Ultrafast extreme ultraviolet photoemission without space charge
Abstract
Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet (XUV) light have previously been limited by either space-charge effects, low photon flux, or limited tuning range. In this article, we describe XUV photoelectron spectroscopy experiments with up to 5 nA of average sample current using a tunable cavity-enhanced high-harmonic source operating at 88 MHz repetition rate. The source delivers >1011 photons/s in isolated harmonics to the sample over a broad photon energy range from 18 to 37 eV with a spot size of 58 × 100 μm2. From photoelectron spectroscopy data, we place conservative upper limits on the XUV pulse duration and photon energy bandwidth of 93 fs and 65 meV, respectively. In conclusion, the high photocurrent, lack of strong space charge distortions of the photoelectron spectra, and excellent isolation of individual harmonic orders allow us to observe laser-induced modifications of the photoelectron spectra at the 10–4 level, enabling time-resolved XUV photoemission experiments in a qualitatively new regime.
- Authors:
-
[3];
- Stony Brook Univ., Stony Brook, NY (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Stony Brook Univ., Stony Brook, NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1483745
- Alternate Identifier(s):
- OSTI ID: 1468879
- Report Number(s):
- BNL-209507-2018-JAAM
Journal ID: ISSN 2329-7778
- Grant/Contract Number:
- SC0012704; SC0016017
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Structural Dynamics
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 5; Journal ID: ISSN 2329-7778
- Publisher:
- American Crystallographic Association/AIP
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY
Citation Formats
Corder, Christopher, Zhao, Peng, Bakalis, Jin, Li, Xinlong, Kershis, Matthew D., Muraca, Amanda R., White, Michael G., and Allison, Thomas K. Ultrafast extreme ultraviolet photoemission without space charge. United States: N. p., 2018.
Web. doi:10.1063/1.5045578.
Corder, Christopher, Zhao, Peng, Bakalis, Jin, Li, Xinlong, Kershis, Matthew D., Muraca, Amanda R., White, Michael G., & Allison, Thomas K. Ultrafast extreme ultraviolet photoemission without space charge. United States. https://doi.org/10.1063/1.5045578
Corder, Christopher, Zhao, Peng, Bakalis, Jin, Li, Xinlong, Kershis, Matthew D., Muraca, Amanda R., White, Michael G., and Allison, Thomas K. Thu .
"Ultrafast extreme ultraviolet photoemission without space charge". United States. https://doi.org/10.1063/1.5045578. https://www.osti.gov/servlets/purl/1483745.
@article{osti_1483745,
title = {Ultrafast extreme ultraviolet photoemission without space charge},
author = {Corder, Christopher and Zhao, Peng and Bakalis, Jin and Li, Xinlong and Kershis, Matthew D. and Muraca, Amanda R. and White, Michael G. and Allison, Thomas K.},
abstractNote = {Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet (XUV) light have previously been limited by either space-charge effects, low photon flux, or limited tuning range. In this article, we describe XUV photoelectron spectroscopy experiments with up to 5 nA of average sample current using a tunable cavity-enhanced high-harmonic source operating at 88 MHz repetition rate. The source delivers >1011 photons/s in isolated harmonics to the sample over a broad photon energy range from 18 to 37 eV with a spot size of 58 × 100 μm2. From photoelectron spectroscopy data, we place conservative upper limits on the XUV pulse duration and photon energy bandwidth of 93 fs and 65 meV, respectively. In conclusion, the high photocurrent, lack of strong space charge distortions of the photoelectron spectra, and excellent isolation of individual harmonic orders allow us to observe laser-induced modifications of the photoelectron spectra at the 10–4 level, enabling time-resolved XUV photoemission experiments in a qualitatively new regime.},
doi = {10.1063/1.5045578},
journal = {Structural Dynamics},
number = 5,
volume = 5,
place = {United States},
year = {Thu Sep 06 00:00:00 EDT 2018},
month = {Thu Sep 06 00:00:00 EDT 2018}
}
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Time-Resolved Momentum Microscopy with a 1 MHz High-Harmonic Extreme Ultraviolet Beamline
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