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The high pressure behavior of miscellaneous minerals
journal, December 1938
- Bridgman, P. W.
- American Journal of Science, Vol. 237, Issue 1
Works referencing / citing this record:
Microdynamic changes of moisture-induced crystallization of amorphous calcium carbonate revealed via in situ FTIR spectroscopy
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