Production and isolation of 197m,gHg

Despotopulos, John D.; Kmak, Kelly N.; Shaughnessy, Dawn A.

doi:10.1007/s10967-018-5927-9

Title: Production and isolation of ^197m,gHg

Abstract

A new procedure has been developed for isolating no-carrier-added ^197m,gHg from 20 to 25 MeV a-particle irradiations of high purity Pt foils. A previously published procedure for isolation of ^197m,gHg from 12 to 15 MeV proton irradiations of Au foils has been further characterized. From these procedures two separate methods have been established to isolate, with high separation factors, ^197m,gHg from Pt to Au target materials.

Authors:

Despotopulos, John D. ^[1]; Kmak, Kelly N. ^[2]; Shaughnessy, Dawn A. ^[1]

Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of California, Berkeley, CA (United States)

Publication Date:: Tue Jun 05 00:00:00 EDT 2018

Research Org.:: Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Berkeley, CA (United States). Nuclear Science and Security Consortium

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation

OSTI Identifier:: 1526853

Alternate Identifier(s):: OSTI ID: 1462385

Report Number(s):: LLNL-JRNL-749092
Journal ID: ISSN 0236-5731; 931375

Grant/Contract Number:: AC52-07NA27344; NA0003180

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Radioanalytical and Nuclear Chemistry

Additional Journal Information:: Journal Volume: 317; Journal Issue: 2; Journal ID: ISSN 0236-5731

Publisher:: Springer

Country of Publication:: United States

Language:: English

Subject:: 07 ISOTOPE AND RADIATION SOURCES; Mercury; No-carrier-added; Separation; Extraction chromatography

Citation Formats


                    Despotopulos, John D., Kmak, Kelly N., and Shaughnessy, Dawn A. Production and isolation of 197m,gHg.  United States: N. p., 2018. 
Web.  doi:10.1007/s10967-018-5927-9.

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                    Despotopulos, John D., Kmak, Kelly N., & Shaughnessy, Dawn A. Production and isolation of 197m,gHg.  United States.  https://doi.org/10.1007/s10967-018-5927-9

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                    Despotopulos, John D., Kmak, Kelly N., and Shaughnessy, Dawn A. Tue .  
"Production and isolation of 197m,gHg".  United States.  https://doi.org/10.1007/s10967-018-5927-9.  https://www.osti.gov/servlets/purl/1526853.

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@article{osti_1526853,

  title        = {Production and isolation of 197m,gHg},

  author       = {Despotopulos, John D. and Kmak, Kelly N. and Shaughnessy, Dawn A.},

  abstractNote = {A new procedure has been developed for isolating no-carrier-added 197m,gHg from 20 to 25 MeV a-particle irradiations of high purity Pt foils. A previously published procedure for isolation of 197m,gHg from 12 to 15 MeV proton irradiations of Au foils has been further characterized. From these procedures two separate methods have been established to isolate, with high separation factors, 197m,gHg from Pt to Au target materials.},

  doi          = {10.1007/s10967-018-5927-9},

  journal      = {Journal of Radioanalytical and Nuclear Chemistry},

  number       = 2,

  volume       = 317,

  place        = {United States},

  year         = {Tue Jun 05 00:00:00 EDT 2018},

  month        = {Tue Jun 05 00:00:00 EDT 2018}

}

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Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (DOE)

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https://doi.org/10.1007/s10967-018-5927-9

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Cited by: 9 works

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Figures / Tables:

Fig. 1: Column elution of 2 mL, pre-packed, Eichrom TEVA resin cartridges at ~1 mL/min flow rate for the separation of trace Hg from Pt foil. Errors presented are counting errors. Lines are to guide the eye only.

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Works referenced in this record:

Theranostic mercury part 1: A new Hg/Au separation by a resin based method
conference, January 2017

Walther, M.; Lebeda, O.; Preusche, S.
WTTC16: Proceedings of the 16th International Workshop on Targetry and Target Chemistry, AIP Conference Proceedings
DOI: 10.1063/1.4983554

Theranostic mercury: 197(m) Hg with high specific activity for imaging and therapy
journal, March 2015

Walther, Martin; Preusche, Stephan; Bartel, Stig
Applied Radiation and Isotopes, Vol. 97
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Distribution of Radiomercury Administered as Labelled Chlormerodrin (Neohydrin®) in the Kidneys of rats and dogs 1
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Greif, Roger L.; Sullivan, W. James; Jacobs, Gloria S.
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(p, n) and (p, 2n) cross sections of nine elements between 7.0 and 15.0 MeV
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Chodil, G.; Jopson, R. C.
Nuclear Physics A, Vol. 93, Issue 3
DOI: 10.1016/0375-9474(67)90312-0

Cross sections for the formation of ${}^{195}{Hg}$ $^{m, g}$ , ${}^{197}{Hg}$ $^{m, g}$ , and ${}^{196}{Au}$ $^{m, g}$ in α and ${}^{3}{He}$ -particle induced reactions on Pt: Effect of level density parameters on the calculated isomeric cross-section ratio
journal, March 2006

Sudár, S.; Qaim, S. M.
Physical Review C, Vol. 73, Issue 3
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Production of Carrier-free 197m,197Hg with a Cyclotron
journal, January 1972

Wilkniss, P. E.; Beach, L. A.; Marlow, K. W.
Radiochimica Acta, Vol. 17, Issue 2
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Cyclotron production of 197mHg and its use for lung tumor imaging
journal, November 1973

Toshihiko Hara,
The International Journal of Applied Radiation and Isotopes, Vol. 24, Issue 11
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Production, separation and speciation of no-carrier-added Hg radionuclides using greener methodologies
journal, January 2010

Mandal, S.; Nayak, Dalia
Radiochimica Acta, Vol. 98, Issue 1
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Measurement of naturally occurring radioactive materials, 238U and 232Th: anomalies in photopeak selection
journal, August 2016

Naskar, Nabanita; Lahiri, Susanta; Chaudhuri, Punarbasu
Journal of Radioanalytical and Nuclear Chemistry, Vol. 310, Issue 3
DOI: 10.1007/s10967-016-4988-x

Production and isolation of homologs of flerovium and element 115 at the Lawrence Livermore National Laboratory Center for Accelerator Mass Spectrometry
journal, October 2015

Despotopulos, John D.; Kmak, Kelly N.; Gharibyan, Narek
Journal of Radioanalytical and Nuclear Chemistry, Vol. 308, Issue 2
DOI: 10.1007/s10967-015-4500-z

Anion Exchange Characteristics of the Elements in Nitric Acid Medium.
journal, May 1964

Faris, J. P.; Buchanan, R. F.
Analytical Chemistry, Vol. 36, Issue 6
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The dissolution and recovery of iridium in a nitrate system
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Silver, G. L.
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Figures / Tables found in this record:

Fig. 1 (p. 8)

Fig 2 (p. 10)

Table-1 (p. 11)

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Similar Records

Title: Production and isolation of 197m,gHg

Abstract

Citation Formats

Figures / Tables:

Theranostic mercury part 1: A new Hg/Au separation by a resin based method conference, January 2017

Theranostic mercury: 197(m) Hg with high specific activity for imaging and therapy journal, March 2015

Distribution of Radiomercury Administered as Labelled Chlormerodrin (Neohydrin®) in the Kidneys of rats and dogs 1 journal, January 1956

(p, n) and (p, 2n) cross sections of nine elements between 7.0 and 15.0 MeV journal, March 1967

Cross sections for the formation of Hg 195 m , g , Hg 197 m , g , and Au 196 m , g in α and He 3 -particle induced reactions on Pt: Effect of level density parameters on the calculated isomeric cross-section ratio journal, March 2006

Production of Carrier-free 197m,197Hg with a Cyclotron journal, January 1972

Cyclotron production of 197mHg and its use for lung tumor imaging journal, November 1973

Production, separation and speciation of no-carrier-added Hg radionuclides using greener methodologies journal, January 2010

Measurement of naturally occurring radioactive materials, 238U and 232Th: anomalies in photopeak selection journal, August 2016

Production and isolation of homologs of flerovium and element 115 at the Lawrence Livermore National Laboratory Center for Accelerator Mass Spectrometry journal, October 2015

Anion Exchange Characteristics of the Elements in Nitric Acid Medium. journal, May 1964

The dissolution and recovery of iridium in a nitrate system journal, April 1975

Title: Production and isolation of ^197m,gHg

Theranostic mercury part 1: A new Hg/Au separation by a resin based method
conference, January 2017

Theranostic mercury: 197(m) Hg with high specific activity for imaging and therapy
journal, March 2015

Distribution of Radiomercury Administered as Labelled Chlormerodrin (Neohydrin®) in the Kidneys of rats and dogs 1
journal, January 1956

(p, n) and (p, 2n) cross sections of nine elements between 7.0 and 15.0 MeV
journal, March 1967

Cross sections for the formation of ${}^{195}{Hg}$ $^{m, g}$ , ${}^{197}{Hg}$ $^{m, g}$ , and ${}^{196}{Au}$ $^{m, g}$ in α and ${}^{3}{He}$ -particle induced reactions on Pt: Effect of level density parameters on the calculated isomeric cross-section ratio
journal, March 2006

Production of Carrier-free 197m,197Hg with a Cyclotron
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Cyclotron production of 197mHg and its use for lung tumor imaging
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Production, separation and speciation of no-carrier-added Hg radionuclides using greener methodologies
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Measurement of naturally occurring radioactive materials, 238U and 232Th: anomalies in photopeak selection
journal, August 2016

Production and isolation of homologs of flerovium and element 115 at the Lawrence Livermore National Laboratory Center for Accelerator Mass Spectrometry
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The dissolution and recovery of iridium in a nitrate system
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