Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation
Abstract
Light-emitting sources and devices permeate every aspect of our lives and are used in lighting, communications, transportation, computing, and medicine. Advances in multifunctional and “smart lighting” would require revolutionary concepts in the control of emission spectra and directionality. Such control might be possible with new schemes and regimes of light–matter interaction paired with developments in light-emitting materials. We show that all-dielectric metasurfaces made from III–V semiconductors with embedded emitters have the potential to provide revolutionary lighting concepts and devices, with new functionality that goes far beyond what is available in existing technologies. Specifically, we use Mie-resonant metasurfaces made from semiconductor heterostructures containing epitaxial quantum dots. By controlling the symmetry of the resonant modes, their overlap with the emission spectra, and other structural parameters, we can enhance the brightness by 2 orders of magnitude, as well as reduce its far-field divergence significantly.
- Authors:
-
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
- Friedrich Schiller Univ. Jena (Germany). Inst. of Applied Physics. Abbe Center of Photonics
- Univ. of New Mexico, Albuquerque, NM (United States). Center for High Technology Materials (CHTM)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA); LANL Laboratory Directed Research and Development (LDRD) Program; German Research Foundation (DFG); Thuringian State Government (Germany)
- OSTI Identifier:
- 1482014
- Report Number(s):
- LA-UR-18-28615
Journal ID: ISSN 1530-6984
- Grant/Contract Number:
- AC52-06NA25396; NA0003525; STA 1426/2-1
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 18; Journal Issue: 11; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; Material Science
Citation Formats
Liu, Sheng, Vaskin, Aleksandr, Addamane, Sadhvikas, Leung, Benjamin, Tsai, Miao-Chan, Yang, Yuanmu, Vabishchevich, Polina P., Keeler, Gordon A., Wang, George, He, Xiaowei, Kim, Younghee, Hartmann, Nicolai F., Htoon, Han, Doorn, Stephen K., Zilk, Matthias, Pertsch, Thomas, Balakrishnan, Ganesh, Sinclair, Michael B., Staude, Isabelle, and Brener, Igal. Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation. United States: N. p., 2018.
Web. doi:10.1021/acs.nanolett.8b02808.
Liu, Sheng, Vaskin, Aleksandr, Addamane, Sadhvikas, Leung, Benjamin, Tsai, Miao-Chan, Yang, Yuanmu, Vabishchevich, Polina P., Keeler, Gordon A., Wang, George, He, Xiaowei, Kim, Younghee, Hartmann, Nicolai F., Htoon, Han, Doorn, Stephen K., Zilk, Matthias, Pertsch, Thomas, Balakrishnan, Ganesh, Sinclair, Michael B., Staude, Isabelle, & Brener, Igal. Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation. United States. https://doi.org/10.1021/acs.nanolett.8b02808
Liu, Sheng, Vaskin, Aleksandr, Addamane, Sadhvikas, Leung, Benjamin, Tsai, Miao-Chan, Yang, Yuanmu, Vabishchevich, Polina P., Keeler, Gordon A., Wang, George, He, Xiaowei, Kim, Younghee, Hartmann, Nicolai F., Htoon, Han, Doorn, Stephen K., Zilk, Matthias, Pertsch, Thomas, Balakrishnan, Ganesh, Sinclair, Michael B., Staude, Isabelle, and Brener, Igal. Fri .
"Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation". United States. https://doi.org/10.1021/acs.nanolett.8b02808. https://www.osti.gov/servlets/purl/1482014.
@article{osti_1482014,
title = {Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation},
author = {Liu, Sheng and Vaskin, Aleksandr and Addamane, Sadhvikas and Leung, Benjamin and Tsai, Miao-Chan and Yang, Yuanmu and Vabishchevich, Polina P. and Keeler, Gordon A. and Wang, George and He, Xiaowei and Kim, Younghee and Hartmann, Nicolai F. and Htoon, Han and Doorn, Stephen K. and Zilk, Matthias and Pertsch, Thomas and Balakrishnan, Ganesh and Sinclair, Michael B. and Staude, Isabelle and Brener, Igal},
abstractNote = {Light-emitting sources and devices permeate every aspect of our lives and are used in lighting, communications, transportation, computing, and medicine. Advances in multifunctional and “smart lighting” would require revolutionary concepts in the control of emission spectra and directionality. Such control might be possible with new schemes and regimes of light–matter interaction paired with developments in light-emitting materials. We show that all-dielectric metasurfaces made from III–V semiconductors with embedded emitters have the potential to provide revolutionary lighting concepts and devices, with new functionality that goes far beyond what is available in existing technologies. Specifically, we use Mie-resonant metasurfaces made from semiconductor heterostructures containing epitaxial quantum dots. By controlling the symmetry of the resonant modes, their overlap with the emission spectra, and other structural parameters, we can enhance the brightness by 2 orders of magnitude, as well as reduce its far-field divergence significantly.},
doi = {10.1021/acs.nanolett.8b02808},
journal = {Nano Letters},
number = 11,
volume = 18,
place = {United States},
year = {Fri Oct 19 00:00:00 EDT 2018},
month = {Fri Oct 19 00:00:00 EDT 2018}
}
Web of Science
Figures / Tables:
Works referenced in this record:
Resonance Absorption by Nuclear Magnetic Moments in a Solid
journal, January 1946
- Purcell, E. M.; Torrey, H. C.; Pound, R. V.
- Physical Review, Vol. 69, Issue 1-2, p. 37-38
Exciton-Photon Strong-Coupling Regime for a Single Quantum Dot Embedded in a Microcavity
journal, August 2005
- Peter, E.; Senellart, P.; Martrou, D.
- Physical Review Letters, Vol. 95, Issue 6
Ultralow-threshold electrically pumped quantum-dot photonic-crystal nanocavity laser
journal, April 2011
- Ellis, Bryan; Mayer, Marie A.; Shambat, Gary
- Nature Photonics, Vol. 5, Issue 5
Coupling of quantum-dot light emission with a three-dimensional photonic-crystal nanocavity
journal, October 2008
- Aoki, Kanna; Guimard, Denis; Nishioka, Masao
- Nature Photonics, Vol. 2, Issue 11
Topological Nature of Optical Bound States in the Continuum
journal, December 2014
- Zhen, Bo; Hsu, Chia Wei; Lu, Ling
- Physical Review Letters, Vol. 113, Issue 25
Controlling multipolar radiation with symmetries for electromagnetic bound states in the continuum
journal, December 2014
- Lepetit, Thomas; Kanté, Boubacar
- Physical Review B, Vol. 90, Issue 24
Enabling enhanced emission and low-threshold lasing of organic molecules using special Fano resonances of macroscopic photonic crystals
journal, August 2013
- Zhen, Bo; Chua, Song-Liang; Lee, Jeongwon
- Proceedings of the National Academy of Sciences, Vol. 110, Issue 34
Probing the mechanisms of large Purcell enhancement in plasmonic nanoantennas
journal, October 2014
- Akselrod, Gleb M.; Argyropoulos, Christos; Hoang, Thang B.
- Nature Photonics, Vol. 8, Issue 11
Large spontaneous emission enhancement in plasmonic nanocavities
journal, May 2012
- Russell, Kasey J.; Liu, Tsung-Li; Cui, Shanying
- Nature Photonics, Vol. 6, Issue 7
Multifold Enhancement of Quantum Dot Luminescence in Plasmonic Metamaterials
journal, November 2010
- Tanaka, K.; Plum, E.; Ou, J. Y.
- Physical Review Letters, Vol. 105, Issue 22
Large single-molecule fluorescence enhancements produced by a bowtie nanoantenna
journal, October 2009
- Kinkhabwala, Anika; Yu, Zongfu; Fan, Shanhui
- Nature Photonics, Vol. 3, Issue 11, p. 654-657
Strong Enhancement of the Radiative Decay Rate of Emitters by Single Plasmonic Nanoantennas
journal, September 2007
- Muskens, O. L.; Giannini, V.; Sánchez-Gil, J. A.
- Nano Letters, Vol. 7, Issue 9
All-Dielectric Silicon Nanogap Antennas To Enhance the Fluorescence of Single Molecules
journal, July 2016
- Regmi, Raju; Berthelot, Johann; Winkler, Pamina M.
- Nano Letters, Vol. 16, Issue 8
Enhancement and Inhibition of Spontaneous Photon Emission by Resonant Silicon Nanoantennas
journal, December 2016
- Bouchet, Dorian; Mivelle, Mathieu; Proust, Julien
- Physical Review Applied, Vol. 6, Issue 6
Dielectric metasurfaces for complete control of phase and polarization with subwavelength spatial resolution and high transmission
journal, August 2015
- Arbabi, Amir; Horie, Yu; Bagheri, Mahmood
- Nature Nanotechnology, Vol. 10, Issue 11, p. 937-943
All-dielectric metamaterials
journal, January 2016
- Jahani, Saman; Jacob, Zubin
- Nature Nanotechnology, Vol. 11, Issue 1
Metalenses at visible wavelengths: Diffraction-limited focusing and subwavelength resolution imaging
journal, June 2016
- Khorasaninejad, Mohammadreza; Chen, Wei Ting; Devlin, Robert C.
- Science, Vol. 352, Issue 6290
Optically resonant dielectric nanostructures
journal, November 2016
- Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L.
- Science, Vol. 354, Issue 6314
Tailoring Directional Scattering through Magnetic and Electric Resonances in Subwavelength Silicon Nanodisks
journal, August 2013
- Staude, Isabelle; Miroshnichenko, Andrey E.; Decker, Manuel
- ACS Nano, Vol. 7, Issue 9, p. 7824-7832
Metamaterial-inspired silicon nanophotonics
journal, April 2017
- Staude, Isabelle; Schilling, Jörg
- Nature Photonics, Vol. 11, Issue 5
Mie resonance-based dielectric metamaterials
journal, December 2009
- Zhao, Qian; Zhou, Ji; Zhang, Fuli
- Materials Today, Vol. 12, Issue 12
Plasmonic Band Structure Controls Single-Molecule Fluorescence
journal, September 2013
- Langguth, Lutz; Punj, Deep; Wenger, Jérôme
- ACS Nano, Vol. 7, Issue 10
Shaping Photoluminescence Spectra with Magnetoelectric Resonances in All-Dielectric Nanoparticles
journal, January 2015
- Staude, Isabelle; Khardikov, Vyacheslav V.; Fofang, Nche T.
- ACS Photonics, Vol. 2, Issue 2
Directional and Spectral Shaping of Light Emission with Mie-Resonant Silicon Nanoantenna Arrays
journal, January 2018
- Vaskin, Aleksandr; Bohn, Justus; Chong, Katie E.
- ACS Photonics, Vol. 5, Issue 4
Active Tuning of Spontaneous Emission by Mie-Resonant Dielectric Metasurfaces
journal, April 2018
- Bohn, Justus; Bucher, Tobias; Chong, Katie E.
- Nano Letters, Vol. 18, Issue 6
Quantum Dot Emission Driven by Mie Resonances in Silicon Nanostructures
journal, October 2017
- Rutckaia, Viktoriia; Heyroth, Frank; Novikov, Alexey
- Nano Letters, Vol. 17, Issue 11
Strong Photoluminescence Enhancement in All-Dielectric Fano Metasurface with High Quality Factor
journal, September 2017
- Yuan, Shuai; Qiu, Xingzhi; Cui, Chengcong
- ACS Nano, Vol. 11, Issue 11
Transition between metamaterial and photonic-crystal behavior in arrays of dielectric rods
journal, January 2014
- Dominec, F.; Kadlec, C.; Němec, H.
- Optics Express, Vol. 22, Issue 25
Phase diagram for the transition from photonic crystals to dielectric metamaterials
journal, December 2015
- Rybin, Mikhail V.; Filonov, Dmitry S.; Samusev, Kirill B.
- Nature Communications, Vol. 6, Issue 1
Broken Symmetry Dielectric Resonators for High Quality Factor Fano Metasurfaces
journal, November 2016
- Campione, Salvatore; Liu, Sheng; Basilio, Lorena I.
- ACS Photonics, Vol. 3, Issue 12, p. 2362-2367
Multi-watt 1.25 [micro sign]m quantum dot VECSEL
journal, January 2010
- Albrecht, A. R.; Rotter, T. J.; Hains, C. P.
- Electronics Letters, Vol. 46, Issue 12
Low-threshold current density 1.3-μm InAs quantum-dot lasers with the dots-in-a-well (DWELL) structure
journal, June 2000
- Stintz, A.; Liu, G. T.; Li, H.
- IEEE Photonics Technology Letters, Vol. 12, Issue 6
III–V Semiconductor Nanoresonators—A New Strategy for Passive, Active, and Nonlinear All‐Dielectric Metamaterials
journal, June 2016
- Liu, Sheng; Keeler, Gordon A.; Reno, John L.
- Advanced Optical Materials, Vol. 4, Issue 10
Modified spontaneous emission in nanophotonic structures
journal, June 2015
- Pelton, Matthew
- Nature Photonics, Vol. 9, Issue 7
Efficient Source of Single Photons: A Single Quantum Dot in a Micropost Microcavity
journal, November 2002
- Pelton, Matthew; Santori, Charles; Vuc̆ković, Jelena
- Physical Review Letters, Vol. 89, Issue 23
Enhanced Spontaneous Emission by Quantum Boxes in a Monolithic Optical Microcavity
journal, August 1998
- Gérard, J.; Sermage, B.; Gayral, B.
- Physical Review Letters, Vol. 81, Issue 5
High-performance mid-infrared quantum dot infrared photodetectors
journal, June 2005
- Chakrabarti, S.; Stiff-Roberts, A. D.; Su, X. H.
- Journal of Physics D: Applied Physics, Vol. 38, Issue 13
Works referencing / citing this record:
Narrow Fano resonances in Si nanocylinder metasurfaces: Refractive index sensing
journal, May 2019
- Abujetas, Diego R.; Sáenz, Juan J.; Sánchez-Gil, José A.
- Journal of Applied Physics, Vol. 125, Issue 18
High- Quasibound States in the Continuum for Nonlinear Metasurfaces
journal, December 2019
- Liu, Zhuojun; Xu, Yi; Lin, Ye
- Physical Review Letters, Vol. 123, Issue 25
Resonant dielectric metasurfaces: active tuning and nonlinear effects
journal, July 2019
- Zou, Chengjun; Sautter, Jürgen; Setzpfandt, Frank
- Journal of Physics D: Applied Physics, Vol. 52, Issue 37
Ideal magnetic dipole resonances with metal-dielectric-metal hybridized nanodisks
journal, January 2019
- Zhang, Yao; Yue, Peng; Liu, Jun-Yan
- Optics Express, Vol. 27, Issue 11
All‐Dielectric Silicon Metasurface with Strong Subterahertz Toroidal Dipole Resonance
journal, July 2019
- Zografopoulos, Dimitrios C.; Ferraro, Antonio; Algorri, José Francisco
- Advanced Optical Materials, Vol. 7, Issue 19
Control of LED Emission with Functional Dielectric Metasurfaces
journal, November 2019
- Khaidarov, Egor; Liu, Zhengtong; Paniagua‐Domínguez, Ramón
- Laser & Photonics Reviews, Vol. 14, Issue 1
Interaction of semiconductor metasurfaces with short laser pulses: From nonlinear-optical response toward spatiotemporal shaping
journal, August 2019
- Shcherbakov, M. R.; Eilenberger, F.; Staude, I.
- Journal of Applied Physics, Vol. 126, Issue 8
Dielectric nanoantennas to manipulate solid-state light emission
journal, September 2019
- Bidault, Sébastien; Mivelle, Mathieu; Bonod, Nicolas
- Journal of Applied Physics, Vol. 126, Issue 9
Multiple toroidal dipole Fano resonances of asymmetric dielectric nanohole arrays
journal, November 2019
- Zhou, Chaobiao; Li, Shiyu; Wang, Yi
- Physical Review B, Vol. 100, Issue 19
Nonradiating photonics with resonant dielectric nanostructures
journal, March 2019
- Koshelev, Kirill; Favraud, Gael; Bogdanov, Andrey
- Nanophotonics, Vol. 8, Issue 5
Light-emitting metasurfaces
journal, July 2019
- Vaskin, Aleksandr; Kolkowski, Radoslaw; Koenderink, A. Femius
- Nanophotonics, Vol. 8, Issue 7
Fano resonant behaviour of waveguide mode in all-dielectric multilayer structure directly monitored by fluorescence of embedded dye molecules
journal, September 2019
- Kang, Byungjun; Motokura, Kengo; Fujii, Minoru
- Journal of Optics, Vol. 21, Issue 10
Active meta-optics and nanophotonics with halide perovskites
journal, September 2019
- Berestennikov, Alexander S.; Voroshilov, Pavel M.; Makarov, Sergey V.
- Applied Physics Reviews, Vol. 6, Issue 3
Controlling spontaneous emission via electronic correlations and temperature in transparent oxides
journal, December 2019
- Silva Neto, M. B.; Pinheiro, F. A.
- Physical Review B, Vol. 100, Issue 23
Beyond quantum confinement: excitonic nonlocality in halide perovskite nanoparticles with Mie resonances
journal, January 2019
- Berestennikov, A. S.; Li, Y.; Iorsh, I. V.
- Nanoscale, Vol. 11, Issue 14
Light emission driven by magnetic and electric toroidal dipole resonances in a silicon metasurface
journal, January 2019
- Cui, Chengcong; Yuan, Shuai; Qiu, Xingzhi
- Nanoscale, Vol. 11, Issue 30
Toroidal metasurface resonances in microwave waveguides
journal, May 2019
- Zografopoulos, Dimitrios C.; Algorri, José Francisco; Ferraro, Antonio
- Scientific Reports, Vol. 9, Issue 1
All-optical tuning of symmetry protected quasi bound states in the continuum
journal, September 2019
- Karl, Nicholas; Vabishchevich, Polina P.; Liu, Sheng
- Applied Physics Letters, Vol. 115, Issue 14
Monolayer MoS2 for nanoscale photonics
journal, February 2020
- Yang, Xianguang; Li, Baojun
- Nanophotonics, Vol. 9, Issue 7
Active meta-optics and nanophotonics with halide perovskites
preprint, January 2019
- Berestennikov, Alexander S.; Voroshilov, Pavel M.; Makarov, Sergey V.
- arXiv
Control of LED Emission with Functional Dielectric Metasurfaces
text, January 2019
- Khaidarov, Egor; Liu, Zhengtong; Paniagua-Dominguez, Ramon
- arXiv
Figures / Tables found in this record: