Dual-comb spectroscopy of laser-induced plasmas

Bergevin, Jenna; Wu, Tsung-Han; Yeak, Jeremy N.; Brumfield, Brian E.; Harilal, Sivanandan S.; Phillips, Mark C.; Jones, R Jason

doi:10.1038/s41467-018-03703-0

Title: Dual-comb spectroscopy of laser-induced plasmas

Abstract

Dual-comb spectroscopy has become a powerful spectroscopic technique in applications that rely on its broad spectral coverage combined with high frequency resolution capabilities. Experiments to date have primarily focused on detection and analysis of multiple gas species under semi-static conditions, with applications ranging from environmental monitoring of greenhouse gases to high resolution molecular spectroscopy. Here, we utilize dual-comb spectroscopy to demonstrate broadband, high-resolution, and time-resolved measurements in a laser induced plasma for the first time. As a first demonstration, we simultaneously detect trace amounts of Rb and K in solid samples with a single laser ablation shot, with transitions separated by over 6 THz (13 nm) and spectral resolution sufficient to resolve isotopic and ground state hyperfine splittings of the Rb D₂ line. This new spectroscopic approach offers the broad spectral coverage found in the powerful techniques of laser-induced breakdown spectroscopy (LIBS) while providing the high-resolution and accuracy of cw laser-based spectroscopies.

Authors:

Bergevin, Jenna ^[1]; Wu, Tsung-Han ^[1]; Yeak, Jeremy N. ^[2]; Brumfield, Brian E. ^[3];

^[3]; Phillips, Mark C. ^[3]; Jones, R Jason ^[1]

Univ. of Arizona, Tucson, AZ (United States)
PM&AM Research, Tucson, AZ (United States)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

Publication Date:: Wed Mar 28 00:00:00 EDT 2018

Research Org.:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1529991

Report Number(s):: PNNL-SA-132479
Journal ID: ISSN 2041-1723

Grant/Contract Number:: AC05-76RL01830

Resource Type:: Accepted Manuscript

Journal Name:: Nature Communications

Additional Journal Information:: Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: Laser-induced breakdown; Optical Sensing; Plasma Diagnostics; Isotope shifts; Frequency comb; laser absorption spectroscopy

Citation Formats


                    Bergevin, Jenna, Wu, Tsung-Han, Yeak, Jeremy N., Brumfield, Brian E., Harilal, Sivanandan S., Phillips, Mark C., and Jones, R Jason. Dual-comb spectroscopy of laser-induced plasmas.  United States: N. p., 2018. 
Web.  doi:10.1038/s41467-018-03703-0.

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                    Bergevin, Jenna, Wu, Tsung-Han, Yeak, Jeremy N., Brumfield, Brian E., Harilal, Sivanandan S., Phillips, Mark C., & Jones, R Jason. Dual-comb spectroscopy of laser-induced plasmas.  United States.  https://doi.org/10.1038/s41467-018-03703-0

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                    Bergevin, Jenna, Wu, Tsung-Han, Yeak, Jeremy N., Brumfield, Brian E., Harilal, Sivanandan S., Phillips, Mark C., and Jones, R Jason. Wed .  
"Dual-comb spectroscopy of laser-induced plasmas".  United States.  https://doi.org/10.1038/s41467-018-03703-0.  https://www.osti.gov/servlets/purl/1529991.

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@article{osti_1529991,

  title        = {Dual-comb spectroscopy of laser-induced plasmas},

  author       = {Bergevin, Jenna and Wu, Tsung-Han and Yeak, Jeremy N. and Brumfield, Brian E. and Harilal, Sivanandan S. and Phillips, Mark C. and Jones, R Jason},

  abstractNote = {Dual-comb spectroscopy has become a powerful spectroscopic technique in applications that rely on its broad spectral coverage combined with high frequency resolution capabilities. Experiments to date have primarily focused on detection and analysis of multiple gas species under semi-static conditions, with applications ranging from environmental monitoring of greenhouse gases to high resolution molecular spectroscopy. Here, we utilize dual-comb spectroscopy to demonstrate broadband, high-resolution, and time-resolved measurements in a laser induced plasma for the first time. As a first demonstration, we simultaneously detect trace amounts of Rb and K in solid samples with a single laser ablation shot, with transitions separated by over 6 THz (13 nm) and spectral resolution sufficient to resolve isotopic and ground state hyperfine splittings of the Rb D2 line. This new spectroscopic approach offers the broad spectral coverage found in the powerful techniques of laser-induced breakdown spectroscopy (LIBS) while providing the high-resolution and accuracy of cw laser-based spectroscopies.},

  doi          = {10.1038/s41467-018-03703-0},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 9,

  place        = {United States},

  year         = {Wed Mar 28 00:00:00 EDT 2018},

  month        = {Wed Mar 28 00:00:00 EDT 2018}

}

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https://doi.org/10.1038/s41467-018-03703-0

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Cited by: 49 works

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Figures / Tables:

Fig. 1 : Schematic of experimental layout. A pair of modelocked fs lasers, Comb-1 and Comb-2, are actively stabilized to a common cw laser using optical phase-locked loops to enable high-resolution dual-comb spectroscopy of a laser-induced plasma. The laser beams are spatially overlapped on a beamsplitter and simultaneously probe amore »

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Optical–optical double-resonance dual-comb spectroscopy with pump-intensity modulation
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Nishiyama, Akiko; Nakajima, Yoshiaki; Nakagawa, Ken’ichi
Optics Express, Vol. 27, Issue 25
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Time-resolved dual-comb measurement of number density and temperature in a laser-induced plasma
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Title: Dual-comb spectroscopy of laser-induced plasmas

Abstract

Citation Formats

Figures / Tables:

Laser ablation absorption spectroscopy for isotopic analysis of plutonium: Spectroscopic properties and analytical performance journal, August 2017

Monitoring Uranium, Hydrogen, and Lithium and Their Isotopes Using a Compact Laser-Induced Breakdown Spectroscopy (LIBS) Probe and High-Resolution Spectrometer journal, March 2012

Exploring laser-induced breakdown spectroscopy for nuclear materials analysis and in-situ applications journal, August 2012

Analysis of relaxing laser-induced plasmas by absorption spectroscopy: Toward a new quantitative diagnostic technique journal, July 2010

Rubidium isotope measurements in solid samples by laser ablation-laser atomic absorption spectroscopy journal, December 1999

Two-dimensional fluorescence spectroscopy of laser-produced plasmas journal, January 2016

Practical high-resolution detection method for laser-induced breakdown spectroscopy journal, January 2012

Analysis of relaxing laser-induced plasmas by absorption spectroscopy: Toward a new quantitative diagnostic technique journal, July 2010

Optical frequency comb spectroscopy journal, January 2011

Absorption spectroscopy of uranium plasma for remote isotope analysis of next-generation nuclear fuel journal, September 2012

Exploring laser-induced breakdown spectroscopy for nuclear materials analysis and in-situ applications journal, August 2012

Evaluation of Na and K in anti-diabetic ayurvedic medicine using LIBS journal, March 2021

Laser-Induced Breakdown Spectroscopy (LIBS), Part I: Review of Basic Diagnostics and Plasma—Particle Interactions: Still-Challenging Issues within the Analytical Plasma Community journal, December 2010

Geological Applications of Laser-Induced Breakdown Spectroscopy journal, August 2014

Isotope ratio analysis on micron-sized particles in complex matrices by Laser Ablation-Absorption Ratio Spectrometry journal, November 2009

A frequency comb in the extreme ultraviolet journal, July 2005

Laser-induced breakdown spectroscopy-based investigation and classification of pharmaceutical tablets using multivariate chemometric analysis journal, December 2011

Laser Ablation journal, September 1995

Laser-Induced Breakdown Spectroscopy (LIBS), Part I: Review of Basic Diagnostics and Plasma—Particle Interactions: Still-Challenging Issues within the Analytical Plasma Community journal, December 2010

Phase-Coherent Frequency Combs in the Vacuum Ultraviolet via High-Harmonic Generation inside a Femtosecond Enhancement Cavity journal, May 2005

Development of ultrafast time-resolved dual-comb spectroscopy journal, February 2017

Development of ultrafast time-resolved dual-comb spectroscopy journal, February 2017

Optical frequency comb spectroscopy journal, January 2011

Hybrid interferometric/dispersive atomic spectroscopy of laser-induced uranium plasma journal, February 2016

High-resolution spectroscopy of laser ablation plumes using laser-induced fluorescence journal, January 2017

Diode laser absorption measurement of uranium isotope ratios in solid samples using laser ablation journal, October 2002

Differential laser absorption spectroscopy of uranium in an atmospheric pressure laser-induced plasma journal, January 2014

Frequency-comb-based remote sensing of greenhouse gases over kilometer air paths journal, January 2014

Measurement of uranium isotope ratios in solid samples using laser ablation and diode laser-excited atomic fluorescence spectrometry journal, June 1999

Cavity-enhanced dual-comb spectroscopy text, January 2009

Review of in-situ process monitoring and in-situ metrology for metal additive manufacturing journal, April 2016

Mid-Infrared Time-Resolved Frequency Comb Spectroscopy of Transient Free Radicals journal, June 2014

The ChemCam Instrument Suite on the Mars Science Laboratory (MSL) Rover: Science Objectives and Mast Unit Description journal, July 2012

Mid-Infrared Time-Resolved Frequency Comb Spectroscopy of Transient Free Radicals journal, June 2014

Two-dimensional fluorescence spectroscopy of uranium isotopes in femtosecond laser ablation plumes journal, June 2017

Mid-infrared frequency combs journal, June 2012

Mid-infrared frequency combs journal, June 2012

Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm journal, July 2015

Sensitivity of coherent dual-comb spectroscopy journal, January 2010

The ChemCam Instrument Suite on the Mars Science Laboratory (MSL) Rover: Science Objectives and Mast Unit Description journal, July 2012

Dual-comb spectroscopy using frequency-doubled combs around 775 nm journal, January 2013

Coherent dual-comb spectroscopy at high signal-to-noise ratio journal, October 2010

Colloquium : Femtosecond optical frequency combs journal, March 2003

Coherent Multiheterodyne Spectroscopy Using Stabilized Optical Frequency Combs journal, January 2008

Multispecies absorption spectroscopy of detonation events at 100 kHz using a fiber-coupled, time-division-multiplexed quantum-cascade-laser system journal, January 2016

Dual-Comb Spectroscopy journal, January 2017

Laser spectrometry for multi-elemental imaging of biological tissues journal, August 2014

Laser Ablation journal, September 1995

Dual-Comb Spectroscopy journal, January 2014

A frequency comb in the extreme ultraviolet conference, January 2005

Cavity-enhanced dual-comb spectroscopy journal, November 2009

Dual-comb spectroscopy journal, January 2016

Comb-Resolved Dual-Comb Spectroscopy Stabilized by Free-Running Continuous-Wave Lasers journal, October 2012

Forensic application of laser-induced breakdown spectroscopy for the discrimination of questioned documents journal, September 2015

Hybrid interferometric/dispersive atomic spectroscopy of laser-induced uranium plasma journal, February 2016

In situ probing of mode-locked vertical-external-cavity-surface-emitting lasers journal, January 2015

Laser spectrometry for multi-elemental imaging of biological tissues journal, August 2014

Two-dimensional fluorescence spectroscopy of uranium isotopes in femtosecond laser ablation plumes journal, June 2017

Coherent, multi-heterodyne spectroscopy using stabilized optical frequency combs text, January 2007

Optical–optical double-resonance dual-comb spectroscopy with pump-intensity modulation journal, January 2019

Time-resolved mid-infrared dual-comb spectroscopy journal, November 2019

Laser induced breakdown in pulsed helium atmospheric pressure plasma jet journal, May 2019

Frequency comb spectroscopy journal, February 2019

Time-resolved dual-comb measurement of number density and temperature in a laser-induced plasma journal, January 2019

Time-resolved mid-infrared dual-comb spectroscopy journal, November 2019

Frequency comb spectroscopy text, January 2019

Physical conditions for UO formation in laser-produced uranium plumes journal, January 2019

Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis journal, June 2018

Broadband Time-Resolved Absorption and Dispersion Spectroscopy of Methane and Ethane in a Plasma Using a Mid-Infrared Dual-Comb Spectrometer journal, November 2020

11-μs time-resolved, continuous dual-comb spectroscopy with spectrally filtered mode-locked frequency combs journal, January 2021

Laser ablation absorption spectroscopy for isotopic analysis of plutonium: Spectroscopic properties and analytical performance
journal, August 2017

Monitoring Uranium, Hydrogen, and Lithium and Their Isotopes Using a Compact Laser-Induced Breakdown Spectroscopy (LIBS) Probe and High-Resolution Spectrometer
journal, March 2012

Exploring laser-induced breakdown spectroscopy for nuclear materials analysis and in-situ applications
journal, August 2012

Analysis of relaxing laser-induced plasmas by absorption spectroscopy: Toward a new quantitative diagnostic technique
journal, July 2010

Rubidium isotope measurements in solid samples by laser ablation-laser atomic absorption spectroscopy
journal, December 1999

Two-dimensional fluorescence spectroscopy of laser-produced plasmas
journal, January 2016

Practical high-resolution detection method for laser-induced breakdown spectroscopy
journal, January 2012

Analysis of relaxing laser-induced plasmas by absorption spectroscopy: Toward a new quantitative diagnostic technique
journal, July 2010

Optical frequency comb spectroscopy
journal, January 2011

Absorption spectroscopy of uranium plasma for remote isotope analysis of next-generation nuclear fuel
journal, September 2012

Exploring laser-induced breakdown spectroscopy for nuclear materials analysis and in-situ applications
journal, August 2012

Evaluation of Na and K in anti-diabetic ayurvedic medicine using LIBS
journal, March 2021

Laser-Induced Breakdown Spectroscopy (LIBS), Part I: Review of Basic Diagnostics and Plasma—Particle Interactions: Still-Challenging Issues within the Analytical Plasma Community
journal, December 2010

Geological Applications of Laser-Induced Breakdown Spectroscopy
journal, August 2014

Isotope ratio analysis on micron-sized particles in complex matrices by Laser Ablation-Absorption Ratio Spectrometry
journal, November 2009

A frequency comb in the extreme ultraviolet
journal, July 2005

Laser-induced breakdown spectroscopy-based investigation and classification of pharmaceutical tablets using multivariate chemometric analysis
journal, December 2011

Laser Ablation
journal, September 1995

Laser-Induced Breakdown Spectroscopy (LIBS), Part I: Review of Basic Diagnostics and Plasma—Particle Interactions: Still-Challenging Issues within the Analytical Plasma Community
journal, December 2010

Phase-Coherent Frequency Combs in the Vacuum Ultraviolet via High-Harmonic Generation inside a Femtosecond Enhancement Cavity
journal, May 2005

Development of ultrafast time-resolved dual-comb spectroscopy
journal, February 2017

Development of ultrafast time-resolved dual-comb spectroscopy
journal, February 2017

Optical frequency comb spectroscopy
journal, January 2011

Hybrid interferometric/dispersive atomic spectroscopy of laser-induced uranium plasma
journal, February 2016

High-resolution spectroscopy of laser ablation plumes using laser-induced fluorescence
journal, January 2017

Diode laser absorption measurement of uranium isotope ratios in solid samples using laser ablation
journal, October 2002

Differential laser absorption spectroscopy of uranium in an atmospheric pressure laser-induced plasma
journal, January 2014

Frequency-comb-based remote sensing of greenhouse gases over kilometer air paths
journal, January 2014

Measurement of uranium isotope ratios in solid samples using laser ablation and diode laser-excited atomic fluorescence spectrometry
journal, June 1999

Cavity-enhanced dual-comb spectroscopy
text, January 2009

Review of in-situ process monitoring and in-situ metrology for metal additive manufacturing
journal, April 2016

Mid-Infrared Time-Resolved Frequency Comb Spectroscopy of Transient Free Radicals
journal, June 2014

The ChemCam Instrument Suite on the Mars Science Laboratory (MSL) Rover: Science Objectives and Mast Unit Description
journal, July 2012

Mid-Infrared Time-Resolved Frequency Comb Spectroscopy of Transient Free Radicals
journal, June 2014

Two-dimensional fluorescence spectroscopy of uranium isotopes in femtosecond laser ablation plumes
journal, June 2017

Mid-infrared frequency combs
journal, June 2012

Mid-infrared frequency combs
journal, June 2012

Ultra-broadband dual-comb spectroscopy across 1.0–1.9 µm
journal, July 2015

Sensitivity of coherent dual-comb spectroscopy
journal, January 2010

The ChemCam Instrument Suite on the Mars Science Laboratory (MSL) Rover: Science Objectives and Mast Unit Description
journal, July 2012

Dual-comb spectroscopy using frequency-doubled combs around 775 nm
journal, January 2013

Coherent dual-comb spectroscopy at high signal-to-noise ratio
journal, October 2010

Colloquium : Femtosecond optical frequency combs
journal, March 2003

Coherent Multiheterodyne Spectroscopy Using Stabilized Optical Frequency Combs
journal, January 2008

Multispecies absorption spectroscopy of detonation events at 100 kHz using a fiber-coupled, time-division-multiplexed quantum-cascade-laser system
journal, January 2016

Dual-Comb Spectroscopy
journal, January 2017

Laser spectrometry for multi-elemental imaging of biological tissues
journal, August 2014

Laser Ablation
journal, September 1995

Dual-Comb Spectroscopy
journal, January 2014

A frequency comb in the extreme ultraviolet
conference, January 2005

Cavity-enhanced dual-comb spectroscopy
journal, November 2009

Dual-comb spectroscopy
journal, January 2016

Comb-Resolved Dual-Comb Spectroscopy Stabilized by Free-Running Continuous-Wave Lasers
journal, October 2012

Forensic application of laser-induced breakdown spectroscopy for the discrimination of questioned documents
journal, September 2015

Hybrid interferometric/dispersive atomic spectroscopy of laser-induced uranium plasma
journal, February 2016

In situ probing of mode-locked vertical-external-cavity-surface-emitting lasers
journal, January 2015

Laser spectrometry for multi-elemental imaging of biological tissues
journal, August 2014

Two-dimensional fluorescence spectroscopy of uranium isotopes in femtosecond laser ablation plumes
journal, June 2017

Coherent, multi-heterodyne spectroscopy using stabilized optical frequency combs
text, January 2007

Optical–optical double-resonance dual-comb spectroscopy with pump-intensity modulation
journal, January 2019

Time-resolved mid-infrared dual-comb spectroscopy
journal, November 2019

Laser induced breakdown in pulsed helium atmospheric pressure plasma jet
journal, May 2019

Frequency comb spectroscopy
journal, February 2019

Time-resolved dual-comb measurement of number density and temperature in a laser-induced plasma
journal, January 2019

Time-resolved mid-infrared dual-comb spectroscopy
journal, November 2019

Frequency comb spectroscopy
text, January 2019

Physical conditions for UO formation in laser-produced uranium plumes
journal, January 2019

Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis
journal, June 2018

Broadband Time-Resolved Absorption and Dispersion Spectroscopy of Methane and Ethane in a Plasma Using a Mid-Infrared Dual-Comb Spectrometer
journal, November 2020

11-μs time-resolved, continuous dual-comb spectroscopy with spectrally filtered mode-locked frequency combs
journal, January 2021