Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

Sun, X. M.; Cong, D. Y.; Li, Z.; Zhang, Y. L.; Chen, Z.; Ren, Y.; Liss, K. -D.; Ma, Z. Y.; Li, R. G.; Qu, Y. H.; Yang, Z.; Wang, L.; Wang, Y. D.

doi:10.1103/PhysRevMaterials.3.034404

Title: Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

Abstract

Promising multifunctional magnetoresponsive effects such as magnetoresistance, magnetostrain, and the magnetocaloric effect have recently been extensively studied in Ni-Mn-based metamagnetic shape memory alloys, but large reversible magnetoresponsive effects are usually obtained under high magnetic fields, which is an obstacle for practical applications. In this work, through manipulating magnetostructural transition, we achieved large reversible magnetoresponsive effects under a relatively low magnetic field of 3 T in a Ni-Co-Mn-In alloy. By systematically tuning the Mn/In ratio and Co substitution, an optimum composition Ni₄₉Co₃Mn₃₄In₁₄ with a low thermal hysteresis (8 K), a narrow transformation interval (7 K) and a high sensitivity of transformation temperature to field change (6KT^-1), was obtained. Good geometric compatibility between austenite and martensite was revealed by in situ synchrotron high-energy x-ray diffraction experiment, which accounts for the low hysteresis and narrow transformation interval. A reversible transformation between pure austenite and pure martensite is induced by a relatively low field of 3 T, which was directly evidenced by in situ neutron diffraction experiments. As a result, a large reversible magnetocaloric effect with entropy change of 16.5Jkg^-1K^-1, a large reversible magnetostrain of 0.26%, and a large reversible magnetoresistance of 60%, under a relatively low field of 3 T, were simultaneously achieved.more »« less

Authors:

Sun, X. M. ^[1]; Cong, D. Y. ^[1]; Li, Z. ^[2]; Zhang, Y. L. ^[2]; Chen, Z. ^[1]; Ren, Y. ^[3]; Liss, K. -D. ^[4]; Ma, Z. Y. ^[5]; Li, R. G. ^[1]; Qu, Y. H. ^[1]; Yang, Z. ^[1]; Wang, L. ^[6]; Wang, Y. D. ^[1]

Univ. of Science and Technology Beijing, (China)
Qujing Normal Univ., (China)
Argonne National Lab. (ANL), Lemont, IL (United States)
Australian Nuclear Science and Technology Organisation (ANSTO), Lucas Heights, NSW (Australia); Guangdong Technion-Israel Inst. of Technology, Shantou (China)
China Univ. of Petroleum, Beijing (China)
Beijing Inst. of Technology, Beijing (China)

Publication Date:: Mon Mar 11 00:00:00 EDT 2019

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; National Natural Science Foundation of China (NSFC)

OSTI Identifier:: 1524778

Alternate Identifier(s):: OSTI ID: 1498811

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Materials

Additional Journal Information:: Journal Volume: 3; Journal Issue: 3; Journal ID: ISSN 2475-9953

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; Metamagnetic shape memory alloy; Martensitic transformation; Magnetocaloric effect; Magnetostrain; Magnetoresistance

Citation Formats


                    Sun, X. M., Cong, D. Y., Li, Z., Zhang, Y. L., Chen, Z., Ren, Y., Liss, K. -D., Ma, Z. Y., Li, R. G., Qu, Y. H., Yang, Z., Wang, L., and Wang, Y. D. Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevMaterials.3.034404.

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                    Sun, X. M., Cong, D. Y., Li, Z., Zhang, Y. L., Chen, Z., Ren, Y., Liss, K. -D., Ma, Z. Y., Li, R. G., Qu, Y. H., Yang, Z., Wang, L., & Wang, Y. D. Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys.  United States.  https://doi.org/10.1103/PhysRevMaterials.3.034404

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                    Sun, X. M., Cong, D. Y., Li, Z., Zhang, Y. L., Chen, Z., Ren, Y., Liss, K. -D., Ma, Z. Y., Li, R. G., Qu, Y. H., Yang, Z., Wang, L., and Wang, Y. D. Mon .  
"Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys".  United States.  https://doi.org/10.1103/PhysRevMaterials.3.034404.  https://www.osti.gov/servlets/purl/1524778.

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@article{osti_1524778,

  title        = {Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys},

  author       = {Sun, X. M. and Cong, D. Y. and Li, Z. and Zhang, Y. L. and Chen, Z. and Ren, Y. and Liss, K. -D. and Ma, Z. Y. and Li, R. G. and Qu, Y. H. and Yang, Z. and Wang, L. and Wang, Y. D.},

  abstractNote = {Promising multifunctional magnetoresponsive effects such as magnetoresistance, magnetostrain, and the magnetocaloric effect have recently been extensively studied in Ni-Mn-based metamagnetic shape memory alloys, but large reversible magnetoresponsive effects are usually obtained under high magnetic fields, which is an obstacle for practical applications. In this work, through manipulating magnetostructural transition, we achieved large reversible magnetoresponsive effects under a relatively low magnetic field of 3 T in a Ni-Co-Mn-In alloy. By systematically tuning the Mn/In ratio and Co substitution, an optimum composition Ni49Co3Mn34In14 with a low thermal hysteresis (8 K), a narrow transformation interval (7 K) and a high sensitivity of transformation temperature to field change (6KT-1), was obtained. Good geometric compatibility between austenite and martensite was revealed by in situ synchrotron high-energy x-ray diffraction experiment, which accounts for the low hysteresis and narrow transformation interval. A reversible transformation between pure austenite and pure martensite is induced by a relatively low field of 3 T, which was directly evidenced by in situ neutron diffraction experiments. As a result, a large reversible magnetocaloric effect with entropy change of 16.5Jkg-1K-1, a large reversible magnetostrain of 0.26%, and a large reversible magnetoresistance of 60%, under a relatively low field of 3 T, were simultaneously achieved. These reversible magnetoresponsive effects are comparable to the maximum reversible values obtained under high fields in other Ni-Mn-based alloys, but the magnetic field we applied is much lower. This research may guide the design of metamagnetic shape memory alloys with low-field-induced magnetoresponsive properties for magnetic refrigeration, magnetic sensing, and magnetic recording applications.},

  doi          = {10.1103/PhysRevMaterials.3.034404},

  journal      = {Physical Review Materials},

  number       = 3,

  volume       = 3,

  place        = {United States},

  year         = {Mon Mar 11 00:00:00 EDT 2019},

  month        = {Mon Mar 11 00:00:00 EDT 2019}

}

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Works referencing / citing this record:

Reversible low-field magnetocaloric effect in Ni-Mn-In-based Heusler alloys
journal, August 2019

Liu, Jun; You, Xinmin; Huang, Bowei
Physical Review Materials, Vol. 3, Issue 8
DOI: 10.1103/physrevmaterials.3.084409

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Title: Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

Abstract

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journal, January 2009

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journal, December 2009

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journal, May 2012

Metamagnetic shape memory effect in a Heusler-type Ni43Co7Mn39Sn11 polycrystalline alloy
journal, May 2006

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Ferromagnetism in the austenitic and martensitic states of $Ni − Mn − In$ alloys
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Tailoring barocaloric and magnetocaloric properties in low-hysteresis magnetic shape memory alloys
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Direct measurements of the magnetocaloric effect in pulsed magnetic fields: The example of the Heusler alloy Ni ₅₀ Mn ₃₅ In ₁₅
journal, February 2015

On the stress-assisted magnetic-field-induced phase transformation in Ni2MnGa ferromagnetic shape memory alloys
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Energy barriers and hysteresis in martensitic phase transformations
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journal, April 2018

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Inverse magnetocaloric effect in ferromagnetic Ni50Mn37+xSb13−x Heusler alloys
journal, March 2007

Effect of niobium addition on the martensitic transformation and magnetocaloric effect in low hysteresis NiCoMnSn magnetic shape memory alloys
journal, December 2014

Compositional instability of β-phase in Ni-Mn-Ga alloys
journal, February 1999

Cooling and heating by adiabatic magnetization in the ${Ni}_{50} {Mn}_{34} {In}_{16}$ magnetic shape-memory alloy
journal, May 2007

Thermomagnetic history dependence of magnetocaloric effect in Ni50Mn34In16
journal, January 2008

The Direct Conversion of Heat to Electricity Using Multiferroic Alloys
journal, December 2010

Boron’s effect on martensitic transformation and magnetocaloric effect in Ni43Mn46Sn11Bx alloys
journal, March 2008

Influence of annealing on magnetic field-induced structural transformation and magnetocaloric effect in Ni–Mn–In–Co ribbons
journal, September 2009

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journal, December 2009

Magnetic-field-induced strains in polycrystalline Ni-Mn-Ga at room temperature
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Large reversible entropy change at the inverse magnetocaloric effect in Ni-Co-Mn-Ga-In magnetic shape memory alloys
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Large magnetic‐field‐induced strains in Ni ₂ MnGa single crystals
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Martensitic transformation and mechanical properties of Ni49+xMn36–xIn15 (x=0, 0.5, 1.0, 1.5 and 2.0) alloys
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Large magnetic entropy change with small thermal hysteresis near room temperature in metamagnetic alloys Ni51Mn49−xInx
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journal, October 2006

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journal, July 2007

Determination of the entropy changes in the compounds with a first-order magnetic transition
journal, January 2007

Tuning martensitic transformation, large magnetoresistance and strain in Ni 50−x Fe x Mn 36 Sn 14 Heusler alloys
journal, September 2015

Asymmetric switchinglike behavior in the magnetoresistance at low fields in bulk metamagnetic Heusler alloys
journal, August 2014

Simultaneously achieved large reversible elastocaloric and magnetocaloric effects and their coupling in a magnetic shape memory alloy
journal, June 2018

Enhanced cyclability of elastocaloric effect in boron-microalloyed Ni-Mn-In magnetic shape memory alloys
journal, April 2017

Magnetic field-induced martensitic transformation and large magnetoresistance in NiCoMnSb alloys
journal, June 2007

Inverse magnetocaloric effect in ferromagnetic Ni–Mn–Sn alloys
journal, May 2005

Metamagnetic shape memory effect in polycrystalline NiCoMnSn alloy fabricated by spark plasma sintering
journal, September 2009

The applicability of CPP-GMR heads for magnetic recording
journal, September 2002

Direct measurement of large reversible magnetic-field-induced strain in Ni–Co–Mn–In metamagnetic shape memory alloys
journal, December 2012

Wombat: The high-intensity powder diffractometer at the OPAL reactor
journal, November 2006

Reduction of hysteresis losses in the magnetic refrigerant Gd5Ge2Si2 by the addition of iron
journal, June 2004

Microstructure in the cubic to monoclinic transition in titanium–nickel shape memory alloys
journal, July 1999

Reversibility of magnetostructural transition and associated magnetocaloric effect in Ni–Mn–In–Co
journal, September 2008

Entropy change linked to the martensitic transformation in metamagnetic shape memory alloys
journal, April 2012

Enhanced reversibility and unusual microstructure of a phase-transforming material
journal, October 2013

Large reversible magnetocaloric effect in Ni-Mn-In-Co
journal, January 2015

Entropy change and effect of magnetic field on martensitic transformation in a metamagnetic Ni–Co–Mn–In shape memory alloy
journal, May 2009

Magnetic properties and large magnetic-field-induced strains in off-stoichiometric Ni–Mn–Al Heusler alloys
journal, November 2000

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journal, August 2012

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journal, January 2016

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journal, August 2013

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journal, April 2016

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journal, April 2007

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journal, January 2010

Magnetocaloric effect in the low hysteresis Ni-Mn-In metamagnetic shape-memory Heusler alloy
journal, May 2014

Elevating the temperature regime of the large magnetocaloric effect in a Ni–Mn–In alloy towards room temperature
journal, March 2011

Magnetic superelasticity and inverse magnetocaloric effect in Ni-Mn-In
journal, March 2007

Giant and reversible room-temperature magnetocaloric effect in Ti-doped Ni-Co-Mn-Sn magnetic shape memory alloys
journal, August 2017

Low-field-actuated giant magnetocaloric effect and excellent mechanical properties in a NiMn-based multiferroic alloy
journal, March 2018

Large magnetic entropy change and magnetoresistance in a Ni41Co9Mn40Sn10 magnetic shape memory alloy
journal, October 2015

Large reversible magnetostrain in polycrystalline Ni50Mn33In17−xGax
journal, October 2016

Magnetocaloric effect in high Ni content Ni52Mn48−xInx alloys under low field change
journal, February 2012

Large magnetoresistance in single-crystalline Ni50Mn50−xInx alloys (x=14–16) upon martensitic transformation
journal, October 2006

Giant caloric effect of low-hysteresis metamagnetic shape memory alloys with exceptional cyclic functionality
journal, July 2017

Origin of anomalous cryogenic magnetic behavior in a Ni-Mn-based magnetic shape memory alloy
journal, March 2017

Magnetic-field-induced shape recovery by reverse phase transformation
journal, February 2006

Ultralow-fatigue shape memory alloy films
journal, May 2015

First-order nature of a metamagnetic transition and mechanism of giant magnetoresistance in ${Mn}_{2} {Sb}_{0.95} {Sn}_{0.05}$
journal, October 2004

Premartensitic transition and relevant magnetic effects in Ni50Mn34In15.5Al0.5 alloy
journal, May 2016

Large magnetoresistance in Ni50Mn34In16 alloy
journal, November 2006

Large reversible magnetostrain of a Ni30Cu8Co12Mn37Ga13 single crystal
journal, November 2016

Reversible low-field magnetocaloric effect in Ni-Mn-In-based Heusler alloys
journal, August 2019